8-O - 16 ENDF/B-VI Distributed by NNDC, Brookhaven Nat. Lab. 6000 0 0 0 8.016000+3 1.585751+1 0 0 0 3 825 1451 1 0.000000+0 0.000000+0 0 0 0 6 825 1451 2 1.000000+0 3.000000+7 8 0 10 6 825 1451 3 0.000000+0 0.000000+0 0 0 816 144 825 1451 4 8-O - 16 LANL EVAL-APR01 HALE,YOUNG,CHADWICK,CARO,LUBITZ 825 1451 5 Ch96ab,Ca98,Ch99,Yo01 DIST-SEP 1 REV2- 20011018 825 1451 6 ----ENDF/B-VI MATERIAL 825 825 1451 7 -----INCIDENT NEUTRON DATA 825 1451 8 ------ENDF-6 FORMAT 825 1451 9 825 1451 10 ****************************************************************** 825 1451 11 825 1451 12 ENDF/B-VI MOD 3 Evaluation, April 2001, P.G. Young, G.M. Hale 825 1451 13 M.B. Chadwick (LANL), E.Caro, C.R. Lubitz (KAPL) 825 1451 14 825 1451 15 This evaluation is a combination of a new MOD 3 evaluation 825 1451 16 below 30 MeV and the previous MOD 2 evaluation from 20 to 150 MeV. 825 1451 17 Both these evaluations are described below. The only change to the 825 1451 18 data above 30 MeV is to add tritium-production data, based on 825 1451 19 experimental yield data and spectra calculated with the GNASH 825 1451 20 Hauser-Feshbach/preequilibrium code. 825 1451 21 This evaluation provides a complete representation of the 825 1451 22 nuclear data needed for transport, damage, heating, radioactivity, 825 1451 23 and shielding applications over the incident neutron energy range 825 1451 24 from 1.0E-11 to 150 MeV. The discussion here is divided into the 825 1451 25 region above and below 30 MeV. 825 1451 26 825 1451 27 ------------------------------------------------------------------ 825 1451 28 825 1451 29 INCIDENT NEUTRON ENERGIES > 30 MeV 825 1451 30 825 1451 31 The evaluation above 30 MeV utilizes MF=6, MT=5 to represent 825 1451 32 all reaction data. Production cross sections and emission 825 1451 33 spectra are given for neutrons, protons, deuterons, alpha 825 1451 34 particles, gamma rays, and all residual nuclides produced (A>5) 825 1451 35 in the reaction chains. To summarize, the ENDF sections with 825 1451 36 non-zero data above En = 30 MeV are: 825 1451 37 825 1451 38 MF=3 MT= 1 Total Cross Section 825 1451 39 MT= 2 Elastic Scattering Cross Section 825 1451 40 MT= 3 Nonelastic Cross Section 825 1451 41 MT= 5 Sum of Binary (n,n') and (n,x) Reactions 825 1451 42 MT=102 Radiative Capture Cross Section (Estimate Only) 825 1451 43 825 1451 44 MF=4 MT= 2 Elastic Angular Distributions 825 1451 45 825 1451 46 MF=6 MT= 5 Production Cross Sections and Energy-Angle 825 1451 47 Distributions for Emission Neutrons, Protons, 825 1451 48 Deuterons, and Alphas; and Angle-Integrated 825 1451 49 Spectra for Gamma Rays and Residual Nuclei That 825 1451 50 Are Stable Against Particle Emission 825 1451 51 825 1451 52 The evaluation is based on nuclear model calculations that 825 1451 53 have been benchmarked to experimental data, especially for n + 825 1451 54 O16 and p + O16 reactions [Ch96a]. We use the GNASH code system 825 1451 55 [Yo92], which utilizes Hauser-Feshbach statistical, preequi- 825 1451 56 librium and direct-reaction theories. Coupled-channel and 825 1451 57 spherical optical model calculations are used to obtain particle 825 1451 58 transmission coefficients for the Hauser-Feshbach calculations, 825 1451 59 as well as for the elastic neutron angular distributions. 825 1451 60 Cross sections and spectra for producing individual residual 825 1451 61 nuclei are included for reactions that exceed a cross section of 825 1451 62 approximately 1 nb at any energy. The energy-angle-correlations 825 1451 63 for all outgoing particles are based on Kalbach systematics 825 1451 64 [Ka88]. 825 1451 65 A model was developed to calculate the energy distributions of 825 1451 66 all recoil nuclei in the GNASH calculations [Ch96b]. The recoil 825 1451 67 energy distributions are represented in the laboratory system in 825 1451 68 MT=5, MF=6, and are given as isotropic in the lab system. Note 825 1451 69 that all other data in MT=5,MF=6 are given in the center-of-mass 825 1451 70 system. This method of representation requires a modification of 825 1451 71 the original ENDF-6 format. 825 1451 72 Preequilibrium corrections were performed in the course of the 825 1451 73 GNASH calculations using either Feshbach, Kerman, Koonin (FKK) 825 1451 74 theory [Ch93] or the exciton model of Kalbach [Ka77, Ka85]. 825 1451 75 Discrete level data from nuclear data sheets were matched to 825 1451 76 continuum level densities using the formulation of Ignatyuk 825 1451 77 [Ig75] and pairing and shell parameters from the Cook [Co67] 825 1451 78 analysis. Neutron and charged-particle transmission coefficients 825 1451 79 were obtained from the optical potentials, as discussed below. 825 1451 80 Gamma-ray transmission coefficients were calculated using the 825 1451 81 Kopecky-Uhl model [Ko90]. 825 1451 82 825 1451 83 ------------------------------------------------------------------ 825 1451 84 825 1451 85 INCIDENT NEUTRON ENERGIES < 30 MeV 825 1451 86 825 1451 87 The evaluation below 30 MeV includes complete data for all 825 1451 88 significant neutron-induced reactions. It is comprised of 825 1451 89 R-parameter [Ca98] and R-matrix analyses below 6.25 MeV, and a 825 1451 90 combination of experimental and theoretical data evaluation 825 1451 91 from 6.25 to 30 MeV. A summary of the evaluation by energy 825 1451 92 range is given below, followed by a detailed description of 825 1451 93 the evaluation, reaction by reaction. 825 1451 94 825 1451 95 NEUTRON ENERGY < 6.25 MeV 825 1451 96 825 1451 97 The evaluation below 3.4 MeV is an R-function fit [Ca98] to 825 1451 98 experimental data. At 3.4 MeV, it is spliced to the LANL R-matrix 825 1451 99 analysis with a transition region of about 60 keV centered at 825 1451 100 3.4 MeV. The LANL analysis is used for the region from 3.40 to 825 1451 101 6.25 MeV. 825 1451 102 825 1451 103 NEUTRON ENERGY > 6.25 MeV 825 1451 104 825 1451 105 The following major modifications were made above 6.25 MeV: 825 1451 106 1. The maximum energy of the evaluation was increased from 20 to 825 1451 107 30 MeV. 825 1451 108 2. New measurements of 16O(n,xgamma) angular distributions (7 825 1451 109 angles, En = 4 - 200 MeV) by Nelson et al. [Ne99] were incor- 825 1451 110 porated into the evaluation. The measurements use a high- 825 1451 111 resolution Ge detector and result in data for some 21 gamma rays. 825 1451 112 The distributions were fit with Legendre expansions to obtain 825 1451 113 angle-integrated cross sections for MF=13 and angular 825 1451 114 distributions for MF=14. Nuclear energy level schemes and gamma 825 1451 115 branching ratios [Aj86,Aj91] were utilized to extract level 825 1451 116 excitation cross sections in MF=3 for discrete states in 16O, 825 1451 117 14-16N, and 13C, corresponding to (n,n'), (n,p), (n,d), (n,t), 825 1451 118 and (n,alpha) reactions. 825 1451 119 3. New measurements of 16O(n,alpha) cross sections at 14 MeV by 825 1451 120 Sanami and Baba [Sa97] were used to adjust the (n,alpha) cross 825 1451 121 sections. 