8-O - 16 ENDF/B-VI, Processed by Red Cullen using PREPRO2004 6000 0 0 0 8.01600E+3 1.58575E+1 0 0 0 3 825 1451 1 0.0 0.0 0 0 0 6 825 1451 2 1.00000E+0 3.00000E+7 8 0 10 6 825 1451 3 2.10000E+3 0.0 1 0 839 144 825 1451 4 8-O - 16 LANL EVAL-APR01 HALE,YOUNG,CHADWICK,CARO,LUBITZ 825 1451 5 Ch96ab,Ca98,Ch99,Yo01 DIST-SEP 1 REV2- 20011018 825 1451 6 ----ENDF/B-VI MATERIAL 825 825 1451 7 -----INCIDENT NEUTRON DATA 825 1451 8 ------ENDF-6 FORMAT 825 1451 9 825 1451 10 ****************************************************************** 825 1451 11 825 1451 12 ENDF/B-VI MOD 3 Evaluation, April 2001, P.G. Young, G.M. Hale 825 1451 13 M.B. Chadwick (LANL), E.Caro, C.R. Lubitz (KAPL) 825 1451 14 825 1451 15 This evaluation is a combination of a new MOD 3 evaluation 825 1451 16 below 30 MeV and the previous MOD 2 evaluation from 20 to 150 MeV. 825 1451 17 Both these evaluations are described below. The only change to the 825 1451 18 data above 30 MeV is to add tritium-production data, based on 825 1451 19 experimental yield data and spectra calculated with the GNASH 825 1451 20 Hauser-Feshbach/preequilibrium code. 825 1451 21 This evaluation provides a complete representation of the 825 1451 22 nuclear data needed for transport, damage, heating, radioactivity, 825 1451 23 and shielding applications over the incident neutron energy range 825 1451 24 from 1.0E-11 to 150 MeV. The discussion here is divided into the 825 1451 25 region above and below 30 MeV. 825 1451 26 825 1451 27 ------------------------------------------------------------------ 825 1451 28 825 1451 29 INCIDENT NEUTRON ENERGIES > 30 MeV 825 1451 30 825 1451 31 The evaluation above 30 MeV utilizes MF=6, MT=5 to represent 825 1451 32 all reaction data. Production cross sections and emission 825 1451 33 spectra are given for neutrons, protons, deuterons, alpha 825 1451 34 particles, gamma rays, and all residual nuclides produced (A>5) 825 1451 35 in the reaction chains. To summarize, the ENDF sections with 825 1451 36 non-zero data above En = 30 MeV are: 825 1451 37 825 1451 38 MF=3 MT= 1 Total Cross Section 825 1451 39 MT= 2 Elastic Scattering Cross Section 825 1451 40 MT= 3 Nonelastic Cross Section 825 1451 41 MT= 5 Sum of Binary (n,n') and (n,x) Reactions 825 1451 42 MT=102 Radiative Capture Cross Section (Estimate Only) 825 1451 43 825 1451 44 MF=4 MT= 2 Elastic Angular Distributions 825 1451 45 825 1451 46 MF=6 MT= 5 Production Cross Sections and Energy-Angle 825 1451 47 Distributions for Emission Neutrons, Protons, 825 1451 48 Deuterons, and Alphas; and Angle-Integrated 825 1451 49 Spectra for Gamma Rays and Residual Nuclei That 825 1451 50 Are Stable Against Particle Emission 825 1451 51 825 1451 52 The evaluation is based on nuclear model calculations that 825 1451 53 have been benchmarked to experimental data, especially for n + 825 1451 54 O16 and p + O16 reactions [Ch96a]. We use the GNASH code system 825 1451 55 [Yo92], which utilizes Hauser-Feshbach statistical, preequi- 825 1451 56 librium and direct-reaction theories. Coupled-channel and 825 1451 57 spherical optical model calculations are used to obtain particle 825 1451 58 transmission coefficients for the Hauser-Feshbach calculations, 825 1451 59 as well as for the elastic neutron angular distributions. 825 1451 60 Cross sections and spectra for producing individual residual 825 1451 61 nuclei are included for reactions that exceed a cross section of 825 1451 62 approximately 1 nb at any energy. The energy-angle-correlations 825 1451 63 for all outgoing particles are based on Kalbach systematics 825 1451 64 [Ka88]. 825 1451 65 A model was developed to calculate the energy distributions of 825 1451 66 all recoil nuclei in the GNASH calculations [Ch96b]. The recoil 825 1451 67 energy distributions are represented in the laboratory system in 825 1451 68 MT=5, MF=6, and are given as isotropic in the lab system. Note 825 1451 69 that all other data in MT=5,MF=6 are given in the center-of-mass 825 1451 70 system. This method of representation requires a modification of 825 1451 71 the original ENDF-6 format. 825 1451 72 Preequilibrium corrections were performed in the course of the 825 1451 73 GNASH calculations using either Feshbach, Kerman, Koonin (FKK) 825 1451 74 theory [Ch93] or the exciton model of Kalbach [Ka77, Ka85]. 825 1451 75 Discrete level data from nuclear data sheets were matched to 825 1451 76 continuum level densities using the formulation of Ignatyuk 825 1451 77 [Ig75] and pairing and shell parameters from the Cook [Co67] 825 1451 78 analysis. Neutron and charged-particle transmission coefficients 825 1451 79 were obtained from the optical potentials, as discussed below. 825 1451 80 Gamma-ray transmission coefficients were calculated using the 825 1451 81 Kopecky-Uhl model [Ko90]. 825 1451 82 825 1451 83 ------------------------------------------------------------------ 825 1451 84 825 1451 85 INCIDENT NEUTRON ENERGIES < 30 MeV 825 1451 86 825 1451 87 The evaluation below 30 MeV includes complete data for all 825 1451 88 significant neutron-induced reactions. It is comprised of 825 1451 89 R-parameter [Ca98] and R-matrix analyses below 6.25 MeV, and a 825 1451 90 combination of experimental and theoretical data evaluation 825 1451 91 from 6.25 to 30 MeV. A summary of the evaluation by energy 825 1451 92 range is given below, followed by a detailed description of 825 1451 93 the evaluation, reaction by reaction. 825 1451 94 825 1451 95 NEUTRON ENERGY < 6.25 MeV 825 1451 96 825 1451 97 The evaluation below 3.4 MeV is an R-function fit [Ca98] to 825 1451 98 experimental data. At 3.4 MeV, it is spliced to the LANL R-matrix 825 1451 99 analysis with a transition region of about 60 keV centered at 825 1451 100 3.4 MeV. The LANL analysis is used for the region from 3.40 to 825 1451 101 6.25 MeV. 825 1451 102 825 1451 103 NEUTRON ENERGY > 6.25 MeV 825 1451 104 825 1451 105 The following major modifications were made above 6.25 MeV: 825 1451 106 1. The maximum energy of the evaluation was increased from 20 to 825 1451 107 30 MeV. 825 1451 108 2. New measurements of 16O(n,xgamma) angular distributions (7 825 1451 109 angles, En = 4 - 200 MeV) by Nelson et al. [Ne99] were incor- 825 1451 110 porated into the evaluation. The measurements use a high- 825 1451 111 resolution Ge detector and result in data for some 21 gamma rays. 825 1451 112 The distributions were fit with Legendre expansions to obtain 825 1451 113 angle-integrated cross sections for MF=13 and angular 825 1451 114 distributions for MF=14. Nuclear energy level schemes and gamma 825 1451 115 branching ratios [Aj86,Aj91] were utilized to extract level 825 1451 116 excitation cross sections in MF=3 for discrete states in 16O, 825 1451 117 14-16N, and 13C, corresponding to (n,n'), (n,p), (n,d), (n,t), 825 1451 118 and (n,alpha) reactions. 825 1451 119 3. New measurements of 16O(n,alpha) cross sections at 14 MeV by 825 1451 120 Sanami and Baba [Sa97] were used to adjust the (n,alpha) cross 825 1451 121 sections. 825 1451 122 4. The neutron total cross section measurements of Finlay [Fi93] 825 1451 123 were incorporated into the evaluation above 7.3 MeV. Adjustments 825 1451 124 of up to 2% were made in the existing evaluation. 