8-O - 16 ENDF/B-VII.0 Processed by Red Cullen using PREPRO2007. 1 0 0 0 8016.00000 15.8575100 0 0 0 3 825 1451 1 0.0 0.0 0 0 0 6 825 1451 2 1.00000000 30000000.0 8 0 10 7 825 1451 3 12000.0000 0.0 1 0 940 143 825 1451 4 8-O - 16 LANL EVAL-DEC05 Hale,Young,Chadwick,Caro,Lubitz 825 1451 5 CH96AB,CA98,Ch99,Yo01 DIST-DEC06 825 1451 6 ----ENDF/B-VII MATERIAL 825 825 1451 7 -----INCIDENT NEUTRON DATA 825 1451 8 ------ENDF-6 FORMAT 825 1451 9 825 1451 10 ****************************************************************** 825 1451 11 ENDF/B-VI MOD 3 Evaluation, April 2001, P.G. Young, G.M. Hale 825 1451 12 M.B. Chadwick (LANL), E.Caro, C.R. Lubitz (KAPL) 825 1451 13 ENDF/B-VII modifications by P.R. Page (LANL) described right here 825 1451 14 825 1451 15 825 1451 16 MODIFICATIONS MADE FOR ENDF/B-VII: 825 1451 17 825 1451 18 The (n,alpha0), (n,alpha) and elastic cross-section magnitudes 825 1451 19 (MF=3, MT=2,107,800) were changed in December 2005 by Philip Page 825 1451 20 (LANL) from the ENDF/B-VI MOD 3 Evaluation (discussed above). 825 1451 21 825 1451 22 The change made to the ENDF/B-VI MOD 3 version is that the 825 1451 23 cross-sections of all the 16O(n,alpha0) data in the region of 825 1451 24 laboratory neutron energy 2.4-8.9 MeV have been been reduced by 825 1451 25 32%. The threshold is at 2.4 MeV. The total 16O n cross-section 825 1451 26 is fixed, so that the difference is put into the elastic 16O n 825 1451 27 cross-section (in the region 2.4-8.9 MeV). The 16O(n,alpha) 825 1451 28 cross-section is also changed to reflect the new 16O(n,alpha0) 825 1451 29 cross-section. 825 1451 30 825 1451 31 The logic is as follows: The ENDF/B-VI evaluation of 825 1451 32 16O(n,alpha0) used three evaluations spliced together: one from 825 1451 33 0-3.4 MeV (KAPL), one from 3.4-6.25 MeV (R-matrix, Gerry Hale), 825 1451 34 and one from 6.25-30 MeV. Inspection of the ENDF/B-VI file and 825 1451 35 comments in the file indicate that continuity is preserved at 825 1451 36 the boundary of these three evaluations. Since the Bair and 825 1451 37 Haas data [Ba73] in the 3.2-6.8 MeV neutron energy region 825 1451 38 set the scale of the R-matrix evaluation, it follows from 825 1451 39 continuity that it sets the scale of all three evaluations. 825 1451 40 Assuming that the new data from Harissopulos et al. [Ha05] 825 1451 41 for 3.0-8.9 MeV (neutron energy), which is on average 32% 825 1451 42 lower than the ENDF/B-VI R-matrix evaluation, are definitive, 825 1451 43 this implies the required reduction of 32% in the 3.0-8.9 MeV 825 1451 44 region. 825 1451 45 825 1451 46 Finer details: 825 1451 47 825 1451 48 (1) The 32% reduction estimate includes the averaged reduction 825 1451 49 estimates given by Harissopulos et al. [Ha05], it assumes their 825 1451 50 actual measured cross-section as reported (not the effective one 825 1451 51 they use to display their data), and takes into account the 825 1451 52 renormalization of the Bair and Haas data [Ba73] that was required 825 1451 53 for the ENDF/B-VI R-matrix analysis. 825 1451 54 825 1451 55 (2) Part of my philosophy with this new file is that one takes 825 1451 56 the view that the new data (Harissopulos [Ha05]) is 100% correct 825 1451 57 and the old data (Bair and Haas [Ba73]) is 100% wrong, as far 825 1451 58 as normalization. 825 1451 59 825 1451 60 (3) Since the ENDF/B-VI evaluation a new measurement by Heil 825 1451 61 [He02] was reported (corresponding to a maximum E_n of 825 1451 62 3.09 MeV). The energy range of this measurement falls in the 825 1451 63 0-3.4 MeV of the KAPL evaluation. The absolute normalization of 825 1451 64 the KAPL evaluation is set by the R-matrix evaluation from 825 1451 65 3.4-6.25 MeV. Since the Heil data [He02] follows the Drotleff data 825 1451 66 [Dr93], and the Drotleff data were renormalized 17% upwards in 825 1451 67 the R-matrix analysis, it means that the ENDF/B-VI evaluation 825 1451 68 should be renormalized downwards by 17% in the region of the Heil 825 1451 69 data (near threshold). To maintain continuity and uniformity in 825 1451 70 appearance with higher energies, the ENDF/B-VI evaluation is 825 1451 71 renormalized downwards by 32% not only from 3.0-8.9 MeV 825 1451 72 (as mentioned above), but from 2.4-8.9 MeV. 825 1451 73 825 1451 74 (4) There is a renormalization only over a finite region 2.4-8.9 825 1451 75 MeV. In the region above 8.9 MeV the cross-section is still what 825 1451 76 it used to be before. To retain continuity, I introduced a region 825 1451 77 around 8.9 MeV where the function was interpolated. So the 825 1451 78 cross-section is technically continuous. The problem with 825 1451 79 changing the cross-section from 8.9-30 MeV from the former 825 1451 80 values is that you apparently have no empirical basis for doing 825 1451 81 so, since no new data is available in there regions. 