825 1451 122 4. The neutron total cross section measurements of Finlay [Fi93] 825 1451 123 were incorporated into the evaluation above 7.3 MeV. Adjustments 825 1451 124 of up to 2% were made in the existing evaluation. 825 1451 125 5. The new evaluation contains no pseudo level or excitation 825 1451 126 energy bin data. Calculations were made with the GNASH code to 825 1451 127 provide continuum emission data in MF=6 format, as well as any 825 1451 128 unmeasured data. Calculated cross sections were renormalized 825 1451 129 whenever possible using experimental data. The GNASH calculations 825 1451 130 utilized transmission coefficients calculated with a spherical 825 1451 131 optical potential and level densities from the Gilbert and 825 1451 132 Cameron model, plus preequilibrium corrections using systematic 825 1451 133 values of parameters. 825 1451 134 6. Comparisons of the evaluation with a large body of 825 1451 135 experimental data have been made to validate the new data. 825 1451 136 825 1451 137 ------------------------------------------------------------------ 825 1451 138 825 1451 139 DETAILED DESCRIPTION REACTION BY REACTION 825 1451 140 825 1451 141 MF=2 RESONANCE PARAMETERS ------------------------------------- 825 1451 142 825 1451 143 The evaluation below 3.4 MeV is an R-function fit [Ca98] to 825 1451 144 experimental data using an optical model to provide a background 825 1451 145 R-function. The procedure is coded in the KAPL code "OPTIC", 825 1451 146 with an extension of the original code to convert the optical- 825 1451 147 model phase shifts to background R-functions. 825 1451 148 The analysis is carried to 3.4 MeV, where it is spliced to the 825 1451 149 LANL R-matrix analysis, with a transition region of about 60 keV 825 1451 150 centered at 3.4 MeV. 825 1451 151 From 3.4 to 6.25 MeV, a test evaluation was obtained from a new 825 1451 152 multi-channel R-matrix analysis of a large part of the available 825 1451 153 experimental data base using the EDA code. The analysis of the 825 1451 154 17O system includes data for n+16O neutron total cross sections 825 1451 155 and elastic scattering angular distributions, as well as data 825 1451 156 for the 16O(n,alpha) reaction in both the (n,alpha) and 825 1451 157 (alpha,n) directions. Also included are excitation functions 825 1451 158 for alpha+13C elastic scattering. The total cross sections in 825 1451 159 the final version of this analysis may change, especially in the 825 1451 160 region above 4 MeV. 825 1451 161 825 1451 162 Effective scattering radius = 5.56256E-13 cm. 825 1451 163 825 1451 164 MF=3 NEUTRON CROSS SECTIONS ----------------------------------- 825 1451 165 825 1451 166 THERMAL (2200 m/s) CROSS SECTIONS 825 1451 167 825 1451 168 TOTAL = 3.89440 B RADIATIVE CAPTURE= 0.1900 MB 825 1451 169 ELASTIC= 3.89421 B 825 1451 170 825 1451 171 MT=1 TOTAL CROSS SECTION 825 1451 172 0.0 to 3.40 MeV, calculated from R-function fit to total cross 825 1451 173 section and elastic angular distributions - see above. 825 1451 174 3.4 to 6.25 MeV, calculated from R-Matrix parameters by 825 1451 175 simultaneously fitting most of the available 16O(n,n)16O and 825 1451 176 16O(n,alpha0)13C data, as well as 13C(alpha,alpha)13C data at 825 1451 177 energies below En = 6.2 MeV. The experimental total cross 825 1451 178 section data fitted in the analysis were the [Jo74] results below 825 1451 179 6.26 MeV, and the [La80] measurements at higher energies, with 825 1451 180 inserts of the high-resolution data of [Jo79] over the resonances 825 1451 181 and in the window at En = 2.3-2.4 MeV. 825 1451 182 6.25 to 30 MeV, based on an adjustment of the covariance 825 1451 183 analysis used for the ENDF/B-VI (Rel. 0) evaluation to 825 1451 184 accommodate the new measurements of Finlay et al. [Fi93]. The 825 1451 185 previous ENDF/B-VI (Rel. 0) evaluations is based on analysis 825 1451 186 with the GLUCS Bayes code [He80] of the remaining major total 825 1451 187 cross section measurements [Fo71], [Pe72], [Sc72], [La80], 825 1451 188 [Ci68], [Ci80], with structure inserted from the high-resolution 825 1451 189 [Ci80] measurement. 825 1451 190 825 1451 191 MT=2 ELASTIC SCATTERING CROSS SECTION 825 1451 192 0.0 to 3.40 MeV, calculated from R-function fit to total cross 825 1451 193 section and elastic angular distributions - see above. 825 1451 194 3.4 to 6.25 MeV, R-matrix analysis that includes all available 825 1451 195 experimental data, as described above. Elastic angular 825 1451 196 distribution data used in the analysis includes [La60], [Ok55], 825 1451 197 [Fo58], [Ma62], [Fo70], [Hu62], [Ph61], [Jo67], [Ki72], [Ch61], 825 1451 198 [Dr76], [Fo64]. 825 1451 199 6.25 to 20 MeV, obtained by subtracting the nonelastic cross 825 1451 200 section (MT=3) from the total cross section (MT=1), although 825 1451 201 small adjustments were made to several of the less well 825 1451 202 determined reaction cross sections in order to enhance agreement 825 1451 203 with the elastic measurements of Borker [Bo89], Glendinning 825 1451 204 [Gl82], and Petler [Pe85]. The magnitude of these adjustments 825 1451 205 was generally small and was greatest near structure and near 825 1451 206 18 MeV. 825 1451 207 825 1451 208 MT=4 INELASTIC CROSS SECTION 825 1451 209 Threshold to 30 MeV, sum of MT=51-57, 91. 825 1451 210 825 1451 211 MT=51-57 INELASTIC CROSS SECTION TO DISCRETE STATES 825 1451 212 Threshold to 30 MeV, the (n,n') cross sections corresponding 825 1451 213 to gamma-emitting excited levels of 16O are included in MT=51-57 825 1451 214 as follows: 825 1451 215 MT=51 Ex= 6.0494 MeV 825 1451 216 MT=52 Ex= 6.129893 MeV 825 1451 217 MT=53 Ex= 6.9171 MeV 825 1451 218 MT=54 Ex= 7.11685 MeV 825 1451 219 MT=55 Ex= 8.8719 MeV 825 1451 220 MT=56 Ex=10.957 MeV 825 1451 221 MT=57 Ex=11.080 MeV 825 1451 222 825 1451 223 Note that the 16O levels at 9.585, 9.8445, and 10.356 are 825 1451 224 omitted because they decay primarily by alpha particle emission 825 1451 225 and those data are included in MT=22. 825 1451 226 825 1451 227 MT=16 (N,2N) CROSS SECTION 825 1451 228 Threshold to 30 MeV, based on GNASH calculation, renormalized 825 1451 229 down by approximately 30% to improve agreement with measurement 825 1451 230 of Brill et al. [Br61]. 825 1451 231 825 1451 232 MT=22 (N,NALPHA) CROSS SECTION 825 1451 233 Threshold to 30 MeV, based on GNASH calculation, with 825 1451 234 adjustments made to improve agreement with experimental data, 825 1451 235 especially data of Bormann et al. [Bo63]. 825 1451 236 825 1451 237 MT=23 (N,N3ALPHA) CROSS SECTION 825 1451 238 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 239 from 28 to 30 MeV to agree with LA150 data. 825 1451 240 825 1451 241 MT=28 (N,NP) CROSS SECTION 825 1451 242 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 243 such that the production cross sections for the 5.2701 and 5.2988 825 1451 244 MeV gamma rays are consistent with Nelson et al.[Ne99] data, and 825 1451 245 normalization of proton spectra consistent with 27-MeV data of 825 1451 246 Subramanian et al. [Su94]. 