825 1451 125 5. The new evaluation contains no pseudo level or excitation 825 1451 126 energy bin data. Calculations were made with the GNASH code to 825 1451 127 provide continuum emission data in MF=6 format, as well as any 825 1451 128 unmeasured data. Calculated cross sections were renormalized 825 1451 129 whenever possible using experimental data. The GNASH calculations 825 1451 130 utilized transmission coefficients calculated with a spherical 825 1451 131 optical potential and level densities from the Gilbert and 825 1451 132 Cameron model, plus preequilibrium corrections using systematic 825 1451 133 values of parameters. 825 1451 134 6. Comparisons of the evaluation with a large body of 825 1451 135 experimental data have been made to validate the new data. 825 1451 136 825 1451 137 ------------------------------------------------------------------ 825 1451 138 825 1451 139 DETAILED DESCRIPTION REACTION BY REACTION 825 1451 140 825 1451 141 MF=2 RESONANCE PARAMETERS ------------------------------------- 825 1451 142 825 1451 143 The evaluation below 3.4 MeV is an R-function fit [Ca98] to 825 1451 144 experimental data using an optical model to provide a background 825 1451 145 R-function. The procedure is coded in the KAPL code "OPTIC", 825 1451 146 with an extension of the original code to convert the optical- 825 1451 147 model phase shifts to background R-functions. 825 1451 148 The analysis is carried to 3.4 MeV, where it is spliced to the 825 1451 149 LANL R-matrix analysis, with a transition region of about 60 keV 825 1451 150 centered at 3.4 MeV. 825 1451 151 From 3.4 to 6.25 MeV, a test evaluation was obtained from a new 825 1451 152 multi-channel R-matrix analysis of a large part of the available 825 1451 153 experimental data base using the EDA code. The analysis of the 825 1451 154 17O system includes data for n+16O neutron total cross sections 825 1451 155 and elastic scattering angular distributions, as well as data 825 1451 156 for the 16O(n,alpha) reaction in both the (n,alpha) and 825 1451 157 (alpha,n) directions. Also included are excitation functions 825 1451 158 for alpha+13C elastic scattering. The total cross sections in 825 1451 159 the final version of this analysis may change, especially in the 825 1451 160 region above 4 MeV. 825 1451 161 825 1451 162 Effective scattering radius = 5.56256E-13 cm. 825 1451 163 825 1451 164 MF=3 NEUTRON CROSS SECTIONS ----------------------------------- 825 1451 165 825 1451 166 THERMAL (2200 m/s) CROSS SECTIONS 825 1451 167 825 1451 168 TOTAL = 3.89440 B RADIATIVE CAPTURE= 0.1900 MB 825 1451 169 ELASTIC= 3.89421 B 825 1451 170 825 1451 171 MT=1 TOTAL CROSS SECTION 825 1451 172 0.0 to 3.40 MeV, calculated from R-function fit to total cross 825 1451 173 section and elastic angular distributions - see above. 825 1451 174 3.4 to 6.25 MeV, calculated from R-Matrix parameters by 825 1451 175 simultaneously fitting most of the available 16O(n,n)16O and 825 1451 176 16O(n,alpha0)13C data, as well as 13C(alpha,alpha)13C data at 825 1451 177 energies below En = 6.2 MeV. The experimental total cross 825 1451 178 section data fitted in the analysis were the [Jo74] results below 825 1451 179 6.26 MeV, and the [La80] measurements at higher energies, with 825 1451 180 inserts of the high-resolution data of [Jo79] over the resonances 825 1451 181 and in the window at En = 2.3-2.4 MeV. 825 1451 182 6.25 to 30 MeV, based on an adjustment of the covariance 825 1451 183 analysis used for the ENDF/B-VI (Rel. 0) evaluation to 825 1451 184 accommodate the new measurements of Finlay et al. [Fi93]. The 825 1451 185 previous ENDF/B-VI (Rel. 0) evaluations is based on analysis 825 1451 186 with the GLUCS Bayes code [He80] of the remaining major total 825 1451 187 cross section measurements [Fo71], [Pe72], [Sc72], [La80], 825 1451 188 [Ci68], [Ci80], with structure inserted from the high-resolution 825 1451 189 [Ci80] measurement. 825 1451 190 825 1451 191 MT=2 ELASTIC SCATTERING CROSS SECTION 825 1451 192 0.0 to 3.40 MeV, calculated from R-function fit to total cross 825 1451 193 section and elastic angular distributions - see above. 825 1451 194 3.4 to 6.25 MeV, R-matrix analysis that includes all available 825 1451 195 experimental data, as described above. Elastic angular 825 1451 196 distribution data used in the analysis includes [La60], [Ok55], 825 1451 197 [Fo58], [Ma62], [Fo70], [Hu62], [Ph61], [Jo67], [Ki72], [Ch61], 825 1451 198 [Dr76], [Fo64]. 825 1451 199 6.25 to 20 MeV, obtained by subtracting the nonelastic cross 825 1451 200 section (MT=3) from the total cross section (MT=1), although 825 1451 201 small adjustments were made to several of the less well 825 1451 202 determined reaction cross sections in order to enhance agreement 825 1451 203 with the elastic measurements of Borker [Bo89], Glendinning 825 1451 204 [Gl82], and Petler [Pe85]. The magnitude of these adjustments 825 1451 205 was generally small and was greatest near structure and near 825 1451 206 18 MeV. 825 1451 207 825 1451 208 MT=4 INELASTIC CROSS SECTION 825 1451 209 Threshold to 30 MeV, sum of MT=51-57, 91. 825 1451 210 825 1451 211 MT=51-57 INELASTIC CROSS SECTION TO DISCRETE STATES 825 1451 212 Threshold to 30 MeV, the (n,n') cross sections corresponding 825 1451 213 to gamma-emitting excited levels of 16O are included in MT=51-57 825 1451 214 as follows: 825 1451 215 MT=51 Ex= 6.0494 MeV 825 1451 216 MT=52 Ex= 6.129893 MeV 825 1451 217 MT=53 Ex= 6.9171 MeV 825 1451 218 MT=54 Ex= 7.11685 MeV 825 1451 219 MT=55 Ex= 8.8719 MeV 825 1451 220 MT=56 Ex=10.957 MeV 825 1451 221 MT=57 Ex=11.080 MeV 825 1451 222 825 1451 223 Note that the 16O levels at 9.585, 9.8445, and 10.356 are 825 1451 224 omitted because they decay primarily by alpha particle emission 825 1451 225 and those data are included in MT=22. 825 1451 226 825 1451 227 MT=16 (N,2N) CROSS SECTION 825 1451 228 Threshold to 30 MeV, based on GNASH calculation, renormalized 825 1451 229 down by approximately 30% to improve agreement with measurement 825 1451 230 of Brill et al. [Br61]. 825 1451 231 825 1451 232 MT=22 (N,NALPHA) CROSS SECTION 825 1451 233 Threshold to 30 MeV, based on GNASH calculation, with 825 1451 234 adjustments made to improve agreement with experimental data, 825 1451 235 especially data of Bormann et al. [Bo63]. 825 1451 236 825 1451 237 MT=23 (N,N3ALPHA) CROSS SECTION 825 1451 238 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 239 from 28 to 30 MeV to agree with LA150 data. 825 1451 240 825 1451 241 MT=28 (N,NP) CROSS SECTION 825 1451 242 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 243 such that the production cross sections for the 5.2701 and 5.2988 825 1451 244 MeV gamma rays are consistent with Nelson et al.[Ne99] data, and 825 1451 245 normalization of proton spectra consistent with 27-MeV data of 825 1451 246 Subramanian et al. [Su94]. 825 1451 247 825 1451 248 MT=32 (N,ND) CROSS SECTION 825 1451 249 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 250 such that difference between total and nonelastic cross sections 825 1451 251 agrees with elastic cross section measurements. 825 1451 252 825 1451 253 MT=41 (N,2NP) CROSS SECTION 825 1451 254 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 255 such that difference between total and nonelastic cross sections 825 1451 256 agrees with elastic cross section measurements. 825 1451 257 825 1451 258 MT=44 (N,N2P) CROSS SECTION 825 1451 259 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 260 such that difference between total and nonelastic cross sections 825 1451 261 agrees with elastic cross section measurements. 