825 1451 82 825 1451 83 [Ba73] J.K. Bair and F.X. Haas, Phys. Rev. C7, 1356 (1973) 825 1451 84 [Dr93] H.W. Drotleff et al., Ap.J. 414, 735 (1993) 825 1451 85 [Ha05] S. Harissopulos et al., Phys. Rev. C72, 062801 (2005) 825 1451 86 [He02] M. Heil, Ph.D. thesis, Forschungszentrum Karlsruhe (2002) 825 1451 87 825 1451 88 ***************************************************************** 825 1451 89 825 1451 90 The ENDF/B-VI evaluation is a combination of a new MOD 3 eval. 825 1451 91 below 30 MeV and the previous MOD 2 evaluation from 20 to 150 MeV. 825 1451 92 Both these evaluations are described below. The only change to the 825 1451 93 data above 30 MeV is to add tritium-production data, based on 825 1451 94 experimental yield data and spectra calculated with the GNASH 825 1451 95 Hauser-Feshbach/preequilibrium code. 825 1451 96 This evaluation provides a complete representation of the 825 1451 97 nuclear data needed for transport, damage, heating, radioactivity, 825 1451 98 and shielding applications over the incident neutron energy range 825 1451 99 from 1.0E-11 to 150 MeV. The discussion here is divided into the 825 1451 100 region above and below 30 MeV. 825 1451 101 825 1451 102 ------------------------------------------------------------------ 825 1451 103 825 1451 104 INCIDENT NEUTRON ENERGIES > 30 MeV 825 1451 105 825 1451 106 The evaluation above 30 MeV utilizes MF=6, MT=5 to represent 825 1451 107 all reaction data. Production cross sections and emission 825 1451 108 spectra are given for neutrons, protons, deuterons, alpha 825 1451 109 particles, gamma rays, and all residual nuclides produced (A>5) 825 1451 110 in the reaction chains. To summarize, the ENDF sections with 825 1451 111 non-zero data above En = 30 MeV are: 825 1451 112 825 1451 113 MF=3 MT= 1 Total Cross Section 825 1451 114 MT= 2 Elastic Scattering Cross Section 825 1451 115 MT= 3 Nonelastic Cross Section 825 1451 116 MT= 5 Sum of Binary (n,n') and (n,x) Reactions 825 1451 117 MT=102 Radiative Capture Cross Section (Estimate Only) 825 1451 118 825 1451 119 MF=4 MT= 2 Elastic Angular Distributions 825 1451 120 825 1451 121 MF=6 MT= 5 Production Cross Sections and Energy-Angle 825 1451 122 Distributions for Emission Neutrons, Protons, 825 1451 123 Deuterons, and Alphas; and Angle-Integrated 825 1451 124 Spectra for Gamma Rays and Residual Nuclei That 825 1451 125 Are Stable Against Particle Emission 825 1451 126 825 1451 127 The evaluation is based on nuclear model calculations that 825 1451 128 have been benchmarked to experimental data, especially for n + 825 1451 129 O16 and p + O16 reactions [Ch96a]. We use the GNASH code system 825 1451 130 [Yo92], which utilizes Hauser-Feshbach statistical, preequi- 825 1451 131 librium and direct-reaction theories. Coupled-channel and 825 1451 132 spherical optical model calculations are used to obtain particle 825 1451 133 transmission coefficients for the Hauser-Feshbach calculations, 825 1451 134 as well as for the elastic neutron angular distributions. 825 1451 135 Cross sections and spectra for producing individual residual 825 1451 136 nuclei are included for reactions that exceed a cross section of 825 1451 137 approximately 1 nb at any energy. The energy-angle-correlations 825 1451 138 for all outgoing particles are based on Kalbach systematics 825 1451 139 [Ka88]. 825 1451 140 A model was developed to calculate the energy distributions of 825 1451 141 all recoil nuclei in the GNASH calculations [Ch96b]. The recoil 825 1451 142 energy distributions are represented in the laboratory system in 825 1451 143 MT=5, MF=6, and are given as isotropic in the lab system. Note 825 1451 144 that all other data in MT=5,MF=6 are given in the center-of-mass 825 1451 145 system. This method of representation requires a modification of 825 1451 146 the original ENDF-6 format. 825 1451 147 Preequilibrium corrections were performed in the course of the 825 1451 148 GNASH calculations using either Feshbach, Kerman, Koonin (FKK) 825 1451 149 theory [Ch93] or the exciton model of Kalbach [Ka77, Ka85]. 825 1451 150 Discrete level data from nuclear data sheets were matched to 825 1451 151 continuum level densities using the formulation of Ignatyuk 825 1451 152 [Ig75] and pairing and shell parameters from the Cook [Co67] 825 1451 153 analysis. Neutron and charged-particle transmission coefficients 825 1451 154 were obtained from the optical potentials, as discussed below. 825 1451 155 Gamma-ray transmission coefficients were calculated using the 825 1451 156 Kopecky-Uhl model [Ko90]. 825 1451 157 825 1451 158 ------------------------------------------------------------------ 825 1451 159 825 1451 160 INCIDENT NEUTRON ENERGIES < 30 MeV 825 1451 161 825 1451 162 The evaluation below 30 MeV includes complete data for all 825 1451 163 significant neutron-induced reactions. It is comprised of 825 1451 164 R-parameter [Ca98] and R-matrix analyses below 6.25 MeV, and a 825 1451 165 combination of experimental and theoretical data evaluation 825 1451 166 from 6.25 to 30 MeV. A summary of the evaluation by energy 825 1451 167 range is given below, followed by a detailed description of 825 1451 168 the evaluation, reaction by reaction. 825 1451 169 825 1451 170 NEUTRON ENERGY < 6.25 MeV 825 1451 171 825 1451 172 The evaluation below 3.4 MeV is an R-function fit [Ca98] to 825 1451 173 experimental data. At 3.4 MeV, it is spliced to the LANL R-matrix 825 1451 174 analysis with a transition region of about 60 keV centered at 825 1451 175 3.4 MeV. The LANL analysis is used for the region from 3.40 to 825 1451 176 6.25 MeV. 825 1451 177 825 1451 178 NEUTRON ENERGY > 6.25 MeV 825 1451 179 825 1451 180 The following major modifications were made above 6.25 MeV: 825 1451 181 1. The maximum energy of the evaluation was increased from 20 to 825 1451 182 30 MeV. 825 1451 183 2. New measurements of 16O(n,xgamma) angular distributions (7 825 1451 184 angles, En = 4 - 200 MeV) by Nelson et al. [Ne99] were incor- 825 1451 185 porated into the evaluation. The measurements use a high- 825 1451 186 resolution Ge detector and result in data for some 21 gamma rays. 825 1451 187 The distributions were fit with Legendre expansions to obtain 825 1451 188 angle-integrated cross sections for MF=13 and angular 825 1451 189 distributions for MF=14. Nuclear energy level schemes and gamma 825 1451 190 branching ratios [Aj86,Aj91] were utilized to extract level 825 1451 191 excitation cross sections in MF=3 for discrete states in 16O, 825 1451 192 14-16N, and 13C, corresponding to (n,n'), (n,p), (n,d), (n,t), 825 1451 193 and (n,alpha) reactions. 