825 1451 247 825 1451 248 MT=32 (N,ND) CROSS SECTION 825 1451 249 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 250 such that difference between total and nonelastic cross sections 825 1451 251 agrees with elastic cross section measurements. 825 1451 252 825 1451 253 MT=41 (N,2NP) CROSS SECTION 825 1451 254 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 255 such that difference between total and nonelastic cross sections 825 1451 256 agrees with elastic cross section measurements. 825 1451 257 825 1451 258 MT=44 (N,N2P) CROSS SECTION 825 1451 259 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 260 such that difference between total and nonelastic cross sections 825 1451 261 agrees with elastic cross section measurements. 825 1451 262 825 1451 263 MT=45 (N,NPALPHA) CROSS SECTION 825 1451 264 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 265 such that difference between total and nonelastic cross sections 825 1451 266 agrees with elastic cross section measurements. 825 1451 267 825 1451 268 MT=91 (N,N'CONTINUUM) CROSS SECTION 825 1451 269 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 270 such that difference between total and nonelastic cross sections 825 1451 271 agrees with elastic cross section measurements. 825 1451 272 825 1451 273 MT=102 (N,GAMMA) CROSS SECTION 825 1451 274 0 to 1 MeV,cross section based on experimental data obtained 825 1451 275 from E. Jurney [Ju64]; higher energy data is crude estimate. 825 1451 276 825 1451 277 MT=103 (N,P) CROSS SECTION 825 1451 278 Sum of MT=600-603. 825 1451 279 825 1451 280 MT=104 (N,D) CROSS SECTION 825 1451 281 Sum of MT=650-669. 825 1451 282 825 1451 283 MT=105 (N,T) CROSS SECTION 825 1451 284 Sum of MT=700-709,749. 825 1451 285 825 1451 286 MT=107 (N,ALPHA) CROSS SECTION 825 1451 287 Sum of MT=800-803. 825 1451 288 825 1451 289 MT=108 (N,2ALPHA) CROSS SECTION 825 1451 290 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 291 such that difference between total and nonelastic cross sections 825 1451 292 agrees with elastic cross section measurements. 825 1451 293 825 1451 294 MT=112 (N,PALPHA) CROSS SECTION 825 1451 295 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 296 such that difference between total and nonelastic cross sections 825 1451 297 agrees with elastic cross section measurements. 825 1451 298 825 1451 299 MT=600 (N,P) INTEGRATED CROSS SECTION TO 16N GROUND STATE 825 1451 300 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 301 renormalization (lowered approximately 30%) from comparison of 825 1451 302 excited state predictions with Nelson et al. [Ne99] 825 1451 303 measurements. 825 1451 304 825 1451 305 MT=601-603 (N,P) CROSS SECTION TO EXCITED LEVELS OF 16N 825 1451 306 Threshold to 30 MeV, the cross sections for the 0.0.297- and 825 1451 307 0.3975-MeV levels are inferred from the (n,p gamma) data of 825 1451 308 Nelson et al. [Ne99], using the level structure diagram of 16N 825 1451 309 by Ajzenberg-Selove [Aj86]. The cross section for the 0.1201- 825 1451 310 MeV level is based on GNASH calculations with some 825 1451 311 renormalization (lowered ~30%) from comparison of excited state 825 1451 312 predictions with Nelson et al. [Ne99] measurements. 825 1451 313 825 1451 314 MT=650 (N,D) INTEGRATED CROSS SECTION TO 15N GROUND STATE 825 1451 315 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 316 renormalization from comparison of excited state predictions 825 1451 317 with Nelson et al. [Ne99] measurements. 825 1451 318 825 1451 319 MT=651-669 (N,D) CROSS SECTION TO EXCITED LEVELS OF 15N 825 1451 320 Threshold to 30 MeV, the cross sections for the 5.2701- and 825 1451 321 5.2988-MeV levels are adjusted based on the (n,xgamma) data of 825 1451 322 Nelson et al. [Ne99], using the level structure diagram for 15N 825 1451 323 by Ajzenberg-Selove [Aj91]. Cross sections for remaining levels 825 1451 324 are based on GNASH calculations with some renormalization from 825 1451 325 comparison of excited state predictions with Nelson et al. 825 1451 326 [Ne99] measurements and 27-Mev data of Subramanian et al. [Su94]. 825 1451 327 825 1451 328 MT=700 (N,T) INTEGRATED CROSS SECTION TO 14N GROUND STATE 825 1451 329 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 330 renormalization from comparison of excited state predictions 825 1451 331 with Nelson et al. [Ne99] measurements. 825 1451 332 825 1451 333 MT=701-709 (N,T) CROSS SECTION TO EXCITED LEVELS OF 14N 825 1451 334 Threshold to 30 MeV, the cross section for the 2.3128-MeV 825 1451 335 levels is inferred from the (n,t gamma) data of Nelson et al. 825 1451 336 [Ne99], using the level structure diagram for 16N by Ajzenberg- 825 1451 337 Selove [Aj91]. Cross sections for the remaining levels are 825 1451 338 based on GNASH calculations with some renormalization from 825 1451 339 comparison of excited state predictions with Nelson et al. 825 1451 340 [Ne99] measurements. 825 1451 341 825 1451 342 MT=749 (N,T) CROSS SECTION TO 14N CONTINUUM 825 1451 343 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 344 renormalization from comparison of excited state predictions 825 1451 345 with Nelson et al. [Ne99] measurements and to enhance agreement 825 1451 346 of elastic cross section with measured data. 825 1451 347 825 1451 348 MT=800 (N,ALPHA0) CROSS SECTION TO 13C GROUND STATE 825 1451 349 0.0 to 6.2 MeV, based on R-matrix analysis described above 825 1451 350 under MT=1. Data of Ba72 were used in the original (alpha,n) 825 1451 351 direction, with no changes in energy scale or normalization. 825 1451 352 Also included were the low-energy (alpha,n) data of [Ke91] and 825 1451 353 [Dr93]. 825 1451 354 6.2 to 20 MeV, based on data of [Da63],[Da68],[Si68],[Ba73], 825 1451 355 and composite of [Mc66b],[Ma68],[Le68] at 14 MeV. Note that the 825 1451 356 [Da63] data were renormalized by factor of 1.5 to bring them 825 1451 357 into rough agreement with the R-matrix analysis of the [Ba73] 825 1451 358 (n,a0) data, together with the total and elastic data in the 825 1451 359 analysis. Because the [Da68] experimental data were normalized 825 1451 360 to [Da63], the former were also renormalized by the factor of 825 1451 361 1.5. 825 1451 362 825 1451 363 MT=801-803 (N,ALPHA) CROSS SECTION TO EXCITED LEVELS OF 13C 825 1451 364 Threshold to 30 MeV, the cross sections of the 3.0894-, 825 1451 365 3.6845-, and 3.8538-MeV levels are inferred from the (n,alpha 825 1451 366 gamma) data of Nelson et al. [Ne99], using the level structure 825 1451 367 diagram of 13C by Ajzenberg-Selove [Aj91]. 825 1451 368 825 1451 369 MF=4 ANGULAR DISTRIBUTIONS ------------------------------------ 825 1451 370 825 1451 371 MT=2 ELASTIC NEUTRON ANGULAR DISTRIBUTIONS 825 1451 372 0.0 to 3.4 MeV, calculated from R-function fit (see MF=3,MT=1). 825 1451 373 3.4 to 6.2 MeV, calculated from R-matrix fit (see MF=3,MT=1). 825 1451 374 Measured angular distributions input to the fit were those of 825 1451 375 [Ch61],[Fo58],[Fo70],[Hi58],[Hu62], [Jo67],[Ki72],[La60],[Li66], 825 1451 376 [Ma62],[Ph61],[Jo79]. Fits were attempted using new data of 825 1451 377 [Sc77], but those measurements were found to have significant 825 1451 378 uncertainties, and some discrepancies with other data were noted. 