825 1451 262 825 1451 263 MT=45 (N,NPALPHA) CROSS SECTION 825 1451 264 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 265 such that difference between total and nonelastic cross sections 825 1451 266 agrees with elastic cross section measurements. 825 1451 267 825 1451 268 MT=91 (N,N'CONTINUUM) CROSS SECTION 825 1451 269 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 270 such that difference between total and nonelastic cross sections 825 1451 271 agrees with elastic cross section measurements. 825 1451 272 825 1451 273 MT=102 (N,GAMMA) CROSS SECTION 825 1451 274 0 to 1 MeV,cross section based on experimental data obtained 825 1451 275 from E. Jurney [Ju64]; higher energy data is crude estimate. 825 1451 276 825 1451 277 MT=103 (N,P) CROSS SECTION 825 1451 278 Sum of MT=600-603. 825 1451 279 825 1451 280 MT=104 (N,D) CROSS SECTION 825 1451 281 Sum of MT=650-669. 825 1451 282 825 1451 283 MT=105 (N,T) CROSS SECTION 825 1451 284 Sum of MT=700-709,749. 825 1451 285 825 1451 286 MT=107 (N,ALPHA) CROSS SECTION 825 1451 287 Sum of MT=800-803. 825 1451 288 825 1451 289 MT=108 (N,2ALPHA) CROSS SECTION 825 1451 290 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 291 such that difference between total and nonelastic cross sections 825 1451 292 agrees with elastic cross section measurements. 825 1451 293 825 1451 294 MT=112 (N,PALPHA) CROSS SECTION 825 1451 295 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 296 such that difference between total and nonelastic cross sections 825 1451 297 agrees with elastic cross section measurements. 825 1451 298 825 1451 299 MT=600 (N,P) INTEGRATED CROSS SECTION TO 16N GROUND STATE 825 1451 300 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 301 renormalization (lowered approximately 30%) from comparison of 825 1451 302 excited state predictions with Nelson et al. [Ne99] 825 1451 303 measurements. 825 1451 304 825 1451 305 MT=601-603 (N,P) CROSS SECTION TO EXCITED LEVELS OF 16N 825 1451 306 Threshold to 30 MeV, the cross sections for the 0.0.297- and 825 1451 307 0.3975-MeV levels are inferred from the (n,p gamma) data of 825 1451 308 Nelson et al. [Ne99], using the level structure diagram of 16N 825 1451 309 by Ajzenberg-Selove [Aj86]. The cross section for the 0.1201- 825 1451 310 MeV level is based on GNASH calculations with some 825 1451 311 renormalization (lowered ~30%) from comparison of excited state 825 1451 312 predictions with Nelson et al. [Ne99] measurements. 825 1451 313 825 1451 314 MT=650 (N,D) INTEGRATED CROSS SECTION TO 15N GROUND STATE 825 1451 315 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 316 renormalization from comparison of excited state predictions 825 1451 317 with Nelson et al. [Ne99] measurements. 825 1451 318 825 1451 319 MT=651-669 (N,D) CROSS SECTION TO EXCITED LEVELS OF 15N 825 1451 320 Threshold to 30 MeV, the cross sections for the 5.2701- and 825 1451 321 5.2988-MeV levels are adjusted based on the (n,xgamma) data of 825 1451 322 Nelson et al. [Ne99], using the level structure diagram for 15N 825 1451 323 by Ajzenberg-Selove [Aj91]. Cross sections for remaining levels 825 1451 324 are based on GNASH calculations with some renormalization from 825 1451 325 comparison of excited state predictions with Nelson et al. 825 1451 326 [Ne99] measurements and 27-Mev data of Subramanian et al. [Su94]. 825 1451 327 825 1451 328 MT=700 (N,T) INTEGRATED CROSS SECTION TO 14N GROUND STATE 825 1451 329 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 330 renormalization from comparison of excited state predictions 825 1451 331 with Nelson et al. [Ne99] measurements. 825 1451 332 825 1451 333 MT=701-709 (N,T) CROSS SECTION TO EXCITED LEVELS OF 14N 825 1451 334 Threshold to 30 MeV, the cross section for the 2.3128-MeV 825 1451 335 levels is inferred from the (n,t gamma) data of Nelson et al. 825 1451 336 [Ne99], using the level structure diagram for 16N by Ajzenberg- 825 1451 337 Selove [Aj91]. Cross sections for the remaining levels are 825 1451 338 based on GNASH calculations with some renormalization from 825 1451 339 comparison of excited state predictions with Nelson et al. 825 1451 340 [Ne99] measurements. 825 1451 341 825 1451 342 MT=749 (N,T) CROSS SECTION TO 14N CONTINUUM 825 1451 343 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 344 renormalization from comparison of excited state predictions 825 1451 345 with Nelson et al. [Ne99] measurements and to enhance agreement 825 1451 346 of elastic cross section with measured data. 825 1451 347 825 1451 348 MT=800 (N,ALPHA0) CROSS SECTION TO 13C GROUND STATE 825 1451 349 0.0 to 6.2 MeV, based on R-matrix analysis described above 825 1451 350 under MT=1. Data of Ba72 were used in the original (alpha,n) 825 1451 351 direction, with no changes in energy scale or normalization. 825 1451 352 Also included were the low-energy (alpha,n) data of [Ke91] and 825 1451 353 [Dr93]. 825 1451 354 6.2 to 20 MeV, based on data of [Da63],[Da68],[Si68],[Ba73], 825 1451 355 and composite of [Mc66b],[Ma68],[Le68] at 14 MeV. Note that the 825 1451 356 [Da63] data were renormalized by factor of 1.5 to bring them 825 1451 357 into rough agreement with the R-matrix analysis of the [Ba73] 825 1451 358 (n,a0) data, together with the total and elastic data in the 825 1451 359 analysis. Because the [Da68] experimental data were normalized 825 1451 360 to [Da63], the former were also renormalized by the factor of 825 1451 361 1.5. 825 1451 362 825 1451 363 MT=801-803 (N,ALPHA) CROSS SECTION TO EXCITED LEVELS OF 13C 825 1451 364 Threshold to 30 MeV, the cross sections of the 3.0894-, 825 1451 365 3.6845-, and 3.8538-MeV levels are inferred from the (n,alpha 825 1451 366 gamma) data of Nelson et al. [Ne99], using the level structure 825 1451 367 diagram of 13C by Ajzenberg-Selove [Aj91]. 825 1451 368 825 1451 369 MF=4 ANGULAR DISTRIBUTIONS ------------------------------------ 825 1451 370 825 1451 371 MT=2 ELASTIC NEUTRON ANGULAR DISTRIBUTIONS 825 1451 372 0.0 to 3.4 MeV, calculated from R-function fit (see MF=3,MT=1). 825 1451 373 3.4 to 6.2 MeV, calculated from R-matrix fit (see MF=3,MT=1). 825 1451 374 Measured angular distributions input to the fit were those of 825 1451 375 [Ch61],[Fo58],[Fo70],[Hi58],[Hu62], [Jo67],[Ki72],[La60],[Li66], 825 1451 376 [Ma62],[Ph61],[Jo79]. Fits were attempted using new data of 825 1451 377 [Sc77], but those measurements were found to have significant 825 1451 378 uncertainties, and some discrepancies with other data were noted. 825 1451 379 6.2 to 20 MeV, smooth curve through coefficients derived from 825 1451 380 fits to elastic data of [Ph61],[Ne72],[Ch61],[Ba63],[Be67], 825 1451 381 [Mc66a],[Ki72],[Bu73],[Ne72],[Gl82],[Ba85],[Bo89],[Pe85]. 825 1451 382 825 1451 383 MT=51-57 DISCRETE (N,N') ANGULAR DISTRIBUTIONS 825 1451 384 Threshold to 10 MeV, assumed isotropic in center of mass. 825 1451 385 Above 10 MeV, based on fits of the 14-MeV data of [Ki72],[Ne72], 825 1451 386 [Ba63],[Mc66a],[Ba85],[Me69], and especially [Bo89]. 825 1451 387 825 1451 388 MT=600-603 DISCRETE (N,P) ANGULAR DISTRIBUTIONS 825 1451 389 Threshold to 30 MeV, assumed isotropic in center of mass. 825 1451 390 825 1451 391 MT=650-669 DISCRETE (N,D) ANGULAR DISTRIBUTIONS 825 1451 392 Threshold to 30 MeV, assumed isotropic in center of mass. 825 1451 393 825 1451 394 MT=700-709 DISCRETE (N,T) ANGULAR DISTRIBUTIONS 825 1451 395 Threshold to 30 MeV, assumed isotropic in center of mass. 825 1451 396 825 1451 397 MT=800 DISCRETE(N,ALPHA0) ANGULAR DISTRIBUTIONS 825 1451 398 0.0 to 6.2 MeV, calculated from R-Matrix fit (see MF=3,MT=1). 