825 1451 194 3. New measurements of 16O(n,alpha) cross sections at 14 MeV by 825 1451 195 Sanami and Baba [Sa97] were used to adjust the (n,alpha) cross 825 1451 196 sections. 825 1451 197 4. The neutron total cross section measurements of Finlay [Fi93] 825 1451 198 were incorporated into the evaluation above 7.3 MeV. Adjustments 825 1451 199 of up to 2% were made in the existing evaluation. 825 1451 200 5. The new evaluation contains no pseudo level or excitation 825 1451 201 energy bin data. Calculations were made with the GNASH code to 825 1451 202 provide continuum emission data in MF=6 format, as well as any 825 1451 203 unmeasured data. Calculated cross sections were renormalized 825 1451 204 whenever possible using experimental data. The GNASH calculations 825 1451 205 utilized transmission coefficients calculated with a spherical 825 1451 206 optical potential and level densities from the Gilbert and 825 1451 207 Cameron model, plus preequilibrium corrections using systematic 825 1451 208 values of parameters. 825 1451 209 6. Comparisons of the evaluation with a large body of 825 1451 210 experimental data have been made to validate the new data. 825 1451 211 825 1451 212 ------------------------------------------------------------------ 825 1451 213 825 1451 214 DETAILED DESCRIPTION REACTION BY REACTION 825 1451 215 825 1451 216 MF=2 RESONANCE PARAMETERS ------------------------------------- 825 1451 217 825 1451 218 The evaluation below 3.4 MeV is an R-function fit [Ca98] to 825 1451 219 experimental data using an optical model to provide a background 825 1451 220 R-function. The procedure is coded in the KAPL code "OPTIC", 825 1451 221 with an extension of the original code to convert the optical- 825 1451 222 model phase shifts to background R-functions. 825 1451 223 The analysis is carried to 3.4 MeV, where it is spliced to the 825 1451 224 LANL R-matrix analysis, with a transition region of about 60 keV 825 1451 225 centered at 3.4 MeV. 825 1451 226 From 3.4 to 6.25 MeV, a test evaluation was obtained from a new 825 1451 227 multi-channel R-matrix analysis of a large part of the available 825 1451 228 experimental data base using the EDA code. The analysis of the 825 1451 229 17O system includes data for n+16O neutron total cross sections 825 1451 230 and elastic scattering angular distributions, as well as data 825 1451 231 for the 16O(n,alpha) reaction in both the (n,alpha) and 825 1451 232 (alpha,n) directions. Also included are excitation functions 825 1451 233 for alpha+13C elastic scattering. The total cross sections in 825 1451 234 the final version of this analysis may change, especially in the 825 1451 235 region above 4 MeV. 825 1451 236 825 1451 237 Effective scattering radius = 5.56256E-13 cm. 825 1451 238 825 1451 239 MF=3 NEUTRON CROSS SECTIONS ----------------------------------- 825 1451 240 825 1451 241 THERMAL (2200 m/s) CROSS SECTIONS 825 1451 242 825 1451 243 TOTAL = 3.89440 B RADIATIVE CAPTURE= 0.1900 MB 825 1451 244 ELASTIC= 3.89421 B 825 1451 245 825 1451 246 MT=1 TOTAL CROSS SECTION 825 1451 247 0.0 to 3.40 MeV, calculated from R-function fit to total cross 825 1451 248 section and elastic angular distributions - see above. 825 1451 249 3.4 to 6.25 MeV, calculated from R-Matrix parameters by 825 1451 250 simultaneously fitting most of the available 16O(n,n)16O and 825 1451 251 16O(n,alpha0)13C data, as well as 13C(alpha,alpha)13C data at 825 1451 252 energies below En = 6.2 MeV. The experimental total cross 825 1451 253 section data fitted in the analysis were the [Jo74] results below 825 1451 254 6.26 MeV, and the [La80] measurements at higher energies, with 825 1451 255 inserts of the high-resolution data of [Jo79] over the resonances 825 1451 256 and in the window at En = 2.3-2.4 MeV. 825 1451 257 6.25 to 30 MeV, based on an adjustment of the covariance 825 1451 258 analysis used for the ENDF/B-VI (Rel. 0) evaluation to 825 1451 259 accommodate the new measurements of Finlay et al. [Fi93]. The 825 1451 260 previous ENDF/B-VI (Rel. 0) evaluations is based on analysis 825 1451 261 with the GLUCS Bayes code [He80] of the remaining major total 825 1451 262 cross section measurements [Fo71], [Pe72], [Sc72], [La80], 825 1451 263 [Ci68], [Ci80], with structure inserted from the high-resolution 825 1451 264 [Ci80] measurement. 825 1451 265 825 1451 266 MT=2 ELASTIC SCATTERING CROSS SECTION 825 1451 267 0.0 to 3.40 MeV, calculated from R-function fit to total cross 825 1451 268 section and elastic angular distributions - see above. 825 1451 269 3.4 to 6.25 MeV, R-matrix analysis that includes all available 825 1451 270 experimental data, as described above. Elastic angular 825 1451 271 distribution data used in the analysis includes [La60], [Ok55], 825 1451 272 [Fo58], [Ma62], [Fo70], [Hu62], [Ph61], [Jo67], [Ki72], [Ch61], 825 1451 273 [Dr76], [Fo64]. 825 1451 274 6.25 to 20 MeV, obtained by subtracting the nonelastic cross 825 1451 275 section (MT=3) from the total cross section (MT=1), although 825 1451 276 small adjustments were made to several of the less well 825 1451 277 determined reaction cross sections in order to enhance agreement 825 1451 278 with the elastic measurements of Borker [Bo89], Glendinning 825 1451 279 [Gl82], and Petler [Pe85]. The magnitude of these adjustments 825 1451 280 was generally small and was greatest near structure and near 825 1451 281 18 MeV. 825 1451 282 825 1451 283 MT=4 INELASTIC CROSS SECTION 825 1451 284 Threshold to 30 MeV, sum of MT=51-57, 91. 