825 1451 379 6.2 to 20 MeV, smooth curve through coefficients derived from 825 1451 380 fits to elastic data of [Ph61],[Ne72],[Ch61],[Ba63],[Be67], 825 1451 381 [Mc66a],[Ki72],[Bu73],[Ne72],[Gl82],[Ba85],[Bo89],[Pe85]. 825 1451 382 825 1451 383 MT=51-57 DISCRETE (N,N') ANGULAR DISTRIBUTIONS 825 1451 384 Threshold to 10 MeV, assumed isotropic in center of mass. 825 1451 385 Above 10 MeV, based on fits of the 14-MeV data of [Ki72],[Ne72], 825 1451 386 [Ba63],[Mc66a],[Ba85],[Me69], and especially [Bo89]. 825 1451 387 825 1451 388 MT=600-603 DISCRETE (N,P) ANGULAR DISTRIBUTIONS 825 1451 389 Threshold to 30 MeV, assumed isotropic in center of mass. 825 1451 390 825 1451 391 MT=650-669 DISCRETE (N,D) ANGULAR DISTRIBUTIONS 825 1451 392 Threshold to 30 MeV, assumed isotropic in center of mass. 825 1451 393 825 1451 394 MT=700-709 DISCRETE (N,T) ANGULAR DISTRIBUTIONS 825 1451 395 Threshold to 30 MeV, assumed isotropic in center of mass. 825 1451 396 825 1451 397 MT=800 DISCRETE(N,ALPHA0) ANGULAR DISTRIBUTIONS 825 1451 398 0.0 to 6.2 MeV, calculated from R-Matrix fit (see MF=3,MT=1). 825 1451 399 Measured angular distributions input to the fit were 825 1451 400 reconstructed from the Legendre coefficients of [Wa57], and 825 1451 401 converted to (n,alpha) angular distributions using detailed 825 1451 402 balance. 825 1451 403 825 1451 404 MT=801-803 DISCRETE (N,T) ANGULAR DISTRIBUTIONS 825 1451 405 Threshold to 6 MeV, 825 1451 406 6 to 30 MeV, assumed isotropic in center of mass. 825 1451 407 825 1451 408 MF=6 PRODUCT ENERGY-ANGLE DISTRIBUTIONS ----------------------- 825 1451 409 825 1451 410 MT=16 (N,2N) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 411 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 412 are given for neutrons, and isotropic energy spectra are given 825 1451 413 for recoiling 15O nuclei. The neutron data were obtained from 825 1451 414 the GNASH calculations; the recoil 15O distributions were 825 1451 415 calculated with the RECOIL code [Ma83]. The discrete gamma rays 825 1451 416 from (n,2ngamma) reactions are given in MF=13 and 14. 825 1451 417 825 1451 418 MT=22 (N,NALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 419 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 420 are given for neutrons and alpha particles, and isotropic energy 825 1451 421 spectra are given for recoiling 12C nuclei. The neutron and 825 1451 422 alpha data were obtained from the GNASH calculations; the recoil 825 1451 423 12C distributions were calculated with the RECOIL code [Ma83]. 825 1451 424 The discrete gamma rays from (n,nalpha gamma) reactions are 825 1451 425 given in MF=13 and 14. 825 1451 426 825 1451 427 MT=28 (N,NP) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 428 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 429 are given for neutrons and protons; isotropic energy spectra are 825 1451 430 given for recoiling 15N nuclei; and isotropic energy spectra are 825 1451 431 given for emitted continuum gamma rays. The neutron, proton, 825 1451 432 and gamma-ray data were obtained from the GNASH calculations; 825 1451 433 the recoil 15N distributions were calculated with the RECOIL 825 1451 434 code [Ma83]. 825 1451 435 825 1451 436 MT=32 (N,ND) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 437 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 438 are given for neutrons and deuterons; isotropic energy spectra 825 1451 439 are given for recoiling 14N nuclei; and isotropic energy spectra 825 1451 440 are given for emitted continuum gamma rays. The neutron, 825 1451 441 deuteron, and gamma-ray data were obtained from the GNASH 825 1451 442 calculations; the recoil 14N distributions were calculated with 825 1451 443 the RECOIL code [Ma83]. 825 1451 444 825 1451 445 MT=41 (N,2NP) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 446 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 447 are given for neutrons and protons; isotropic energy spectra are 825 1451 448 given for recoiling 14N nuclei; and isotropic energy spectra are 825 1451 449 given for emitted continuum gamma rays. The neutron, proton, 825 1451 450 and gamma-ray data were obtained from the GNASH calculations; 825 1451 451 the recoil 14N distributions were calculated with the RECOIL 825 1451 452 code [Ma83]. 825 1451 453 825 1451 454 MT=44 (N,N2P) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 455 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 456 are given for neutrons and protons; isotropic energy spectra are 825 1451 457 given for recoiling 14C nuclei; and isotropic energy spectra are 825 1451 458 given for emitted continuum gamma rays. The neutron, proton, 825 1451 459 and gamma-ray data were obtained from the GNASH calculations; 825 1451 460 the recoil 14C distributions were calculated with the RECOIL 825 1451 461 code [Ma83]. 825 1451 462 825 1451 463 MT=45 (N,NPALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 464 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 465 are given for neutrons, protons, and alphas; isotropic energy 825 1451 466 spectra are given for recoiling 11B nuclei; and isotropic energy 825 1451 467 spectra are given for emitted continuum gamma rays. The 825 1451 468 neutron, proton, alpha, and gamma-ray data were obtained from 825 1451 469 the GNASH calculations; the recoil 11B distributions were 825 1451 470 calculated with the RECOIL code [Ma83]. 825 1451 471 825 1451 472 MT=91 (N,N'CONTINUUM) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 473 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 474 are given for neutrons; isotropic energy spectra are given for 825 1451 475 recoiling 16O nuclei; and isotropic energy spectra are given for 825 1451 476 emitted continuum gamma rays. The neutron and gamma-ray data 825 1451 477 were obtained from the GNASH calculations; the recoil 16O 825 1451 478 distributions were calculated with the RECOIL code [Ma83]. 825 1451 479 825 1451 480 MT=108 (N,2ALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 481 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 482 are given for alphas; isotropic energy spectra are given for 825 1451 483 recoiling 9Be nuclei; and isotropic energy spectra are given for 825 1451 484 emitted continuum gamma rays. The alpha, and gamma-ray data 825 1451 485 were obtained from the GNASH calculations; the recoil 9Be 825 1451 486 distributions were calculated with the RECOIL code [Ma83]. 825 1451 487 825 1451 488 MT=112 (N,PALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 489 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 490 are given for protons, and alphas; isotropic energy spectra are 825 1451 491 given for recoiling 12B nuclei; and isotropic energy spectra are 825 1451 492 given for emitted continuum gamma rays. The proton, alpha, and 825 1451 493 gamma-ray data were obtained from the GNASH calculations; the 825 1451 494 recoil 12B distributions were calculated with the RECOIL code 825 1451 495 [Ma83]. 