825 1451 399 Measured angular distributions input to the fit were 825 1451 400 reconstructed from the Legendre coefficients of [Wa57], and 825 1451 401 converted to (n,alpha) angular distributions using detailed 825 1451 402 balance. 825 1451 403 825 1451 404 MT=801-803 DISCRETE (N,T) ANGULAR DISTRIBUTIONS 825 1451 405 Threshold to 6 MeV, 825 1451 406 6 to 30 MeV, assumed isotropic in center of mass. 825 1451 407 825 1451 408 MF=6 PRODUCT ENERGY-ANGLE DISTRIBUTIONS ----------------------- 825 1451 409 825 1451 410 MT=16 (N,2N) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 411 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 412 are given for neutrons, and isotropic energy spectra are given 825 1451 413 for recoiling 15O nuclei. The neutron data were obtained from 825 1451 414 the GNASH calculations; the recoil 15O distributions were 825 1451 415 calculated with the RECOIL code [Ma83]. The discrete gamma rays 825 1451 416 from (n,2ngamma) reactions are given in MF=13 and 14. 825 1451 417 825 1451 418 MT=22 (N,NALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 419 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 420 are given for neutrons and alpha particles, and isotropic energy 825 1451 421 spectra are given for recoiling 12C nuclei. The neutron and 825 1451 422 alpha data were obtained from the GNASH calculations; the recoil 825 1451 423 12C distributions were calculated with the RECOIL code [Ma83]. 825 1451 424 The discrete gamma rays from (n,nalpha gamma) reactions are 825 1451 425 given in MF=13 and 14. 825 1451 426 825 1451 427 MT=28 (N,NP) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 428 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 429 are given for neutrons and protons; isotropic energy spectra are 825 1451 430 given for recoiling 15N nuclei; and isotropic energy spectra are 825 1451 431 given for emitted continuum gamma rays. The neutron, proton, 825 1451 432 and gamma-ray data were obtained from the GNASH calculations; 825 1451 433 the recoil 15N distributions were calculated with the RECOIL 825 1451 434 code [Ma83]. 825 1451 435 825 1451 436 MT=32 (N,ND) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 437 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 438 are given for neutrons and deuterons; isotropic energy spectra 825 1451 439 are given for recoiling 14N nuclei; and isotropic energy spectra 825 1451 440 are given for emitted continuum gamma rays. The neutron, 825 1451 441 deuteron, and gamma-ray data were obtained from the GNASH 825 1451 442 calculations; the recoil 14N distributions were calculated with 825 1451 443 the RECOIL code [Ma83]. 825 1451 444 825 1451 445 MT=41 (N,2NP) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 446 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 447 are given for neutrons and protons; isotropic energy spectra are 825 1451 448 given for recoiling 14N nuclei; and isotropic energy spectra are 825 1451 449 given for emitted continuum gamma rays. The neutron, proton, 825 1451 450 and gamma-ray data were obtained from the GNASH calculations; 825 1451 451 the recoil 14N distributions were calculated with the RECOIL 825 1451 452 code [Ma83]. 825 1451 453 825 1451 454 MT=44 (N,N2P) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 455 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 456 are given for neutrons and protons; isotropic energy spectra are 825 1451 457 given for recoiling 14C nuclei; and isotropic energy spectra are 825 1451 458 given for emitted continuum gamma rays. The neutron, proton, 825 1451 459 and gamma-ray data were obtained from the GNASH calculations; 825 1451 460 the recoil 14C distributions were calculated with the RECOIL 825 1451 461 code [Ma83]. 825 1451 462 825 1451 463 MT=45 (N,NPALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 464 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 465 are given for neutrons, protons, and alphas; isotropic energy 825 1451 466 spectra are given for recoiling 11B nuclei; and isotropic energy 825 1451 467 spectra are given for emitted continuum gamma rays. The 825 1451 468 neutron, proton, alpha, and gamma-ray data were obtained from 825 1451 469 the GNASH calculations; the recoil 11B distributions were 825 1451 470 calculated with the RECOIL code [Ma83]. 825 1451 471 825 1451 472 MT=91 (N,N'CONTINUUM) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 473 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 474 are given for neutrons; isotropic energy spectra are given for 825 1451 475 recoiling 16O nuclei; and isotropic energy spectra are given for 825 1451 476 emitted continuum gamma rays. The neutron and gamma-ray data 825 1451 477 were obtained from the GNASH calculations; the recoil 16O 825 1451 478 distributions were calculated with the RECOIL code [Ma83]. 825 1451 479 825 1451 480 MT=108 (N,2ALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 481 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 482 are given for alphas; isotropic energy spectra are given for 825 1451 483 recoiling 9Be nuclei; and isotropic energy spectra are given for 825 1451 484 emitted continuum gamma rays. The alpha, and gamma-ray data 825 1451 485 were obtained from the GNASH calculations; the recoil 9Be 825 1451 486 distributions were calculated with the RECOIL code [Ma83]. 825 1451 487 825 1451 488 MT=112 (N,PALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 489 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 490 are given for protons, and alphas; isotropic energy spectra are 825 1451 491 given for recoiling 12B nuclei; and isotropic energy spectra are 825 1451 492 given for emitted continuum gamma rays. The proton, alpha, and 825 1451 493 gamma-ray data were obtained from the GNASH calculations; the 825 1451 494 recoil 12B distributions were calculated with the RECOIL code 825 1451 495 [Ma83]. 825 1451 496 825 1451 497 MT=749 (N,ALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 498 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 499 are given for alpha particles; isotropic energy spectra are 825 1451 500 given for recoiling 13C nuclei; and isotropic energy spectra are 825 1451 501 given for emitted continuum gamma rays. The alpha and gamma-ray 825 1451 502 data were obtained from the GNASH calculations; the recoil 13C 825 1451 503 distributions were calculated with the RECOIL code [Ma83]. 825 1451 504 825 1451 505 MF=12 PHOTON PRODUCTION MULTIPLICITIES ------------------------ 825 1451 506 825 1451 507 MT=102 (N,GAMMA) PHOTON PRODUCTION MULTIPLICITIES 825 1451 508 Photon multiplicities for radiative capture are based on 825 1451 509 experimental data obtained from Jurney [Ju64]. 