825 1451 285 825 1451 286 MT=51-57 INELASTIC CROSS SECTION TO DISCRETE STATES 825 1451 287 Threshold to 30 MeV, the (n,n') cross sections corresponding 825 1451 288 to gamma-emitting excited levels of 16O are included in MT=51-57 825 1451 289 as follows: 825 1451 290 MT=51 Ex= 6.0494 MeV 825 1451 291 MT=52 Ex= 6.129893 MeV 825 1451 292 MT=53 Ex= 6.9171 MeV 825 1451 293 MT=54 Ex= 7.11685 MeV 825 1451 294 MT=55 Ex= 8.8719 MeV 825 1451 295 MT=56 Ex=10.957 MeV 825 1451 296 MT=57 Ex=11.080 MeV 825 1451 297 825 1451 298 Note that the 16O levels at 9.585, 9.8445, and 10.356 are 825 1451 299 omitted because they decay primarily by alpha particle emission 825 1451 300 and those data are included in MT=22. 825 1451 301 825 1451 302 MT=16 (N,2N) CROSS SECTION 825 1451 303 Threshold to 30 MeV, based on GNASH calculation, renormalized 825 1451 304 down by approximately 30% to improve agreement with measurement 825 1451 305 of Brill et al. [Br61]. 825 1451 306 825 1451 307 MT=22 (N,NALPHA) CROSS SECTION 825 1451 308 Threshold to 30 MeV, based on GNASH calculation, with 825 1451 309 adjustments made to improve agreement with experimental data, 825 1451 310 especially data of Bormann et al. [Bo63]. 825 1451 311 825 1451 312 MT=23 (N,N3ALPHA) CROSS SECTION 825 1451 313 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 314 from 28 to 30 MeV to agree with LA150 data. 825 1451 315 825 1451 316 MT=28 (N,NP) CROSS SECTION 825 1451 317 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 318 such that the production cross sections for the 5.2701 and 5.2988 825 1451 319 MeV gamma rays are consistent with Nelson et al.[Ne99] data, and 825 1451 320 normalization of proton spectra consistent with 27-MeV data of 825 1451 321 Subramanian et al. [Su94]. 825 1451 322 825 1451 323 MT=32 (N,ND) CROSS SECTION 825 1451 324 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 325 such that difference between total and nonelastic cross sections 825 1451 326 agrees with elastic cross section measurements. 825 1451 327 825 1451 328 MT=41 (N,2NP) CROSS SECTION 825 1451 329 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 330 such that difference between total and nonelastic cross sections 825 1451 331 agrees with elastic cross section measurements. 825 1451 332 825 1451 333 MT=44 (N,N2P) CROSS SECTION 825 1451 334 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 335 such that difference between total and nonelastic cross sections 825 1451 336 agrees with elastic cross section measurements. 825 1451 337 825 1451 338 MT=45 (N,NPALPHA) CROSS SECTION 825 1451 339 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 340 such that difference between total and nonelastic cross sections 825 1451 341 agrees with elastic cross section measurements. 825 1451 342 825 1451 343 MT=91 (N,N'CONTINUUM) CROSS SECTION 825 1451 344 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 345 such that difference between total and nonelastic cross sections 825 1451 346 agrees with elastic cross section measurements. 825 1451 347 825 1451 348 MT=102 (N,GAMMA) CROSS SECTION 825 1451 349 0 to 1 MeV,cross section based on experimental data obtained 825 1451 350 from E. Jurney [Ju64]; higher energy data is crude estimate. 825 1451 351 825 1451 352 MT=103 (N,P) CROSS SECTION 825 1451 353 Sum of MT=600-603. 825 1451 354 825 1451 355 MT=104 (N,D) CROSS SECTION 825 1451 356 Sum of MT=650-669. 825 1451 357 825 1451 358 MT=105 (N,T) CROSS SECTION 825 1451 359 Sum of MT=700-709,749. 825 1451 360 825 1451 361 MT=107 (N,ALPHA) CROSS SECTION 825 1451 362 Sum of MT=800-803. 825 1451 363 825 1451 364 MT=108 (N,2ALPHA) CROSS SECTION 825 1451 365 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 366 such that difference between total and nonelastic cross sections 825 1451 367 agrees with elastic cross section measurements. 825 1451 368 825 1451 369 MT=112 (N,PALPHA) CROSS SECTION 825 1451 370 Threshold to 30 MeV, based on GNASH calculations, adjusted 825 1451 371 such that difference between total and nonelastic cross sections 825 1451 372 agrees with elastic cross section measurements. 825 1451 373 825 1451 374 MT=600 (N,P) INTEGRATED CROSS SECTION TO 16N GROUND STATE 825 1451 375 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 376 renormalization (lowered approximately 30%) from comparison of 825 1451 377 excited state predictions with Nelson et al. [Ne99] 825 1451 378 measurements. 825 1451 379 825 1451 380 MT=601-603 (N,P) CROSS SECTION TO EXCITED LEVELS OF 16N 825 1451 381 Threshold to 30 MeV, the cross sections for the 0.0.297- and 825 1451 382 0.3975-MeV levels are inferred from the (n,p gamma) data of 825 1451 383 Nelson et al. [Ne99], using the level structure diagram of 16N 825 1451 384 by Ajzenberg-Selove [Aj86]. The cross section for the 0.1201- 825 1451 385 MeV level is based on GNASH calculations with some 825 1451 386 renormalization (lowered ~30%) from comparison of excited state 825 1451 387 predictions with Nelson et al. [Ne99] measurements. 825 1451 388 825 1451 389 MT=650 (N,D) INTEGRATED CROSS SECTION TO 15N GROUND STATE 825 1451 390 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 391 renormalization from comparison of excited state predictions 825 1451 392 with Nelson et al. [Ne99] measurements. 825 1451 393 825 1451 394 MT=651-669 (N,D) CROSS SECTION TO EXCITED LEVELS OF 15N 825 1451 395 Threshold to 30 MeV, the cross sections for the 5.2701- and 825 1451 396 5.2988-MeV levels are adjusted based on the (n,xgamma) data of 825 1451 397 Nelson et al. [Ne99], using the level structure diagram for 15N 825 1451 398 by Ajzenberg-Selove [Aj91]. Cross sections for remaining levels 825 1451 399 are based on GNASH calculations with some renormalization from 825 1451 400 comparison of excited state predictions with Nelson et al. 825 1451 401 [Ne99] measurements and 27-Mev data of Subramanian et al. [Su94]. 