825 1451 496 825 1451 497 MT=749 (N,ALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 498 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 499 are given for alpha particles; isotropic energy spectra are 825 1451 500 given for recoiling 13C nuclei; and isotropic energy spectra are 825 1451 501 given for emitted continuum gamma rays. The alpha and gamma-ray 825 1451 502 data were obtained from the GNASH calculations; the recoil 13C 825 1451 503 distributions were calculated with the RECOIL code [Ma83]. 825 1451 504 825 1451 505 MF=12 PHOTON PRODUCTION MULTIPLICITIES ------------------------ 825 1451 506 825 1451 507 MT=102 (N,GAMMA) PHOTON PRODUCTION MULTIPLICITIES 825 1451 508 Photon multiplicities for radiative capture are based on 825 1451 509 experimental data obtained from Jurney [Ju64]. 825 1451 510 825 1451 511 MF=13 PHOTON PRODUCTION CROSS SECTIONS ------------------------ 825 1451 512 825 1451 513 MT=4 (N,N'GAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 514 Threshold to 30 MeV: Based almost entirely on new angular 825 1451 515 distribution measurements by Nelson et al. [Ne99], which 825 1451 516 utilized a white neutron source and covered the energy range 825 1451 517 from threshold to 200 MeV. The measurements were made at 7 825 1451 518 angles using high-resolution Ge detectors and resulted in data 825 1451 519 for some 23 gamma rays from 7 different reactions. The angular 825 1451 520 distributions were fit with Legendre expansions to obtain angle- 825 1451 521 integrated cross sections. The fitted cross sections were 825 1451 522 smoothed somewhat for this evaluation, although much of the 825 1451 523 measured structure was preserved, particularly for the intense 825 1451 524 6.129-MeV gamma. The evaluated data for the following gamma 825 1451 525 rays are based directly on the measurements: 825 1451 526 825 1451 527 EG= 2.742 MeV (decay of 8.8719-MeV level of 16O) 825 1451 528 EG= 3.839 MeV (decay of 10.957-MeV level of 16O) 825 1451 529 EG= 4.950 MeV (decay of 11.080-MeV level of 16O) 825 1451 530 EG= 6.130 MeV (decay of 6.130-MeV level of 16O) 825 1451 531 EG= 6.917 MeV (decay of 6.917-MeV level of 16O) 825 1451 532 EG= 7.117 MeV (decay of 7.117-MeV level of 16O) 825 1451 533 825 1451 534 The evaluated cross sections for the remaining (n,n') gamma 825 1451 535 rays are inferred from these data using the energy level scheme 825 1451 536 of Ajzenberg-Selove [Aj86]. Data were also obtained for gamma 825 1451 537 rays of energy 1.755 and 1.955 from decay of the 8.8719-MeV 825 1451 538 level but the 2.742-MeV gamma was used to determine the level 825 1451 539 excitation cross section because it is the most intense. 825 1451 540 Similarly, data were obtained on a 4.179-MeV gamma from decay of 825 1451 541 the 11.080-MeV level, but the 4.950-MeV gamma is more intense 825 1451 542 and was used to determine the level excitation cross section. 825 1451 543 The evaluated data were compared to older gamma-ray 825 1451 544 measurements by [Be70], [Ne90], [No78], [Ha59], [Di70], [Or70], 825 1451 545 [Dr70], [Cl69], [Lu70], [Bu71], [Ny69]. Considering that very 825 1451 546 few (e.g., [Be70], [Dr70]) of these measurements are of full 825 1451 547 angular distributions, the agreement is reasonable. 825 1451 548 825 1451 549 MT=16 (N,2NGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 550 Threshold to 30 MeV: The cross section for the 5.2409-MeV 825 1451 551 gamma ray was obtained directly from the Nelson et al. [Ne99] 825 1451 552 data. The remaining discrete gammas are based on GNASH 825 1451 553 calculations, with some renomalization based on the experimental 825 1451 554 data. 825 1451 555 825 1451 556 MT=22 (N,NALPHA GAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 557 Threshold to 30 MeV: Only the 4.438-MeV discrete gamma ray 825 1451 558 is given and it is based on the Nelson et al. [Ne99] data. 825 1451 559 825 1451 560 MT=103 (N,PGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 561 Threshold to 30 MeV: The cross sections for the 0.2774- and 825 1451 562 0.297-MeV gamma rays are based on the Nelson et al. [Ne99] data. 825 1451 563 The 0.3975-MeV gamma is inferred from the 0.2774-MeV gamma data 825 1451 564 through the Ajzenberg-Selove level scheme [Aj86] for 16N. The 825 1451 565 0.1201-MeV gamma cross section is based partially on GNASH 825 1451 566 calculations and partially inferred from the [Ne99] data using 825 1451 567 the 16N level scheme. 825 1451 568 825 1451 569 MT=104 (N,DGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 570 Threshold to 30 MeV: The cross sections for the 5.2701- and 825 1451 571 5.2988-MeV gamma rays are based on the Nelson et al. [Ne99] 825 1451 572 data. The cross sections for the remaining 60 (n,dg) gamma rays 825 1451 573 are based on GNASH calculations and the Ajzenberg-Selove level 825 1451 574 scheme [Aj91] for 15N, after renomalization to agree with the 825 1451 575 measured 5.2701- and 5.2988-MeV gamma-ray data. 825 1451 576 825 1451 577 MT=105 (N,TGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 578 Threshold to 30 MeV: The cross section for the 2.313-MeV 825 1451 579 gamma ray is based on the Nelson et al. [Ne99] measurement. The 825 1451 580 cross sections for the remaining 20 (n,tg) gamma rays are based 825 1451 581 on GNASH calculations and the Ajzenberg-Selove level scheme 825 1451 582 [Aj91] for 14N, after renomalization to agree with the measured 825 1451 583 2.313-MeV gamma-ray data. 825 1451 584 825 1451 585 MT=107 (N,ALPHA GAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 586 Threshold to 30 MeV: The cross sections for the 3.0894-, 825 1451 587 3.6845- and 3.8538-MeV gamma rays are based on the Nelson et 825 1451 588 al. [Ne99] data. The 0.1693-, 0.5951- and 0.7644-MeV gamma-ray 825 1451 589 cross sections are inferred from the above data through the 825 1451 590 Ajzenberg-Selove level scheme [Aj91]. Note that the 0.1693-MeV 825 1451 591 gamma from decay of the 3.8538-MeV level also was measured, but 825 1451 592 the 3.8538-MeV gamma is more intense and was used to determine 825 1451 593 the level excitation cross section. 825 1451 594 825 1451 595 MF=14 PHOTON ANGULAR DISTRIBUTIONS ---------------------------- 825 1451 596 825 1451 597 MT=4 (N,N'GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 598 Anisotropic angular distributions in Legendre polynomial 825 1451 599 representation are given for the 1.755-, 2.742-, 6.130-, 6.917-, 825 1451 600 and 7.117-MeV gamma rays, obtained by fitting the measurements 825 1451 601 of Nelson et al. [Ne99]. Isotropic angular distributions are 825 1451 602 assumed for the remaining gamma rays. 825 1451 603 825 1451 604 MT=16 (N,2NGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 605 An anisotropic angular distribution in Legendre polynomial 825 1451 606 representation is given for the 5.2409-MeV gamma ray, obtained 825 1451 607 by fitting the measurements of Nelson et al. [Ne99]. Isotropic 825 1451 608 angular distributions are assumed for the remaining gamma rays. 825 1451 609 825 1451 610 MT=22 (N,NALPHA GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 611 An anisotropic angular distribution in Legendre polynomial 825 1451 612 representation is given for the 4.438-MeV gamma ray, obtained by 825 1451 613 fitting the measurements of Nelson et al. [Ne99]. 