825 1451 510 825 1451 511 MF=13 PHOTON PRODUCTION CROSS SECTIONS ------------------------ 825 1451 512 825 1451 513 MT=4 (N,N'GAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 514 Threshold to 30 MeV: Based almost entirely on new angular 825 1451 515 distribution measurements by Nelson et al. [Ne99], which 825 1451 516 utilized a white neutron source and covered the energy range 825 1451 517 from threshold to 200 MeV. The measurements were made at 7 825 1451 518 angles using high-resolution Ge detectors and resulted in data 825 1451 519 for some 23 gamma rays from 7 different reactions. The angular 825 1451 520 distributions were fit with Legendre expansions to obtain angle- 825 1451 521 integrated cross sections. The fitted cross sections were 825 1451 522 smoothed somewhat for this evaluation, although much of the 825 1451 523 measured structure was preserved, particularly for the intense 825 1451 524 6.129-MeV gamma. The evaluated data for the following gamma 825 1451 525 rays are based directly on the measurements: 825 1451 526 825 1451 527 EG= 2.742 MeV (decay of 8.8719-MeV level of 16O) 825 1451 528 EG= 3.839 MeV (decay of 10.957-MeV level of 16O) 825 1451 529 EG= 4.950 MeV (decay of 11.080-MeV level of 16O) 825 1451 530 EG= 6.130 MeV (decay of 6.130-MeV level of 16O) 825 1451 531 EG= 6.917 MeV (decay of 6.917-MeV level of 16O) 825 1451 532 EG= 7.117 MeV (decay of 7.117-MeV level of 16O) 825 1451 533 825 1451 534 The evaluated cross sections for the remaining (n,n') gamma 825 1451 535 rays are inferred from these data using the energy level scheme 825 1451 536 of Ajzenberg-Selove [Aj86]. Data were also obtained for gamma 825 1451 537 rays of energy 1.755 and 1.955 from decay of the 8.8719-MeV 825 1451 538 level but the 2.742-MeV gamma was used to determine the level 825 1451 539 excitation cross section because it is the most intense. 825 1451 540 Similarly, data were obtained on a 4.179-MeV gamma from decay of 825 1451 541 the 11.080-MeV level, but the 4.950-MeV gamma is more intense 825 1451 542 and was used to determine the level excitation cross section. 825 1451 543 The evaluated data were compared to older gamma-ray 825 1451 544 measurements by [Be70], [Ne90], [No78], [Ha59], [Di70], [Or70], 825 1451 545 [Dr70], [Cl69], [Lu70], [Bu71], [Ny69]. Considering that very 825 1451 546 few (e.g., [Be70], [Dr70]) of these measurements are of full 825 1451 547 angular distributions, the agreement is reasonable. 825 1451 548 825 1451 549 MT=16 (N,2NGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 550 Threshold to 30 MeV: The cross section for the 5.2409-MeV 825 1451 551 gamma ray was obtained directly from the Nelson et al. [Ne99] 825 1451 552 data. The remaining discrete gammas are based on GNASH 825 1451 553 calculations, with some renomalization based on the experimental 825 1451 554 data. 825 1451 555 825 1451 556 MT=22 (N,NALPHA GAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 557 Threshold to 30 MeV: Only the 4.438-MeV discrete gamma ray 825 1451 558 is given and it is based on the Nelson et al. [Ne99] data. 825 1451 559 825 1451 560 MT=103 (N,PGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 561 Threshold to 30 MeV: The cross sections for the 0.2774- and 825 1451 562 0.297-MeV gamma rays are based on the Nelson et al. [Ne99] data. 825 1451 563 The 0.3975-MeV gamma is inferred from the 0.2774-MeV gamma data 825 1451 564 through the Ajzenberg-Selove level scheme [Aj86] for 16N. The 825 1451 565 0.1201-MeV gamma cross section is based partially on GNASH 825 1451 566 calculations and partially inferred from the [Ne99] data using 825 1451 567 the 16N level scheme. 825 1451 568 825 1451 569 MT=104 (N,DGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 570 Threshold to 30 MeV: The cross sections for the 5.2701- and 825 1451 571 5.2988-MeV gamma rays are based on the Nelson et al. [Ne99] 825 1451 572 data. The cross sections for the remaining 60 (n,dg) gamma rays 825 1451 573 are based on GNASH calculations and the Ajzenberg-Selove level 825 1451 574 scheme [Aj91] for 15N, after renomalization to agree with the 825 1451 575 measured 5.2701- and 5.2988-MeV gamma-ray data. 825 1451 576 825 1451 577 MT=105 (N,TGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 578 Threshold to 30 MeV: The cross section for the 2.313-MeV 825 1451 579 gamma ray is based on the Nelson et al. [Ne99] measurement. The 825 1451 580 cross sections for the remaining 20 (n,tg) gamma rays are based 825 1451 581 on GNASH calculations and the Ajzenberg-Selove level scheme 825 1451 582 [Aj91] for 14N, after renomalization to agree with the measured 825 1451 583 2.313-MeV gamma-ray data. 825 1451 584 825 1451 585 MT=107 (N,ALPHA GAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 586 Threshold to 30 MeV: The cross sections for the 3.0894-, 825 1451 587 3.6845- and 3.8538-MeV gamma rays are based on the Nelson et 825 1451 588 al. [Ne99] data. The 0.1693-, 0.5951- and 0.7644-MeV gamma-ray 825 1451 589 cross sections are inferred from the above data through the 825 1451 590 Ajzenberg-Selove level scheme [Aj91]. Note that the 0.1693-MeV 825 1451 591 gamma from decay of the 3.8538-MeV level also was measured, but 825 1451 592 the 3.8538-MeV gamma is more intense and was used to determine 825 1451 593 the level excitation cross section. 825 1451 594 825 1451 595 MF=14 PHOTON ANGULAR DISTRIBUTIONS ---------------------------- 825 1451 596 825 1451 597 MT=4 (N,N'GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 598 Anisotropic angular distributions in Legendre polynomial 825 1451 599 representation are given for the 1.755-, 2.742-, 6.130-, 6.917-, 825 1451 600 and 7.117-MeV gamma rays, obtained by fitting the measurements 825 1451 601 of Nelson et al. [Ne99]. Isotropic angular distributions are 825 1451 602 assumed for the remaining gamma rays. 825 1451 603 825 1451 604 MT=16 (N,2NGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 605 An anisotropic angular distribution in Legendre polynomial 825 1451 606 representation is given for the 5.2409-MeV gamma ray, obtained 825 1451 607 by fitting the measurements of Nelson et al. [Ne99]. Isotropic 825 1451 608 angular distributions are assumed for the remaining gamma rays. 825 1451 609 825 1451 610 MT=22 (N,NALPHA GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 611 An anisotropic angular distribution in Legendre polynomial 825 1451 612 representation is given for the 4.438-MeV gamma ray, obtained by 825 1451 613 fitting the measurements of Nelson et al. [Ne99]. 825 1451 614 825 1451 615 MT=102 (N,GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 616 All gamma rays from radiative capture are assumed to be 825 1451 617 isotropic. 825 1451 618 825 1451 619 MT=103 (N,PGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 620 Anisotropic angular distributions in Legendre polynomial 825 1451 621 representation are given for the 0.2774-, 0.297-, and 0.3975-MeV 825 1451 622 gamma rays, obtained by fitting the measurements of Nelson et 825 1451 623 al. [Ne99]. The angular distributions for all remaining gamma 825 1451 624 rays are assumed to be isotropic. 825 1451 625 825 1451 626 MT=104 (N,DGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 627 An anisotropic angular distribution in Legendre polynomial 825 1451 628 representation is given for the 5.2701-MeV gamma ray, obtained 825 1451 629 by fitting the measurements of Nelson et al. [Ne99]. The 825 1451 630 angular distributions for all remaining gamma rays are assumed 825 1451 631 to be isotropic. 825 1451 632 825 1451 633 MT=105 (N,TGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 634 All gamma rays from (n,tg) reactions are assumed to be 825 1451 635 isotropic. 