825 1451 402 825 1451 403 MT=700 (N,T) INTEGRATED CROSS SECTION TO 14N GROUND STATE 825 1451 404 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 405 renormalization from comparison of excited state predictions 825 1451 406 with Nelson et al. [Ne99] measurements. 825 1451 407 825 1451 408 MT=701-709 (N,T) CROSS SECTION TO EXCITED LEVELS OF 14N 825 1451 409 Threshold to 30 MeV, the cross section for the 2.3128-MeV 825 1451 410 levels is inferred from the (n,t gamma) data of Nelson et al. 825 1451 411 [Ne99], using the level structure diagram for 16N by Ajzenberg- 825 1451 412 Selove [Aj91]. Cross sections for the remaining levels are 825 1451 413 based on GNASH calculations with some renormalization from 825 1451 414 comparison of excited state predictions with Nelson et al. 825 1451 415 [Ne99] measurements. 825 1451 416 825 1451 417 MT=749 (N,T) CROSS SECTION TO 14N CONTINUUM 825 1451 418 Threshold to 30 MeV, based on GNASH calculations with some 825 1451 419 renormalization from comparison of excited state predictions 825 1451 420 with Nelson et al. [Ne99] measurements and to enhance agreement 825 1451 421 of elastic cross section with measured data. 825 1451 422 825 1451 423 MT=800 (N,ALPHA0) CROSS SECTION TO 13C GROUND STATE 825 1451 424 0.0 to 6.2 MeV, based on R-matrix analysis described above 825 1451 425 under MT=1. Data of Ba72 were used in the original (alpha,n) 825 1451 426 direction, with no changes in energy scale or normalization. 825 1451 427 Also included were the low-energy (alpha,n) data of [Ke91] and 825 1451 428 [Dr93]. 825 1451 429 6.2 to 20 MeV, based on data of [Da63],[Da68],[Si68],[Ba73], 825 1451 430 and composite of [Mc66b],[Ma68],[Le68] at 14 MeV. Note that the 825 1451 431 [Da63] data were renormalized by factor of 1.5 to bring them 825 1451 432 into rough agreement with the R-matrix analysis of the [Ba73] 825 1451 433 (n,a0) data, together with the total and elastic data in the 825 1451 434 analysis. Because the [Da68] experimental data were normalized 825 1451 435 to [Da63], the former were also renormalized by the factor of 825 1451 436 1.5. 825 1451 437 825 1451 438 MT=801-803 (N,ALPHA) CROSS SECTION TO EXCITED LEVELS OF 13C 825 1451 439 Threshold to 30 MeV, the cross sections of the 3.0894-, 825 1451 440 3.6845-, and 3.8538-MeV levels are inferred from the (n,alpha 825 1451 441 gamma) data of Nelson et al. [Ne99], using the level structure 825 1451 442 diagram of 13C by Ajzenberg-Selove [Aj91]. 825 1451 443 825 1451 444 MF=4 ANGULAR DISTRIBUTIONS ------------------------------------ 825 1451 445 825 1451 446 MT=2 ELASTIC NEUTRON ANGULAR DISTRIBUTIONS 825 1451 447 0.0 to 3.4 MeV, calculated from R-function fit (see MF=3,MT=1). 825 1451 448 3.4 to 6.2 MeV, calculated from R-matrix fit (see MF=3,MT=1). 825 1451 449 Measured angular distributions input to the fit were those of 825 1451 450 [Ch61],[Fo58],[Fo70],[Hi58],[Hu62], [Jo67],[Ki72],[La60],[Li66], 825 1451 451 [Ma62],[Ph61],[Jo79]. Fits were attempted using new data of 825 1451 452 [Sc77], but those measurements were found to have significant 825 1451 453 uncertainties, and some discrepancies with other data were noted. 825 1451 454 6.2 to 20 MeV, smooth curve through coefficients derived from 825 1451 455 fits to elastic data of [Ph61],[Ne72],[Ch61],[Ba63],[Be67], 825 1451 456 [Mc66a],[Ki72],[Bu73],[Ne72],[Gl82],[Ba85],[Bo89],[Pe85]. 825 1451 457 825 1451 458 MT=51-57 DISCRETE (N,N') ANGULAR DISTRIBUTIONS 825 1451 459 Threshold to 10 MeV, assumed isotropic in center of mass. 825 1451 460 Above 10 MeV, based on fits of the 14-MeV data of [Ki72],[Ne72], 825 1451 461 [Ba63],[Mc66a],[Ba85],[Me69], and especially [Bo89]. 825 1451 462 825 1451 463 MT=600-603 DISCRETE (N,P) ANGULAR DISTRIBUTIONS 825 1451 464 Threshold to 30 MeV, assumed isotropic in center of mass. 825 1451 465 825 1451 466 MT=650-669 DISCRETE (N,D) ANGULAR DISTRIBUTIONS 825 1451 467 Threshold to 30 MeV, assumed isotropic in center of mass. 825 1451 468 825 1451 469 MT=700-709 DISCRETE (N,T) ANGULAR DISTRIBUTIONS 825 1451 470 Threshold to 30 MeV, assumed isotropic in center of mass. 825 1451 471 825 1451 472 MT=800 DISCRETE(N,ALPHA0) ANGULAR DISTRIBUTIONS 825 1451 473 0.0 to 6.2 MeV, calculated from R-Matrix fit (see MF=3,MT=1). 825 1451 474 Measured angular distributions input to the fit were 825 1451 475 reconstructed from the Legendre coefficients of [Wa57], and 825 1451 476 converted to (n,alpha) angular distributions using detailed 825 1451 477 balance. 825 1451 478 825 1451 479 MT=801-803 DISCRETE (N,T) ANGULAR DISTRIBUTIONS 825 1451 480 Threshold to 6 MeV, 825 1451 481 6 to 30 MeV, assumed isotropic in center of mass. 825 1451 482 825 1451 483 MF=6 PRODUCT ENERGY-ANGLE DISTRIBUTIONS ----------------------- 825 1451 484 825 1451 485 MT=16 (N,2N) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 486 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 487 are given for neutrons, and isotropic energy spectra are given 825 1451 488 for recoiling 15O nuclei. The neutron data were obtained from 825 1451 489 the GNASH calculations; the recoil 15O distributions were 825 1451 490 calculated with the RECOIL code [Ma83]. The discrete gamma rays 825 1451 491 from (n,2ngamma) reactions are given in MF=13 and 14. 825 1451 492 825 1451 493 MT=22 (N,NALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 494 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 495 are given for neutrons and alpha particles, and isotropic energy 825 1451 496 spectra are given for recoiling 12C nuclei. The neutron and 825 1451 497 alpha data were obtained from the GNASH calculations; the recoil 825 1451 498 12C distributions were calculated with the RECOIL code [Ma83]. 