825 1451 614 825 1451 615 MT=102 (N,GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 616 All gamma rays from radiative capture are assumed to be 825 1451 617 isotropic. 825 1451 618 825 1451 619 MT=103 (N,PGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 620 Anisotropic angular distributions in Legendre polynomial 825 1451 621 representation are given for the 0.2774-, 0.297-, and 0.3975-MeV 825 1451 622 gamma rays, obtained by fitting the measurements of Nelson et 825 1451 623 al. [Ne99]. The angular distributions for all remaining gamma 825 1451 624 rays are assumed to be isotropic. 825 1451 625 825 1451 626 MT=104 (N,DGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 627 An anisotropic angular distribution in Legendre polynomial 825 1451 628 representation is given for the 5.2701-MeV gamma ray, obtained 825 1451 629 by fitting the measurements of Nelson et al. [Ne99]. The 825 1451 630 angular distributions for all remaining gamma rays are assumed 825 1451 631 to be isotropic. 825 1451 632 825 1451 633 MT=105 (N,TGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 634 All gamma rays from (n,tg) reactions are assumed to be 825 1451 635 isotropic. 825 1451 636 825 1451 637 MT=107 (N,ALPHA GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 638 Anisotropic angular distributions in Legendre polynomial 825 1451 639 representation are given for the 0.1693-, 3.6845- and 3.8538- 825 1451 640 MeV gamma rays, obtained by fitting the measurements of Nelson 825 1451 641 et al. [Ne99]. Isotropic angular distributions are assumed for 825 1451 642 all the remaining gamma rays. 825 1451 643 825 1451 644 **************************************************************** 825 1451 645 825 1451 646 SUMMARY OF DATA VALIDATION OF THIS FILE AGAINST INTEGRAL 825 1451 647 BENCHMARKS 825 1451 648 825 1451 649 KAPL (Weinman, Caro, Lubitz) performed a number of data 825 1451 650 validation benchmark calculations to test the performance of this 825 1451 651 file (June-August 2001). This O16 evaluation gives consistently 825 1451 652 good results for the 21 CSWEG solution critical calculations, the 825 1451 653 liquid-oxygen broomstick neutron-transmission experiment, and the 825 1451 654 neutron age in water experiment (see below for more details). 825 1451 655 825 1451 656 A) 21 CSWEG solution critical calculations. Weinman calculated a 825 1451 657 set of 21 ORNL and Rocky Flats benchmark solution criticals used 825 1451 658 for CSEWG analyses. These calculations were run with ENDF/B-VI 825 1451 659 release 5 U235 (Leal,Larson,wright,Derrien) and hydrogen (332.0 825 1451 660 mbarns 2200m/s). Four different oxygen 16 cross section 825 1451 661 evaluations were considered. 825 1451 662 825 1451 663 1. KAPL-Caro 825 1451 664 2. This evaluation (which contains the KAPL data below 3.4 MeV) 825 1451 665 3. ENDF/B-VI MOD 2 825 1451 666 4. JENDL 3.2 825 1451 667 825 1451 668 All four O16 cross section evaluations gave good reactivity 825 1451 669 responses versus our fitting parameter above-thermal-leakage ATL. 825 1451 670 The ATL parameter is a sensitive trending variable to high energy 825 1451 671 scattering cross sections. All four O16 evaluations produced 825 1451 672 eigenvalues whose mean values were all close to unity and only 825 1451 673 the older ENDF/B-VI.2 cross section evaluation gave a slight 825 1451 674 reactivity trend (about .0020 Delta Keff over the range). The 825 1451 675 average eigenvalues and slopes are listed below. 825 1451 676 825 1451 677 Library Av. Keff Slope 825 1451 678 825 1451 679 KAPL-Caro 0.9993 +.0001 825 1451 680 This file 0.9996 +.0004 825 1451 681 ENDF/B-VI.2 1.0003 +.0032 825 1451 682 JENDL 3.2 1.0004 -.0002 825 1451 683 825 1451 684 Thus the reactivity trend, labeled "slope" in the table above, is 825 1451 685 much smaller in the new file compared to the previous ENDF/B-VI.2 825 1451 686 evaluation. 825 1451 687 825 1451 688 B) The liquid-oxygen broomstick experiment. The oxygen window at 825 1451 689 2.3 MeV is the most important feature at which energy the 825 1451 690 greatest transmission takes place. The new evaluation produces 825 1451 691 close to exact agreement with the experiment in the energy range 825 1451 692 of the oxygen window. The previous ENDF/B-VI value is slightly 825 1451 693 below the experimental value. At energies higher than 5.5 MeV, 825 1451 694 the new evaluation produces slightly better results than does the 825 1451 695 previous ENDF/B-VI results. 825 1451 696 825 1451 697 C) Neutron age in water. KAPL obtained 26.4 to be compared 825 1451 698 against an experimental value of 26.6 +/- 0.6. The previous 825 1451 699 ENDF/B-VI file gave a result of 26.3. 825 1451 700 825 1451 701 Additionally, A.C. (Skip) Kahler at Bettis lab undertook 825 1451 702 benchmark testing of this file (memo, May 16, 2001) against 825 1451 703 thermal benchmarks documented in the Int. Handbook of Evaluated 825 1451 704 Criticality Safety Benchmark Experiments, as well as the L5 and 825 1451 705 L6 ORNL benchmarks. 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Chadwick, Los Alamos 825 1451 817 report LA-12343-MS (1992) 825 1451 818 825 1451 819 ************************ C O N T E N T S *********************** 825 1451 820 1 451 964 3 825 1451 821 2 151 4 3 825 1451 822 3 1 775 3 825 1451 823 3 2 775 3 825 1451 824 3 3 775 3 825 1451 825 3 4 97 3 825 1451 826 3 5 38 3 825 1451 827 3 16 32 3 825 1451 828 3 22 50 3 825 1451 829 3 23 33 3 825 1451 830 3 28 41 3 825 1451 831 3 32 20 3 825 1451 832 3 41 15 3 825 1451 833 3 44 16 3 825 1451 834 3 45 14 3 825 1451 835 3 51 97 3 825 1451 836 3 52 96 3 825 1451 837 3 53 90 3 825 1451 838 3 54 88 3 825 1451 839 3 55 74 3 825 1451 840 3 56 63 3 825 1451 841 3 57 62 3 825 1451 842 3 91 69 3 825 1451 843 3 102 5 3 825 1451 844 3 103 60 3 825 1451 845 3 104 64 3 825 1451 846 3 105 41 3 825 1451 847 3 107 406 3 825 1451 848 3 108 39 3 825 1451 849 3 112 22 3 825 1451 850 3 600 60 3 825 1451 851 3 601 59 3 825 1451 852 3 602 58 3 825 1451 853 3 603 57 3 825 1451 854 3 650 64 3 825 1451 855 3 651 41 3 825 1451 856 3 652 41 3 825 1451 857 3 653 37 3 825 1451 858 3 654 34 3 825 1451 859 3 655 33 3 825 1451 860 3 656 32 3 825 1451 861 3 657 29 3 825 1451 862 3 658 27 3 825 1451 863 3 659 25 3 825 1451 864 3 660 25 3 825 1451 865 3 661 25 3 825 1451 866 3 662 24 3 825 1451 867 3 663 23 3 825 1451 868 3 664 22 3 825 1451 869 3 665 22 3 825 1451 870 3 666 21 3 825 1451 871 3 667 20 3 825 1451 872 3 668 20 3 825 1451 873 3 669 19 3 825 1451 874 3 700 41 3 825 1451 875 3 701 32 3 825 1451 876 3 702 26 3 825 1451 877 3 703 23 3 825 1451 878 3 704 23 3 825 1451 879 3 705 21 3 825 1451 880 3 706 20 3 825 1451 881 3 707 20 3 825 1451 882 3 708 19 3 825 1451 883 3 709 17 3 825 1451 884 3 749 6 3 825 1451 885 3 800 406 3 825 1451 886 3 801 217 3 825 1451 887 3 802 162 3 825 1451 888 3 803 134 3 825 1451 889 4 2 3867 3 825 1451 890 