825 1451 636 825 1451 637 MT=107 (N,ALPHA GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 638 Anisotropic angular distributions in Legendre polynomial 825 1451 639 representation are given for the 0.1693-, 3.6845- and 3.8538- 825 1451 640 MeV gamma rays, obtained by fitting the measurements of Nelson 825 1451 641 et al. [Ne99]. Isotropic angular distributions are assumed for 825 1451 642 all the remaining gamma rays. 825 1451 643 825 1451 644 **************************************************************** 825 1451 645 825 1451 646 SUMMARY OF DATA VALIDATION OF THIS FILE AGAINST INTEGRAL 825 1451 647 BENCHMARKS 825 1451 648 825 1451 649 KAPL (Weinman, Caro, Lubitz) performed a number of data 825 1451 650 validation benchmark calculations to test the performance of this 825 1451 651 file (June-August 2001). This O16 evaluation gives consistently 825 1451 652 good results for the 21 CSWEG solution critical calculations, the 825 1451 653 liquid-oxygen broomstick neutron-transmission experiment, and the 825 1451 654 neutron age in water experiment (see below for more details). 825 1451 655 825 1451 656 A) 21 CSWEG solution critical calculations. Weinman calculated a 825 1451 657 set of 21 ORNL and Rocky Flats benchmark solution criticals used 825 1451 658 for CSEWG analyses. These calculations were run with ENDF/B-VI 825 1451 659 release 5 U235 (Leal,Larson,wright,Derrien) and hydrogen (332.0 825 1451 660 mbarns 2200m/s). Four different oxygen 16 cross section 825 1451 661 evaluations were considered. 825 1451 662 825 1451 663 1. KAPL-Caro 825 1451 664 2. This evaluation (which contains the KAPL data below 3.4 MeV) 825 1451 665 3. ENDF/B-VI MOD 2 825 1451 666 4. JENDL 3.2 825 1451 667 825 1451 668 All four O16 cross section evaluations gave good reactivity 825 1451 669 responses versus our fitting parameter above-thermal-leakage ATL. 825 1451 670 The ATL parameter is a sensitive trending variable to high energy 825 1451 671 scattering cross sections. All four O16 evaluations produced 825 1451 672 eigenvalues whose mean values were all close to unity and only 825 1451 673 the older ENDF/B-VI.2 cross section evaluation gave a slight 825 1451 674 reactivity trend (about .0020 Delta Keff over the range). The 825 1451 675 average eigenvalues and slopes are listed below. 825 1451 676 825 1451 677 Library Av. Keff Slope 825 1451 678 825 1451 679 KAPL-Caro 0.9993 +.0001 825 1451 680 This file 0.9996 +.0004 825 1451 681 ENDF/B-VI.2 1.0003 +.0032 825 1451 682 JENDL 3.2 1.0004 -.0002 825 1451 683 825 1451 684 Thus the reactivity trend, labeled "slope" in the table above, is 825 1451 685 much smaller in the new file compared to the previous ENDF/B-VI.2 825 1451 686 evaluation. 825 1451 687 825 1451 688 B) The liquid-oxygen broomstick experiment. The oxygen window at 825 1451 689 2.3 MeV is the most important feature at which energy the 825 1451 690 greatest transmission takes place. The new evaluation produces 825 1451 691 close to exact agreement with the experiment in the energy range 825 1451 692 of the oxygen window. The previous ENDF/B-VI value is slightly 825 1451 693 below the experimental value. At energies higher than 5.5 MeV, 825 1451 694 the new evaluation produces slightly better results than does the 825 1451 695 previous ENDF/B-VI results. 825 1451 696 825 1451 697 C) Neutron age in water. KAPL obtained 26.4 to be compared 825 1451 698 against an experimental value of 26.6 +/- 0.6. The previous 825 1451 699 ENDF/B-VI file gave a result of 26.3. 825 1451 700 825 1451 701 Additionally, A.C. (Skip) Kahler at Bettis lab undertook 825 1451 702 benchmark testing of this file (memo, May 16, 2001) against 825 1451 703 thermal benchmarks documented in the Int. Handbook of Evaluated 825 1451 704 Criticality Safety Benchmark Experiments, as well as the L5 and 825 1451 705 L6 ORNL benchmarks. From a thermal reactor benchmark perspective, 825 1451 706 there is little to distinguish the performance of the present 825 1451 707 file compared to the previous ENDF file and JENDL-3.2. 825 1451 708 825 1451 709 ***************************************************************** 825 1451 710 825 1451 711 REFERENCES 825 1451 712 825 1451 713 [Aj86] F. Ajzenberg-Selove, Nucl.Phys. A460, 1 (1986) 825 1451 714 [Aj91] F. Ajzenberg-Selove, Nucl.Phys. A523, 1 (1991) 825 1451 715 [Ba63] R.W. Bauer et al., Nucl.Phys. 47, 241 (1963) 825 1451 716 [Ba73] J.K. Bair and F.X. Haas, Phys.Rev.C 7, 1356 (1973) 825 1451 717 (n,a0) cross sect. obtained by detailed balance from this ref. 825 1451 718 [Ba85] M. Baba et al., Nuclear Data for Basic and Applied Sci., 825 1451 719 Proc. Conf., Santa Fe, NM, May 1985, Vol.1 (Gordon and Breach, 825 1451 720 1986) p.223 825 1451 721 [Be67] P.L. Beach et al., Phys.Rev. 156, 1201 (1967) 825 1451 722 [Be70] P. Bertin, report CEA-R-4047 (1970) 825 1451 723 [Bo63] M. 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MacFarlane, and A.J. 825 1451 736 Koning, "High-Energy Nuclear Data Libraries for Accelerator- 825 1451 737 Driven Technologies: Calculational Method for Heavy Recoils," 825 1451 738 Proc. of 2nd Int. Conf. on Accelerator Driven Transmutation 825 1451 739 Technology and Applications, Kalmar, Sweden, 3-7 June 1996. 825 1451 740 [Ch99] M.B. Chadwick, P.G. Young, G.M. Hale, et al., Los Alamos 825 1451 741 National Laboratory report, LA-UR-99-1222 (1999) 825 1451 742 [Ci68] S. Cierjacks et al., report KFK-1000 (1968) 825 1451 743 [Ci80] S. Cierjacks et al., Nucl.Inst.Meth. 169, 185 (1980) 825 1451 744 [Cl69] G. Clayeux and G. Grenier, report CEA-R-3807 (1969) 825 1451 745 [Co67] J.L. Cook, H. Ferguson, and A.R. De L Musgrove, Aust.J. 825 1451 746 Phys. 20, 477 (1967) 825 1451 747 [Da63] E.A. Davis et al., Nucl.Phys. 48, 169 (1963) 825 1451 748 [Da68] D. Dandy et al., report AWRE O60/68 (1968) 825 1451 749 [Di70] J.K. Dickens and F.G. Perey, Nucl.Sci.Eng. 40, 283 (1970) 825 1451 750 [Dr70] D.M. Drake et al., Nucl.Sci.Eng. 40, 294 (1970) 825 1451 751 [Dr76] L. Drigo et al., Nuovo cim. A 31 (1), 1 (1976) 825 1451 752 [Dr93] H.W.Drotleff et al., Ap.J. 414, 735 (1993) 825 1451 753 [Fi93] R. Finlay et al., Phys.Rev. C 47, 237 (1993) 825 1451 754 [Fo58] J.L. Fowler and H.O. Cohn, Phys.Rev. 109, 89 (1958) 825 1451 755 [Fo64] J.L. Fowler and C.H. Johnson, report ORNL-3582 (1964) p.90 825 1451 756 [Fo70] J.L. Fowler and C.H. Johnson, Phys.Rev.C 2,124 (1970) 825 1451 757 [Fo71] D.G. Foster and D.W. Glasgow, Phys.Rev.C 3, 576 (1971) 825 1451 758 [Gl82] S.L. Glendinning et al., Nuc.Sci.Eng. 82, 393 (1982) 825 1451 759 [Ha59] H.E. Hall et al., Nucl.Phys. 14, 295 (1959) 825 1451 760 [Ha92] G.M. Hale, P.G. Young, M. Chadwick, and Z.-P. Chen, 825 1451 761 Nuclear Data for Science and Technology, Proc. Conf., Juelich, 825 1451 762 Germany, May 1991 [LA-UR-91-1516], (Ed. S. M. Qaim, Springer- 825 1451 763 Verlag, Germany, 1992), p.921 825 1451 764 [He80] D.M. Hetrick and C.Y. Fu, report ORNL/TM-7341 (1980) 825 1451 765 [Hi58] R.W. Hill, Phys.Rev. 109, 2105 (1958) 825 1451 766 [Hu62] W. Hunzinger and P. Huber, Helv.Phys.Acta 35, 351 (1962) 825 1451 767 [Ig75] A.V. Ignatyuk, G.N. Smirenkin, and A.S. Tishin, Sov.J. 825 1451 768 Nucl.Phys. 21, 255 (1975); transl. of Yad.Fiz. 21, 485 (1975) 825 1451 769 [Jo67] C.H. Johnson and J.L. Fowler, Phys.Rev. 162, 890 (1967) 825 1451 770 [Jo73] C.H. Johnson, Phys.Rev.C 7, 561 (1973) 825 1451 771 [Jo74] C.H. Johnson et al., report ORNL-4937 (1974) 825 1451 772 [Jo79] C.H. Johnson, et al., Nuclear Cross Sections for 825 1451 773 Technology, Proc. Conf., Knoxville, TN, Oct. 1979 (National 825 1451 774 Bureau of Standards, 1980) p.807 825 1451 775 [Ju64] E.T. Jurney and H.T. Motz, Bull.Am.Phys.Soc. 9, 176 (1964) 825 1451 776 [Ka77] C. Kalbach, Z.Phys.A 283, 401 (1977) 825 1451 777 [Ka85] C. Kalbach, Los Alamos National Laboratory report 825 1451 778 LA-10248-MS (1985) 825 1451 779 [Ka88] C. Kalbach, Phys.Rev.C 37, 2350 (1988); see also 825 1451 780 C. Kalbach and F. M. Mann, Phys.Rev.C 23, 112 (1981) 825 1451 781 [Ke93] S.Kellogg, reported by C.R.Brune et al., Phys. Rev. C 48, 825 1451 782 3119 (1993). Data renormalized substantially. 