825 1451 499 The discrete gamma rays from (n,nalpha gamma) reactions are 825 1451 500 given in MF=13 and 14. 825 1451 501 825 1451 502 MT=28 (N,NP) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 503 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 504 are given for neutrons and protons; isotropic energy spectra are 825 1451 505 given for recoiling 15N nuclei; and isotropic energy spectra are 825 1451 506 given for emitted continuum gamma rays. The neutron, proton, 825 1451 507 and gamma-ray data were obtained from the GNASH calculations; 825 1451 508 the recoil 15N distributions were calculated with the RECOIL 825 1451 509 code [Ma83]. 825 1451 510 825 1451 511 MT=32 (N,ND) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 512 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 513 are given for neutrons and deuterons; isotropic energy spectra 825 1451 514 are given for recoiling 14N nuclei; and isotropic energy spectra 825 1451 515 are given for emitted continuum gamma rays. The neutron, 825 1451 516 deuteron, and gamma-ray data were obtained from the GNASH 825 1451 517 calculations; the recoil 14N distributions were calculated with 825 1451 518 the RECOIL code [Ma83]. 825 1451 519 825 1451 520 MT=41 (N,2NP) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 521 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 522 are given for neutrons and protons; isotropic energy spectra are 825 1451 523 given for recoiling 14N nuclei; and isotropic energy spectra are 825 1451 524 given for emitted continuum gamma rays. The neutron, proton, 825 1451 525 and gamma-ray data were obtained from the GNASH calculations; 825 1451 526 the recoil 14N distributions were calculated with the RECOIL 825 1451 527 code [Ma83]. 825 1451 528 825 1451 529 MT=44 (N,N2P) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 530 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 531 are given for neutrons and protons; isotropic energy spectra are 825 1451 532 given for recoiling 14C nuclei; and isotropic energy spectra are 825 1451 533 given for emitted continuum gamma rays. The neutron, proton, 825 1451 534 and gamma-ray data were obtained from the GNASH calculations; 825 1451 535 the recoil 14C distributions were calculated with the RECOIL 825 1451 536 code [Ma83]. 825 1451 537 825 1451 538 MT=45 (N,NPALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 539 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 540 are given for neutrons, protons, and alphas; isotropic energy 825 1451 541 spectra are given for recoiling 11B nuclei; and isotropic energy 825 1451 542 spectra are given for emitted continuum gamma rays. The 825 1451 543 neutron, proton, alpha, and gamma-ray data were obtained from 825 1451 544 the GNASH calculations; the recoil 11B distributions were 825 1451 545 calculated with the RECOIL code [Ma83]. 825 1451 546 825 1451 547 MT=91 (N,N'CONTINUUM) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 548 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 549 are given for neutrons; isotropic energy spectra are given for 825 1451 550 recoiling 16O nuclei; and isotropic energy spectra are given for 825 1451 551 emitted continuum gamma rays. The neutron and gamma-ray data 825 1451 552 were obtained from the GNASH calculations; the recoil 16O 825 1451 553 distributions were calculated with the RECOIL code [Ma83]. 825 1451 554 825 1451 555 MT=108 (N,2ALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 556 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 557 are given for alphas; isotropic energy spectra are given for 825 1451 558 recoiling 9Be nuclei; and isotropic energy spectra are given for 825 1451 559 emitted continuum gamma rays. The alpha, and gamma-ray data 825 1451 560 were obtained from the GNASH calculations; the recoil 9Be 825 1451 561 distributions were calculated with the RECOIL code [Ma83]. 825 1451 562 825 1451 563 MT=112 (N,PALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 564 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 565 are given for protons, and alphas; isotropic energy spectra are 825 1451 566 given for recoiling 12B nuclei; and isotropic energy spectra are 825 1451 567 given for emitted continuum gamma rays. The proton, alpha, and 825 1451 568 gamma-ray data were obtained from the GNASH calculations; the 825 1451 569 recoil 12B distributions were calculated with the RECOIL code 825 1451 570 [Ma83]. 825 1451 571 825 1451 572 MT=749 (N,ALPHA) CONTINUUM ENERGY-ANGLE EMISSION DATA 825 1451 573 Threshold to 30 MeV, energy-angle correlated energy spectra 825 1451 574 are given for alpha particles; isotropic energy spectra are 825 1451 575 given for recoiling 13C nuclei; and isotropic energy spectra are 825 1451 576 given for emitted continuum gamma rays. The alpha and gamma-ray 825 1451 577 data were obtained from the GNASH calculations; the recoil 13C 825 1451 578 distributions were calculated with the RECOIL code [Ma83]. 825 1451 579 825 1451 580 MF=12 PHOTON PRODUCTION MULTIPLICITIES ------------------------ 825 1451 581 825 1451 582 MT=102 (N,GAMMA) PHOTON PRODUCTION MULTIPLICITIES 825 1451 583 Photon multiplicities for radiative capture are based on 825 1451 584 experimental data obtained from Jurney [Ju64]. 