4 51 84 3 825 1451 891 4 52 84 3 825 1451 892 4 53 66 3 825 1451 893 4 54 64 3 825 1451 894 4 55 50 3 825 1451 895 4 56 2 3 825 1451 896 4 57 2 3 825 1451 897 4 600 2 3 825 1451 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1.500000+6 2.056900+0 825 3 2 1847 1.550000+6 1.961300+0 1.600000+6 1.890200+0 1.620000+6 1.880300+0 825 3 2 1848 1.630000+6 1.902400+0 1.640000+6 2.068300+0 1.642000+6 2.187600+0 825 3 2 1849 1.643000+6 2.283400+0 1.644000+6 2.421900+0 1.645000+6 2.630600+0 825 3 2 1850 1.646000+6 2.961500+0 1.647000+6 3.517500+0 1.648000+6 4.500500+0 825 3 2 1851 1.648500+6 5.250100+0 1.649000+6 6.213700+0 1.649500+6 7.339200+0 825 3 2 1852 1.650000+6 8.388900+0 1.650500+6 8.928200+0 1.651000+6 8.646400+0 825 3 2 1853 1.651500+6 7.715000+0 1.652000+6 6.579200+0 1.653000+6 4.733300+0 825 3 2 1854 1.654000+6 3.649300+0 1.655000+6 3.036800+0 1.656000+6 2.673700+0 825 3 2 1855 1.657000+6 2.445300+0 1.658000+6 2.293700+0 1.659000+6 2.188500+0 825 3 2 1856 1.660000+6 2.112500+0 1.665000+6 1.929100+0 1.670000+6 1.861100+0 825 3 2 1857 1.675000+6 1.826400+0 1.680000+6 1.804500+0 1.682000+6 1.797109+0 825 3 2 1858 1.684000+6 1.791370+0 1.685000+6 1.788800+0 1.686000+6 1.807018+0 825 3 2 1859 1.687000+6 1.854791+0 1.688000+6 1.913920+0 1.689000+6 1.964395+0 825 3 2 1860 1.690000+6 1.984300+0 1.691000+6 1.958873+0 1.692000+6 1.903361+0 825 3 2 1861 1.694000+6 1.787958+0 1.695000+6 1.765500+0 1.696000+6 1.763461+0 825 3 2 1862 1.698000+6 1.759507+0 1.700000+6 1.755900+0 1.720000+6 1.722800+0 825 3 2 1863 1.740000+6 1.692300+0 1.760000+6 1.660600+0 1.780000+6 1.624700+0 825 3 2 1864 1.800000+6 1.579200+0 1.820000+6 1.569700+0 1.822000+6 1.605600+0 825 3 2 1865 1.824000+6 1.683200+0 1.826000+6 1.853000+0 1.828000+6 2.239300+0 825 3 2 1866 1.830000+6 3.096400+0 1.831000+6 3.746300+0 1.832000+6 4.386900+0 825 3 2 1867 1.833000+6 4.736500+0 1.834000+6 4.656700+0 1.835000+6 4.296300+0 825 3 2 1868 1.836000+6 3.868500+0 1.837000+6 3.485600+0 1.838000+6 3.176300+0 825 3 2 1869 1.839000+6 2.934600+0 1.840000+6 2.746600+0 1.842000+6 2.482700+0 825 3 2 1870 1.844000+6 2.312700+0 1.846000+6 2.197500+0 1.848000+6 2.116200+0 825 3 2 1871 1.850000+6 2.056800+0 1.852000+6 2.012600+0 1.854000+6 1.979200+0 825 3 2 1872 1.856000+6 1.953900+0 1.858000+6 1.935100+0 1.860000+6 1.921500+0 825 3 2 1873 1.865000+6 1.906500+0 1.870000+6 1.916100+0 1.875000+6 1.953200+0 825 3 2 1874 1.880000+6 2.028300+0 1.885000+6 2.161500+0 1.890000+6 2.383100+0 825 3 2 1875 1.895000+6 2.712800+0 1.900000+6 3.066000+0 1.905000+6 3.182300+0 825 3 2 1876 1.910000+6 2.959300+0 1.915000+6 2.624800+0 1.920000+6 2.347600+0 825 3 2 1877 1.925000+6 2.151700+0 1.930000+6 2.016700+0 1.935000+6 1.921700+0 825 3 2 1878 1.940000+6 1.852700+0 1.950000+6 1.760200+0 1.960000+6 1.701200+0 825 3 2 1879 1.970000+6 1.659400+0 1.980000+6 1.627500+0 1.990000+6 1.601600+0 825 3 2 1880 2.000000+6 1.579500+0 2.050000+6 1.495100+0 2.100000+6 1.422000+0 825 3 2 1881 2.150000+6 1.338900+0 2.200000+6 1.220500+0 2.220000+6 1.152100+0 825 3 2 1882 2.240000+6 1.062400+0 2.260000+6 9.414400-1 2.280000+6 7.772500-1 825 3 2 1883 2.300000+6 5.632600-1 2.305000+6 5.035000-1 2.310000+6 4.426600-1 825 3 2 1884 2.315000+6 3.819600-1 2.320000+6 3.229400-1 2.321000+6 3.115000-1 825 3 2 1885 2.322000+6 3.002100-1 2.323000+6 2.891000-1 2.324000+6 2.781800-1 825 3 2 1886 2.325000+6 2.674600-1 2.326000+6 2.569600-1 2.327000+6 2.467100-1 825 3 2 1887 2.328000+6 2.367100-1 2.329000+6 2.269800-1 2.330000+6 2.175400-1 825 3 2 1888 2.331000+6 2.084100-1 2.332000+6 1.996100-1 2.333000+6 1.911400-1 825 3 2 1889 2.334000+6 1.830300-1 2.335000+6 1.752900-1 2.336000+6 1.679300-1 825 3 2 1890 2.337000+6 1.609700-1 2.338000+6 1.544200-1 2.339000+6 1.483000-1 825 3 2 1891 2.340000+6 1.426100-1 2.341000+6 1.373700-1 2.342000+6 1.325900-1 825 3 2 1892 2.343000+6 1.282800-1 2.344000+6 1.244300-1 2.345000+6 1.210700-1 825 3 2 1893 2.346000+6 1.182000-1 2.347000+6 1.158200-1 2.348000+6 1.139300-1 825 3 2 1894 2.349000+6 1.125300-1 2.350000+6 1.116400-1 2.351000+6 1.112400-1 825 3 2 1895 2.352000+6 1.113300-1 2.353000+6 1.119200-1 2.354000+6 1.130000-1 825 3 2 1896 2.354170+6 1.132245-1 2.355000+6 1.145500-1 2.355318+6 1.151584-1 825 3 2 1897 2.355319+6 1.151604-1 2.355357+6 1.152358-1 2.357000+6 1.190900-1 825 3 2 1898 2.358000+6 1.220600-1 2.359000+6 1.254800-1 2.360000+6 1.293300-1 825 3 2 1899 2.361000+6 1.336200-1 2.362000+6 1.383300-1 2.363000+6 1.434400-1 825 3 2 1900 2.364000+6 1.489400-1 2.365000+6 1.548200-1 2.366000+6 1.610600-1 825 3 2 1901 2.367000+6 1.676500-1 2.368000+6 1.745700-1 2.370000+6 1.893400-1 825 3 2 1902 2.375000+6 2.309700-1 2.380000+6 2.776700-1 2.390000+6 3.788800-1 825 3 2 1903 2.400000+6 4.807000-1 2.410000+6 5.755000-1 2.420000+6 6.596800-1 825 3 2 1904 2.430000+6 7.322800-1 2.440000+6 7.938100-1 2.450000+6 8.454400-1 825 3 2 1905 2.460000+6 8.885300-1 2.470000+6 9.244200-1 2.480000+6 9.542700-1 825 3 2 1906 2.490000+6 9.791200-1 2.500000+6 9.998100-1 2.520000+6 1.031400+0 825 3 2 1907 2.540000+6 1.053300+0 2.560000+6 1.068400+0 2.580000+6 1.078600+0 825 3 2 1908 2.600000+6 1.085300+0 2.650000+6 1.092500+0 2.700000+6 1.092800+0 825 3 2 1909 2.750000+6 1.091200+0 2.800000+6 1.091900+0 2.850000+6 1.100500+0 825 3 2 1910 2.860000+6 1.104800+0 2.870000+6 1.112100+0 2.880000+6 1.130700+0 825 3 2 1911 2.882000+6 1.140000+0 2.884000+6 1.156500+0 2.886000+6 1.195200+0 825 3 2 1912 2.887000+6 1.244200+0 2.888000+6 1.391800+0 2.888200+6 1.462900+0 825 3 2 1913 2.888400+6 1.574300+0 2.888500+6 1.655800+0 2.888600+6 1.765300+0 825 3 2 1914 2.888700+6 1.916200+0 2.888800+6 2.127900+0 2.888900+6 2.420600+0 825 3 2 1915 2.889000+6 2.774800+0 2.889100+6 3.001000+0 2.889200+6 2.737500+0 825 3 2 1916 2.889300+6 2.095300+0 2.889400+6 1.563200+0 2.889500+6 1.260900+0 825 3 2 1917 2.889600+6 1.107000+0 2.889700+6 1.030200+0 2.889800+6 9.921497-1 825 3 2 1918 2.890000+6 9.665597-1 2.890500+6 9.772397-1 2.891000+6 9.985097-1 825 3 2 1919 2.892000+6 1.028300+0 2.894000+6 1.057400+0 2.896000+6 1.071500+0 825 3 2 1920 2.898000+6 1.080000+0 2.900000+6 1.085800+0 2.950000+6 1.136999+0 825 3 2 1921 3.000000+6 1.206495+0 3.005000+6 1.229594+0 3.005500+6 1.237094+0 825 3 2 1922 3.006000+6 1.250994+0 3.006100+6 1.255494+0 3.006200+6 1.260894+0 825 3 2 1923 3.006300+6 1.267794+0 3.006400+6 1.276794+0 3.006500+6 1.288894+0 825 3 2 1924 3.006600+6 1.306294+0 3.006700+6 1.333294+0 3.006800+6 1.380394+0 825 3 2 1925 3.006900+6 1.479694+0 3.007000+6 1.782594+0 3.007100+6 3.063894+0 825 3 2 1926 3.007200+6 1.312494+0 3.007300+6 1.128394+0 3.007400+6 1.127994+0 825 3 2 1927 3.007500+6 1.139494+0 3.007600+6 1.149994+0 3.007700+6 1.158394+0 825 3 2 1928 3.007800+6 1.165094+0 3.007900+6 1.170494+0 3.008000+6 1.174994+0 825 3 2 1929 3.008200+6 1.181894+0 3.008400+6 1.186994+0 3.008600+6 1.190894+0 825 3 2 1930 3.008800+6 1.194094+0 3.009000+6 1.196694+0 3.010000+6 1.205394+0 825 3 2 1931 3.015000+6 1.223693+0 3.020000+6 1.236092+0 3.040000+6 1.286887+0 825 3 2 1932 3.050000+6 1.316184+0 3.060000+6 1.348981+0 3.080000+6 1.426870+0 825 3 2 1933 3.100000+6 1.524055+0 3.120000+6 1.644034+0 