825 1451 783 [Ki72] W.E. Kinney and F.G. Perey, report ORNL-4780 (1972) 825 1451 784 [Ko90] J. Kopecky and M. Uhl, Phys.Rev.C 41, 1941 (1990) 825 1451 785 [La60] R.O. Lane et.al., Argonne report ANL-6172 (1960) 825 1451 786 [La80] D. Larson et al., Symp. on Neutron Cross Sections from 10 825 1451 787 to 50 MeV, BNL, May 1980, report BNL-NCS-51243, Vol. 1 (1980) 825 1451 788 p.277 and private communication (1989) 825 1451 789 [Le68] B. Leroux et al., Nucl.Phys. A116, 196 (1968) 825 1451 790 [Li66] D. Lister and A. Sayres, Phys.Rev. 143, 745 (1966) 825 1451 791 [Lu70] B. Lundberg et al., Phys.Scripta 2, 273 (1970) 825 1451 792 [Ma62] J.P. Martin and M.S. Zucker, B.Am.Phys.Soc. 7, 72 (1962) 825 1451 793 [Ma68] D.R. Maxson and R.D. Murphy, Nucl.Phys. A110, 555 (1968) 825 1451 794 [Mc66a] W.J. McDonald et al., Nucl.Phys. 75, 353 (1966) 825 1451 795 [Mc66b] W.N. McDicken and W. Jack, Nucl.Phys. 88, 457 (1966) 825 1451 796 [Ne72] D.O. Nellis and P.S. Buchanan, report DNA-2716 (1972) 825 1451 797 [Ne90] R. Nelson et al., LANL, private communication, 1990 825 1451 798 [Ne99] R.O. Nelson and A. Michaudon, Los Alamos report LA-UR-99- 825 1451 799 4170 (1999). 825 1451 800 [No78] C. Nordborg et al., Nucl.Sci.Eng. 66, 75 (1978) 825 1451 801 [Ok55] A. Okazaki, Phys.Rev. 99, 55 (1955) 825 1451 802 [Ol90] N. Olsson et al., Nucl.Phys.A 509, 161 (1990) 825 1451 803 [Or70] V.J. Orphan et al., Nucl.Sci.Eng. 42, 352 (1970) 825 1451 804 [Pe72] F.G. Perey et al., report ORNL-4823 [ENDF-178] (1972) 825 1451 805 [Pe85] J.S. Petler et al., Phys.Rev.C 32, 673 (1985) 825 1451 806 [Ph61] D.D. Phillips, private communication to BNL (1961) 825 1451 807 [Sa97] T. Sanami and M. Baba, Trieste Conf.(1997)p.616 825 1451 808 [Sc72] R.A. Schrack, Bull.Am.Phy.Soc. 17, 555 [HE1] (1972) 825 1451 809 [Sc77] I. Schouky et al., report KFK-2503 825 1451 810 [Si68] I. Sick et al., Helv.Phys.Acta 41, 573 (1968) 825 1451 811 [Su94] T.S. Subramanian et al., Phys. Rev. C 34, 1580 (1986), and 825 1451 812 private communication to Chadwick (1994). 825 1451 813 [Wa57] R.B.Walton et al., Phys. Rev. 107, 1065 (1957) 825 1451 814 [Yo01] P.G. Young, G.M. Hale, and M.B. Chadwick, LANL report to 825 1451 815 be issued (2001). 825 1451 816 [Yo92] P.G. Young, E.D. Arthur, and M.B. Chadwick, Los Alamos 825 1451 817 report LA-12343-MS (1992) 825 1451 818 825 1451 819 ************************ C O N T E N T S *********************** 825 1451 820 ***************** Program LINEAR (VERSION 2004-1) *************** 825 1451 821 For All Data Greater than 1.0000E-10 barns in Absolute Value 825 1451 822 Data Linearized to Within an Accuracy of .100000000 per-cent 825 1451 823 ***************** Program SIGMA1 (VERSION 2004-1) *************** 825 1451 824 Data Doppler Broadened to 2100.00000 Kelvin 825 1451 825 for All Data Greater than 1.0000E-10 barns in Absolute Value 825 1451 826 Data Linearized to Within an Accuracy pf .100000000 per-cent 825 1451 827 ***************** Program FIXUP (Version 2004-1) **************** 825 1451 828 Corrected ZA/AWR in All Sections-----------------------------Yes 825 1451 829 Corrected Thresholds-----------------------------------------No 825 1451 830 Extended Cross Sections to 20 MeV----------------------------No 825 1451 831 Allow Cross Section Deletion---------------------------------No 825 1451 832 Allow Cross Section Reconstruction---------------------------Yes 825 1451 833 Make All Cross Sections Non-Negative-------------------------Yes 825 1451 834 Delete Energies Not in Ascending Order-----------------------Yes 825 1451 835 Deleted Duplicate Points-------------------------------------Yes 825 1451 836 Check for Ascending MAT/MF/MT Order--------------------------Yes 825 1451 837 Check for Legal MF/MT Numbers--------------------------------Yes 825 1451 838 Allow Creation of Missing Sections---------------------------No 825 1451 839 Allow Insertion of Energy Points-----------------------------No 825 1451 840 Create Uniform Energy Grid-----------------------------------No 825 1451 841 Delete Section if Cross Section =0 at All Energies-----------Yes 825 1451 842 **************** Program DICTIN (VERSION 2004-1) **************** 825 1451 843 1 451 987 3 825 1451 844 2 151 4 3 825 1451 845 3 1 1236 3 825 1451 846 3 2 571 3 825 1451 847 3 3 856 3 825 1451 848 3 4 97 3 825 1451 849 3 5 11 3 825 1451 850 3 16 16 3 825 1451 851 3 22 30 3 825 1451 852 3 23 25 3 825 1451 853 3 28 31 3 825 1451 854 3 32 14 3 825 1451 855 3 41 12 3 825 1451 856 3 44 12 3 825 1451 857 3 45 12 3 825 1451 858 3 51 47 3 825 1451 859 3 52 85 3 825 1451 860 3 53 82 3 825 1451 861 3 54 80 3 825 1451 862 3 55 67 3 825 1451 863 3 56 32 3 825 1451 864 3 57 31 3 825 1451 865 3 91 34 3 825 1451 866 3 102 139 3 825 1451 867 3 103 60 3 825 1451 868 3 104 55 3 825 1451 869 3 105 38 3 825 1451 870 3 107 689 3 825 1451 871 3 108 30 3 825 1451 872 3 112 19 3 825 1451 873 3 600 52 3 825 1451 874 3 601 42 3 825 1451 875 3 602 53 3 825 1451 876 3 603 53 3 825 1451 877 3 650 33 3 825 1451 878 3 651 26 3 825 1451 879 3 652 26 3 825 1451 880 3 653 23 3 825 1451 881 3 654 23 3 825 1451 882 3 655 21 3 825 1451 883 3 656 22 3 825 1451 884 3 657 14 3 825 1451 885 3 658 20 3 825 1451 886 3 659 14 3 825 1451 887 3 660 19 3 825 1451 888 3 661 20 3 825 1451 889 3 662 17 3 825 1451 890 3 663 18 3 825 1451 891 3 664 16 3 825 1451 892 3 665 16 3 825 1451 893 3 666 14 3 825 1451 894 3 667 15 3 825 1451 895 3 668 16 3 825 1451 896 3 669 14 3 825 1451 897 3 700 30 3 825 1451 898 3 701 27 3 825 1451 899 3 702 20 3 825 1451 900 3 703 15 3 825 1451 901 3 704 20 3 825 1451 902 3 705 16 3 825 1451 903 3 706 18 3 825 1451 904 3 707 16 3 825 1451 905 3 708 14 3 825 1451 906 3 709 16 3 825 1451 907 3 749 6 3 825 1451 908 3 800 639 3 825 1451 909 3 801 104 3 825 1451 910 3 802 87 3 825 1451 911 3 803 107 3 825 1451 912 4 2 3867 3 825 1451 913 4 51 84 3 825 1451 914 4 52 84 3 825 1451 915 4 53 66 3 825 1451 916 4 54 64 3 825 1451 917 4 55 50 3 825 1451 918 4 56 2 3 825 1451 919 4 57 2 3 825 1451 920 4 600 2 3 825 1451 921 4 601 2 3 825 1451 922 4 602 2 3 825 1451 923 4 603 2 3 825 1451 924 4 650 2 3 825 1451 925 4 651 2 3 825 1451 926 4 652 2 3 825 1451 927 4 653 2 3 825 1451 928 4 654 2 3 825 1451 929 4 655 2 3 825 1451 930 4 656 2 3 825 1451 931 4 657 2 3 825 1451 932 4 658 2 3 825 1451 933 4 659 2 3 825 1451 934 4 660 2 3 825 1451 935 4 661 2 3 825 1451 936 4 662 2 3 825 1451 937 4 663 2 3 825 1451 938 4 664 2 3 825 1451 939 4 665 2 3 825 1451 940 4 666 2 3 825 1451 941 4 667 2 3 825 1451 942 4 668 2 3 825 1451 943 4 669 2 3 825 1451 944 4 700 2 3 825 1451 945 4 701 2 3 825 1451 946 4 702 2 3 825 1451 947 4 703 2 3 825 1451 948 4 704 2 3 825 1451 949 4 705 2 3 825 1451 950 4 706 2 3 825 1451 951 4 707 2 3 825 1451 952 4 708 2 3 825 1451 953 4 709 2 3 825 1451 954 4 800 2188 3 825 1451 955 4 801 2 3 825 1451 956 4 802 2 3 825 1451 957 4 803 2 3 825 1451 958 6 5 4784 3 825 1451 959 6 16 522 3 825 1451 960 6 22 2279 3 825 1451 961 6 23 