825 1451 585 825 1451 586 MF=13 PHOTON PRODUCTION CROSS SECTIONS ------------------------ 825 1451 587 825 1451 588 MT=4 (N,N'GAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 589 Threshold to 30 MeV: Based almost entirely on new angular 825 1451 590 distribution measurements by Nelson et al. [Ne99], which 825 1451 591 utilized a white neutron source and covered the energy range 825 1451 592 from threshold to 200 MeV. The measurements were made at 7 825 1451 593 angles using high-resolution Ge detectors and resulted in data 825 1451 594 for some 23 gamma rays from 7 different reactions. The angular 825 1451 595 distributions were fit with Legendre expansions to obtain angle- 825 1451 596 integrated cross sections. The fitted cross sections were 825 1451 597 smoothed somewhat for this evaluation, although much of the 825 1451 598 measured structure was preserved, particularly for the intense 825 1451 599 6.129-MeV gamma. The evaluated data for the following gamma 825 1451 600 rays are based directly on the measurements: 825 1451 601 825 1451 602 EG= 2.742 MeV (decay of 8.8719-MeV level of 16O) 825 1451 603 EG= 3.839 MeV (decay of 10.957-MeV level of 16O) 825 1451 604 EG= 4.950 MeV (decay of 11.080-MeV level of 16O) 825 1451 605 EG= 6.130 MeV (decay of 6.130-MeV level of 16O) 825 1451 606 EG= 6.917 MeV (decay of 6.917-MeV level of 16O) 825 1451 607 EG= 7.117 MeV (decay of 7.117-MeV level of 16O) 825 1451 608 825 1451 609 The evaluated cross sections for the remaining (n,n') gamma 825 1451 610 rays are inferred from these data using the energy level scheme 825 1451 611 of Ajzenberg-Selove [Aj86]. Data were also obtained for gamma 825 1451 612 rays of energy 1.755 and 1.955 from decay of the 8.8719-MeV 825 1451 613 level but the 2.742-MeV gamma was used to determine the level 825 1451 614 excitation cross section because it is the most intense. 825 1451 615 Similarly, data were obtained on a 4.179-MeV gamma from decay of 825 1451 616 the 11.080-MeV level, but the 4.950-MeV gamma is more intense 825 1451 617 and was used to determine the level excitation cross section. 825 1451 618 The evaluated data were compared to older gamma-ray 825 1451 619 measurements by [Be70], [Ne90], [No78], [Ha59], [Di70], [Or70], 825 1451 620 [Dr70], [Cl69], [Lu70], [Bu71], [Ny69]. Considering that very 825 1451 621 few (e.g., [Be70], [Dr70]) of these measurements are of full 825 1451 622 angular distributions, the agreement is reasonable. 825 1451 623 825 1451 624 MT=16 (N,2NGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 625 Threshold to 30 MeV: The cross section for the 5.2409-MeV 825 1451 626 gamma ray was obtained directly from the Nelson et al. [Ne99] 825 1451 627 data. The remaining discrete gammas are based on GNASH 825 1451 628 calculations, with some renomalization based on the experimental 825 1451 629 data. 825 1451 630 825 1451 631 MT=22 (N,NALPHA GAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 632 Threshold to 30 MeV: Only the 4.438-MeV discrete gamma ray 825 1451 633 is given and it is based on the Nelson et al. [Ne99] data. 825 1451 634 825 1451 635 MT=103 (N,PGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 636 Threshold to 30 MeV: The cross sections for the 0.2774- and 825 1451 637 0.297-MeV gamma rays are based on the Nelson et al. [Ne99] data. 825 1451 638 The 0.3975-MeV gamma is inferred from the 0.2774-MeV gamma data 825 1451 639 through the Ajzenberg-Selove level scheme [Aj86] for 16N. The 825 1451 640 0.1201-MeV gamma cross section is based partially on GNASH 825 1451 641 calculations and partially inferred from the [Ne99] data using 825 1451 642 the 16N level scheme. 825 1451 643 825 1451 644 MT=104 (N,DGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 645 Threshold to 30 MeV: The cross sections for the 5.2701- and 825 1451 646 5.2988-MeV gamma rays are based on the Nelson et al. [Ne99] 825 1451 647 data. The cross sections for the remaining 60 (n,dg) gamma rays 825 1451 648 are based on GNASH calculations and the Ajzenberg-Selove level 825 1451 649 scheme [Aj91] for 15N, after renomalization to agree with the 825 1451 650 measured 5.2701- and 5.2988-MeV gamma-ray data. 825 1451 651 825 1451 652 MT=105 (N,TGAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 653 Threshold to 30 MeV: The cross section for the 2.313-MeV 825 1451 654 gamma ray is based on the Nelson et al. [Ne99] measurement. The 825 1451 655 cross sections for the remaining 20 (n,tg) gamma rays are based 825 1451 656 on GNASH calculations and the Ajzenberg-Selove level scheme 825 1451 657 [Aj91] for 14N, after renomalization to agree with the measured 825 1451 658 2.313-MeV gamma-ray data. 825 1451 659 825 1451 660 MT=107 (N,ALPHA GAMMA) PHOTON PRODUCTION CROSS SECTIONS 825 1451 661 Threshold to 30 MeV: The cross sections for the 3.0894-, 825 1451 662 3.6845- and 3.8538-MeV gamma rays are based on the Nelson et 825 1451 663 al. [Ne99] data. The 0.1693-, 0.5951- and 0.7644-MeV gamma-ray 825 1451 664 cross sections are inferred from the above data through the 825 1451 665 Ajzenberg-Selove level scheme [Aj91]. Note that the 0.1693-MeV 825 1451 666 gamma from decay of the 3.8538-MeV level also was measured, but 825 1451 667 the 3.8538-MeV gamma is more intense and was used to determine 825 1451 668 the level excitation cross section. 825 1451 669 825 1451 670 MF=14 PHOTON ANGULAR DISTRIBUTIONS ---------------------------- 825 1451 671 825 1451 672 MT=4 (N,N'GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 673 Anisotropic angular distributions in Legendre polynomial 825 1451 674 representation are given for the 1.755-, 2.742-, 6.130-, 6.917-, 825 1451 675 and 7.117-MeV gamma rays, obtained by fitting the measurements 825 1451 676 of Nelson et al. [Ne99]. Isotropic angular distributions are 825 1451 677 assumed for the remaining gamma rays. 825 1451 678 825 1451 679 MT=16 (N,2NGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 680 An anisotropic angular distribution in Legendre polynomial 825 1451 681 representation is given for the 5.2409-MeV gamma ray, obtained 825 1451 682 by fitting the measurements of Nelson et al. [Ne99]. Isotropic 825 1451 683 angular distributions are assumed for the remaining gamma rays. 825 1451 684 825 1451 685 MT=22 (N,NALPHA GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 686 An anisotropic angular distribution in Legendre polynomial 825 1451 687 representation is given for the 4.438-MeV gamma ray, obtained by 825 1451 688 fitting the measurements of Nelson et al. [Ne99]. 