3.140000+6 1.789604+0 825 3 2 1934 3.160000+6 1.962262+0 3.170000+6 2.058236+0 3.180000+6 2.160204+0 825 3 2 1935 3.190000+6 2.267764+0 3.200000+6 2.385788+0 3.201000+6 2.399273+0 825 3 2 1936 3.202000+6 2.413554+0 3.203000+6 2.429129+0 3.204000+6 2.446495+0 825 3 2 1937 3.205000+6 2.466746+0 3.206000+6 2.492070+0 3.207000+6 2.526742+0 825 3 2 1938 3.208000+6 2.581499+0 3.209000+6 2.686057+0 3.210000+6 2.951963+0 825 3 2 1939 3.210500+6 3.272821+0 3.211000+6 3.929082+0 3.211100+6 4.120706+0 825 3 2 1940 3.211200+6 4.331318+0 3.211300+6 4.554244+0 3.211400+6 4.776702+0 825 3 2 1941 3.211500+6 4.979195+0 3.211600+6 5.137213+0 3.211700+6 5.226934+0 825 3 2 1942 3.211800+6 5.232328+0 3.211900+6 5.152267+0 3.212000+6 5.000823+0 825 3 2 1943 3.212200+6 4.578611+0 3.212400+6 4.139895+0 3.212600+6 3.772647+0 825 3 2 1944 3.212800+6 3.491673+0 3.213000+6 3.283394+0 3.213200+6 3.129731+0 825 3 2 1945 3.213400+6 3.015301+0 3.213600+6 2.929219+0 3.213800+6 2.863296+0 825 3 2 1946 3.214000+6 2.812343+0 3.214200+6 2.772264+0 3.214400+6 2.740465+0 825 3 2 1947 3.214600+6 2.714951+0 3.214800+6 2.694323+0 3.215000+6 2.677486+0 825 3 2 1948 3.216000+6 2.628692+0 3.217000+6 2.609903+0 3.218000+6 2.603967+0 825 3 2 1949 3.219000+6 2.604308+0 3.220000+6 2.608233+0 3.222000+6 2.621462+0 825 3 2 1950 3.224000+6 2.638174+0 3.226000+6 2.656478+0 3.228000+6 2.675478+0 825 3 2 1951 3.230000+6 2.694674+0 3.235000+6 2.743058+0 3.240000+6 2.790337+0 825 3 2 1952 3.245000+6 2.836012+0 3.250000+6 2.879486+0 3.255000+6 2.920458+0 825 3 2 1953 3.260000+6 2.958829+0 3.265000+6 2.994299+0 3.270000+6 3.026768+0 825 3 2 1954 3.275000+6 3.056137+0 3.280000+6 3.082506+0 3.285000+6 3.105674+0 825 3 2 1955 3.290000+6 3.125741+0 3.295000+6 3.142809+0 3.300000+6 3.156976+0 825 3 2 1956 3.305000+6 3.168344+0 3.310000+6 3.177111+0 3.312000+6 3.179899+0 825 3 2 1957 3.314000+6 3.182286+0 3.316000+6 3.184373+0 3.318000+6 3.186060+0 825 3 2 1958 3.320000+6 3.187347+0 3.322000+6 3.188334+0 3.324000+6 3.188921+0 825 3 2 1959 3.326000+6 3.189309+0 3.328000+6 3.189296+0 3.330000+6 3.189083+0 825 3 2 1960 3.332000+6 3.188571+0 3.334000+6 3.187758+0 3.336000+6 3.186746+0 825 3 2 1961 3.338000+6 3.185433+0 3.340000+6 3.183921+0 3.345000+6 3.179290+0 825 3 2 1962 3.350000+6 3.173460+0 3.355000+6 3.166630+0 3.360000+6 3.158901+0 825 3 2 1963 3.370000+6 3.141743+0 3.380000+6 3.122887+0 3.390000+6 3.103332+0 825 3 2 1964 3.400000+6 3.087500+0 3.400500+6 3.086805+0 3.410000+6 3.074596+0 825 3 2 1965 3.420000+6 3.062263+0 3.430000+6 3.051348+0 3.435000+6 3.052700+0 825 3 2 1966 3.436000+6 3.055914+0 3.437000+6 3.062485+0 3.437500+6 3.068780+0 825 3 2 1967 3.438000+6 3.081273+0 3.438500+6 3.128890+0 3.439000+6 3.878781+0 825 3 2 1968 3.439500+6 3.994489+0 3.440000+6 3.590247+0 3.440500+6 3.722370+0 825 3 2 1969 3.441000+6 4.214025+0 3.441500+6 5.264789+0 3.441600+6 5.465223+0 825 3 2 1970 3.441700+6 5.594964+0 3.441800+6 5.623470+0 3.441900+6 5.541999+0 825 3 2 1971 3.442000+6 5.368579+0 3.442500+6 4.233530+0 3.443000+6 3.637057+0 825 3 2 1972 3.443500+6 3.381517+0 3.444000+6 3.258104+0 3.444500+6 3.190595+0 825 3 2 1973 3.445000+6 3.149838+0 3.450000+6 3.053235+0 3.455000+6 3.037005+0 825 3 2 1974 3.460000+6 3.029114+0 3.465000+6 3.023904+0 3.470000+6 3.019988+0 825 3 2 1975 3.475000+6 3.016868+0 3.480000+6 3.014545+0 3.490000+6 3.011797+0 825 3 2 1976 3.500000+6 3.011145+0 3.510000+6 3.012490+0 3.520000+6 3.015632+0 825 3 2 1977 3.530000+6 3.020271+0 3.540000+6 3.026307+0 3.550000+6 3.033239+0 825 3 2 1978 3.560000+6 3.040966+0 3.570000+6 3.048990+0 3.580000+6 3.056908+0 825 3 2 1979 3.590000+6 3.064420+0 3.600000+6 3.071026+0 3.610000+6 3.076325+0 825 3 2 1980 3.620000+6 3.079816+0 3.630000+6 3.081197+0 3.640000+6 3.080165+0 825 3 2 1981 3.642000+6 3.079631+0 3.644000+6 3.078975+0 3.645000+6 3.078580+0 825 3 2 1982 3.645200+6 3.078532+0 3.645400+6 3.078454+0 3.645600+6 3.078411+0 825 3 2 1983 3.645800+6 3.078297+0 3.646000+6 3.078180+0 3.646200+6 3.078158+0 825 3 2 1984 3.646400+6 3.078294+0 3.646600+6 3.078034+0 3.646800+6 3.077851+0 825 3 2 1985 3.647000+6 3.077737+0 3.647200+6 3.077660+0 3.647400+6 3.077566+0 825 3 2 1986 3.647600+6 3.077524+0 3.647800+6 3.077459+0 3.648000+6 3.077280+0 825 3 2 1987 3.649000+6 3.076816+0 3.650000+6 3.076317+0 3.651000+6 3.075808+0 825 3 2 1988 3.652000+6 3.075197+0 3.653000+6 3.074584+0 3.654000+6 3.073971+0 825 3 2 1989 3.655000+6 3.073356+0 3.660000+6 3.069581+0 3.665000+6 3.065101+0 825 3 2 1990 3.670000+6 3.059918+0 3.675000+6 3.054030+0 3.680000+6 3.047439+0 825 3 2 1991 3.685000+6 3.040243+0 3.690000+6 3.032542+0 3.695000+6 3.024537+0 825 3 2 1992 3.700000+6 3.016427+0 3.710000+6 3.000988+0 3.720000+6 2.991023+0 825 3 2 1993 3.730000+6 2.998923+0 3.740000+6 3.065868+0 3.745000+6 3.165849+0 825 3 2 1994 3.750000+6 3.395066+0 3.755000+6 3.978216+0 3.760000+6 5.339004+0 825 3 2 1995 3.761000+6 5.629029+0 3.762000+6 5.828192+0 3.763000+6 5.884917+0 825 3 2 1996 3.764000+6 5.782112+0 3.765000+6 5.548266+0 3.766000+6 5.238854+0 825 3 2 1997 3.767000+6 4.908853+0 3.768000+6 4.595445+0 3.769000+6 4.317022+0 825 3 2 1998 3.770000+6 4.078781+0 3.772000+6 3.712151+0 3.774000+6 3.458069+0 825 3 2 1999 3.776000+6 3.279552+0 3.778000+6 3.150410+0 3.780000+6 3.054252+0 825 3 2 2000 3.785000+6 2.896959+0 3.790000+6 2.801524+0 3.795000+6 2.735261+0 825 3 2 2001 3.800000+6 2.684475+0 3.810000+6 2.606340+0 3.820000+6 2.543723+0 825 3 2 2002 3.830000+6 2.488918+0 3.840000+6 2.439215+0 3.850000+6 2.393503+0 825 3 2 2003 3.860000+6 2.351271+0 3.870000+6 2.312303+0 3.880000+6 2.276784+0 825 3 2 2004 3.890000+6 2.244596+0 3.900000+6 2.216019+0 3.920000+6 2.168908+0 825 3 2 2005 3.940000+6 2.134116+0 3.960000+6 2.106465+0 3.980000+6 2.074346+0 825 3 2 2006 4.000000+6 2.011619+0 4.010000+6 1.953242+0 4.020000+6 1.864569+0 825 3 2 2007 4.030000+6 1.737386+0 4.040000+6 1.574436+0 4.050000+6 1.399791+0 825 3 2 2008 4.060000+6 1.251620+0 4.070000+6 1.154243+0 4.080000+6 1.103707+0 825 3 2 2009 4.090000+6 1.082658+0 4.100000+6 1.077278+0 4.110000+6 1.083223+0 825 3 2 2010 4.120000+6 1.106214+0 4.130000+6 1.160348+0 4.140000+6 1.265590+0 825 3 2 2011 4.150000+6 1.437440+0 4.160000+6 1.663060+0 4.165000+6 1.779570+0 825 3 2 2012 4.170000+6 1.885690+0 4.175000+6 1.972910+0 4.180000+6 2.035540+0 825 3 2 2013 4.185000+6 2.072110+0 4.190000+6 2.084140+0 4.195000+6 2.075400+0 825 3 2 2014 4.200000+6 2.050350+0 4.205000+6 2.013250+0 4.210000+6 1.967680+0 825 3 2 2015 4.215000+6 1.916450+0 4.220000+6 1.861520+0 4.225000+6 1.804400+0 825 3 2 2016 4.230000+6 1.746060+0 4.235000+6 1.687060+0 4.240000+6 1.627960+0 825 3 2 2017 4.245000+6 1.568950+0 4.250000+6 1.510480+0 4.255000+6 1.453120+0 825 3 2 2018 4.260000+6 1.398010+0 4.265000+6 1.347340+0 4.270000+6 1.305400+0 825 3 2 2019 4.275000+6 1.279990+0 4.280000+6 1.284940+0 4.285000+6 1.342110+0 825 3 2 2020 4.290000+6 1.475960+0 4.295000+6 1.695160+0 4.300000+6 1.972410+0 825 3 2 2021 4.305000+6 2.255790+0 4.310000+6 2.502910+0 4.315000+6 2.692500+0 825 3 2 2022 4.320000+6 2.816410+0 4.321000+6 2.833210+0 4.322000+6 2.847460+0 825 3 2 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