915 3 825 1451 962 6 28 1451 3 825 1451 963 6 32 476 3 825 1451 964 6 41 258 3 825 1451 965 6 44 246 3 825 1451 966 6 45 275 3 825 1451 967 6 91 2341 3 825 1451 968 6 108 798 3 825 1451 969 6 112 454 3 825 1451 970 6 749 320 3 825 1451 971 12 102 16 3 825 1451 972 13 4 1251 3 825 1451 973 13 16 134 3 825 1451 974 13 22 51 3 825 1451 975 13 103 286 3 825 1451 976 13 104 1540 3 825 1451 977 13 105 472 3 825 1451 978 13 107 1161 3 825 1451 979 14 4 933 3 825 1451 980 14 16 17 3 825 1451 981 14 22 187 3 825 1451 982 14 102 1 3 825 1451 983 14 103 554 3 825 1451 984 14 104 242 3 825 1451 985 14 105 1 3 825 1451 986 14 107 400 3 825 1451 987 825 1 0 988 825 0 0 989 8.01600E+3 1.58575E+1 0 0 1 0 825 2151 990 8.01600E+3 1.00000E+0 0 0 1 0 825 2151 991 1.00000E-5 2.00000E+7 0 0 0 0 825 2151 992 0.0 5.56256E-1 0 0 0 0 825 2151 993 825 2 0 994 825 0 0 995 8.01600E+3 1.58575E+1 0 0 0 0 825 3 1 996 0.0 0.0 0 0 1 3699 825 3 1 997 3699 2 825 3 1 998 1.00000E-5 146.874264 1.08624E-5 140.926849 1.17903E-5 135.271237 825 3 1 999 1.28071E-5 129.794382 1.39012E-5 124.586013 1.51000E-5 119.573903 825 3 1 1000 1.52258E-5 119.047945 1.63900E-5 114.814806 1.67440E-5 113.527639 825 3 1 1001 1.78034E-5 110.162782 1.82344E-5 108.793855 1.93243E-5 105.780440 825 3 1 1002 2.01417E-5 103.520466 2.09909E-5 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1.31055423 5780000.00 1.29563111 5790000.00 1.26585886 825 3 1 1860 5795000.00 1.25303302 5800000.00 1.24020736 5810000.00 1.21465904 825 3 1 1861 5815000.00 1.20396422 5820000.00 1.19331057 5825000.00 1.18270592 825 3 1 1862 5830000.00 1.17215927 5835000.00 1.16373297 5840000.00 1.15539290 825 3 1 1863 5845000.00 1.14715883 5850000.00 1.14108187 5855000.00 1.13517291 825 3 1 1864 5860000.00 1.13251559 5865000.00 1.13014351 5867500.00 1.12914997 825 3 1 1865 5870000.00 1.12938100 5875000.00 1.13301292 5880000.00 1.14126465 825 3 1 1866 5885000.00 1.15624569 5890000.00 1.18128278 5895000.00 1.22202778 825 3 1 1867 5900000.00 1.28844886 5905000.00 1.39715754 5907250.00 1.46786918 825 3 1 1868 5908000.00 1.49338618 5910000.00 1.57831568 5912000.00 1.68335873 825 3 1 1869 5914250.00 1.82592266 5915000.00 1.87681210 5915500.00 1.91201639 825 3 1 1870 5916000.00 1.95212809 5917000.00 2.03311149 5918000.00 2.11487488 825 3 1 1871 5920000.00 2.28463800 5921000.00 2.36907956 5922000.00 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5990000.00 1.02072880 5990500.00 1.06874546 825 3 1 1885 5992000.00 1.22630613 5993500.00 1.39157915 5994000.00 1.44321864 825 3 1 1886 5994250.00 1.46906751 5995000.00 1.53528948 5995750.00 1.58872372 825 3 1 1887 5996000.00 1.60278569 5996250.00 1.61694893 5997000.00 1.64821662 825 3 1 1888 5997750.00 1.66694604 5998000.00 1.66955643 5998500.00 1.67496720 825 3 1 1889 5998875.00 1.67561857 5999000.00 1.67493464 5999500.00 1.67235495 825 3 1 1890 6000000.00 1.66539308 6000500.00 1.65855071 6001000.00 1.64701997 825 3 1 1891 6002000.00 1.62413448 6003000.00 1.59713137 6004000.00 1.57021227 825 3 1 1892 6006000.00 1.51651207 6007000.00 1.48970297 6009000.00 1.44129998 825 3 1 1893 6011000.00 1.39849887 6012000.00 1.37896081 6015000.00 1.32824457 825 3 1 1894 6016000.00 1.31431003 6018000.00 1.28639596 6020000.00 1.26272241 825 3 1 1895 6025000.00 1.21433337 6030000.00 1.17725482 6035000.00 1.14828052 825 3 1 1896 6040000.00 1.12554234 6045000.00 1.10784834 6050000.00 1.09554774 825 3 1 1897 6052000.00 1.09091870 6055000.00 1.08783869 6058000.00 1.08571833 825 3 1 1898 6060000.00 1.08680218 6061000.00 1.08779110 6062000.00 1.09015042 825 3 1 1899 6064000.00 1.09579207 6066000.00 1.10744819 6067500.00 1.11802102 825 3 1 1900 6068000.00 1.12372370 6070000.00 1.15082842 6071000.00 1.17165049 825 3 1 1901 6071500.00 1.18341752 6072000.00 1.19750185 6072500.00 1.21350268 825 3 1 1902 6073000.00 1.23195984 6073500.00 1.25314099 6074000.00 1.27738901 825 3 1 1903 6074500.00 1.30547153 6075000.00 1.33708302 6075500.00 1.37388951 825 3 1 1904 6076000.00 1.41378671 6077000.00 1.50607111 6078000.00 1.60888551 825 3 1 1905 6078500.00 1.65235128 6079000.00 1.68855792 6079375.00 1.69947441 825 3 1 1906 6079750.00 1.70455012 6080000.00 1.70329375 6080125.00 1.69531743 825 3 1 1907 6080500.00 1.66439377 6082000.00 1.52694437 6082500.00 1.46758040 825 3 1 1908 6083750.00 1.32463563 6084000.00 1.29840764 6084250.00 1.27601339 825 3 1 1909 6084750.00 1.23626761 6085250.00 1.20165267 6086000.00 1.15744368 825 3 1 1910 6087500.00 1.10079533 6088000.00 1.08325451 6090000.00 1.04074286 825 3 1 1911 6092000.00 1.01521815 6094000.00 .999476999 6096000.00 .986977853 825 3 1 1912 6098000.00 .979085834 6100000.00 .972575816 6102000.00 .967018798 825 3 1 1913 6104000.00 .962144780 6106000.00 .958667212 6108000.00 .955569643 825 3 1 1914 6110000.00 .952768075 6115000.00 .946684653 6120000.00 .941486232 825 3 1 1915 6125000.00 .936857810 6130000.00 .932619908 6140000.00 .926910546 825 3 1 1916 6150000.00 .921794184 6160000.00 .919146117 6170000.00 .916499203 825 3 1 1917 6175000.00 .914997997 6180000.00 .914760840 6190000.00 .913725527 825 3 1 1918 6200000.00 .911950214 6210000.00 .911346810 6220000.00 .909898406 825 3 1 1919 6225000.00 .908882384 6230000.00 .907687002 6240000.00 .905936361 825 3 1 1920 6250000.00 .903766721 6260000.00 .897947881 6270000.00 .896668103 825 3 1 1921 6272170.00 .895823178 6275000.00 .896378050 6280000.00 .895682178 825 3 1 1922 6284856.25 .894718064 6290000.00 .894248659 6300000.00 .894186864 825 3 1 1923 6302000.00 .893911154 6304000.00 .893966044 6306000.00 .894804504 825 3 1 1924 6308000.00 .896270089 6310000.00 .897735698 6314000.00 .900307773 825 3 1 1925 6316000.00 .902894172 6318000.00 .905561173 6322000.00 .910895231 825 3 1 1926 6324000.00 .914895054 6325000.00 .916718099 6328000.00 .922187751 825 3 1 1927 6330000.00 .926276326 6332000.00 .931007070 6336000.00 .941141393 825 3 1 1928 6338000.00 .946208609 6340000.00 .951486119 6342000.00 .957377809 825 3 1 1929 6344000.00 .963839644 6346000.00 .970301535 6352000.00 .994637637 825 3 1 1930 6354000.00 1.00578570 6356000.00 1.01714282 6358000.00 1.02924424 825 3 1 1931 6359000.00 1.03599050 6360000.00 1.04336050 6362000.00 1.05960030 825 3 1 1932 6364000.00 1.07584048 6366000.00 1.09495530 6368000.00 1.11365539 825 3 1 1933 6370000.00 1.13416670 6372000.00 1.15601241 6375000.00 1.19063893 825 3 1 1934 6376000.00 1.20222829 6379000.00 1.24397366 6380000.00 1.25988051 825 3 1 1935 6382000.00 1.29326466 6384000.00 1.33004011 6388000.00 1.40331706 825 3 1 1936 6391000.00 1.45535458 6392000.00 1.47098274 6394000.00 1.49563160 825 3 1 1937 6395500.00 1.51411830 6396500.00 1.52261676 6399000.00 1.53771763 825 3 1 1938 6400000.00 1.54125255 6402000.00 1.54755786 6404000.00 1.54326966 825 3 1 1939 6405500.00 1.52989419 6406000.00 1.52259615 6408000.00 1.49029569 825 3 1 1940 6410000.00 1.44752474 6412000.00 1.40194359 6414000.00 1.35812368 825 3 1 1941 6415500.00 1.32396657 6416000.00 1.31416156 6418000.00 1.27074174 825 3 1 1942 6420000.00 1.22966299 6422000.00 1.19197356 6425000.00 1.13543954 825 3 1 1943 6426000.00 1.11768442 6428000.00 1.08246995 6430000.00 1.04970865 825 3 1 1944 6430885.00 1.03489060 6432000.00 1.01622156 6434000.00 .985678489 825 3 1 1945 6436000.00 .955746421 6438000.00 .927266349 6439000.00 .913343812 825 3 1 1946 6440000.00 .900761800 6442000.00 .876210277 6444000.00 .855288961 825 3 1 1947 6446000.00 .837355496 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