825 1451 689 825 1451 690 MT=102 (N,GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 691 All gamma rays from radiative capture are assumed to be 825 1451 692 isotropic. 825 1451 693 825 1451 694 MT=103 (N,PGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 695 Anisotropic angular distributions in Legendre polynomial 825 1451 696 representation are given for the 0.2774-, 0.297-, and 0.3975-MeV 825 1451 697 gamma rays, obtained by fitting the measurements of Nelson et 825 1451 698 al. [Ne99]. The angular distributions for all remaining gamma 825 1451 699 rays are assumed to be isotropic. 825 1451 700 825 1451 701 MT=104 (N,DGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 702 An anisotropic angular distribution in Legendre polynomial 825 1451 703 representation is given for the 5.2701-MeV gamma ray, obtained 825 1451 704 by fitting the measurements of Nelson et al. [Ne99]. The 825 1451 705 angular distributions for all remaining gamma rays are assumed 825 1451 706 to be isotropic. 825 1451 707 825 1451 708 MT=105 (N,TGAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 709 All gamma rays from (n,tg) reactions are assumed to be 825 1451 710 isotropic. 825 1451 711 825 1451 712 MT=107 (N,ALPHA GAMMA) PHOTON ANGULAR DISTRIBUTIONS 825 1451 713 Anisotropic angular distributions in Legendre polynomial 825 1451 714 representation are given for the 0.1693-, 3.6845- and 3.8538- 825 1451 715 MeV gamma rays, obtained by fitting the measurements of Nelson 825 1451 716 et al. [Ne99]. Isotropic angular distributions are assumed for 825 1451 717 all the remaining gamma rays. 825 1451 718 825 1451 719 **************************************************************** 825 1451 720 825 1451 721 SUMMARY OF DATA VALIDATION OF THIS FILE AGAINST INTEGRAL 825 1451 722 BENCHMARKS 825 1451 723 825 1451 724 KAPL (Weinman, Caro, Lubitz) performed a number of data 825 1451 725 validation benchmark calculations to test the performance of this 825 1451 726 file (June-August 2001). This O16 evaluation gives consistently 825 1451 727 good results for the 21 CSWEG solution critical calculations, the 825 1451 728 liquid-oxygen broomstick neutron-transmission experiment, and the 825 1451 729 neutron age in water experiment (see below for more details). 825 1451 730 825 1451 731 A) 21 CSWEG solution critical calculations. Weinman calculated a 825 1451 732 set of 21 ORNL and Rocky Flats benchmark solution criticals used 825 1451 733 for CSEWG analyses. These calculations were run with ENDF/B-VI 825 1451 734 release 5 U235 (Leal,Larson,wright,Derrien) and hydrogen (332.0 825 1451 735 mbarns 2200m/s). Four different oxygen 16 cross section 825 1451 736 evaluations were considered. 825 1451 737 825 1451 738 1. KAPL-Caro 825 1451 739 2. This evaluation (which contains the KAPL data below 3.4 MeV) 825 1451 740 3. ENDF/B-VI MOD 2 825 1451 741 4. JENDL 3.2 825 1451 742 825 1451 743 All four O16 cross section evaluations gave good reactivity 825 1451 744 responses versus our fitting parameter above-thermal-leakage ATL. 825 1451 745 The ATL parameter is a sensitive trending variable to high energy 825 1451 746 scattering cross sections. All four O16 evaluations produced 825 1451 747 eigenvalues whose mean values were all close to unity and only 825 1451 748 the older ENDF/B-VI.2 cross section evaluation gave a slight 825 1451 749 reactivity trend (about .0020 Delta Keff over the range). The 825 1451 750 average eigenvalues and slopes are listed below. 825 1451 751 825 1451 752 Library Av. Keff Slope 825 1451 753 825 1451 754 KAPL-Caro 0.9993 +.0001 825 1451 755 This file 0.9996 +.0004 825 1451 756 ENDF/B-VI.2 1.0003 +.0032 825 1451 757 JENDL 3.2 1.0004 -.0002 825 1451 758 825 1451 759 Thus the reactivity trend, labeled "slope" in the table above, is 825 1451 760 much smaller in the new file compared to the previous ENDF/B-VI.2 825 1451 761 evaluation. 825 1451 762 825 1451 763 B) The liquid-oxygen broomstick experiment. The oxygen window at 825 1451 764 2.3 MeV is the most important feature at which energy the 825 1451 765 greatest transmission takes place. The new evaluation produces 825 1451 766 close to exact agreement with the experiment in the energy range 825 1451 767 of the oxygen window. The previous ENDF/B-VI value is slightly 825 1451 768 below the experimental value. At energies higher than 5.5 MeV, 825 1451 769 the new evaluation produces slightly better results than does the 825 1451 770 previous ENDF/B-VI results. 825 1451 771 825 1451 772 C) Neutron age in water. KAPL obtained 26.4 to be compared 825 1451 773 against an experimental value of 26.6 +/- 0.6. The previous 825 1451 774 ENDF/B-VI file gave a result of 26.3. 825 1451 775 825 1451 776 Additionally, A.C. (Skip) Kahler at Bettis lab undertook 825 1451 777 benchmark testing of this file (memo, May 16, 2001) against 825 1451 778 thermal benchmarks documented in the Int. Handbook of Evaluated 825 1451 779 Criticality Safety Benchmark Experiments, as well as the L5 and 825 1451 780 L6 ORNL benchmarks. From a thermal reactor benchmark perspective, 825 1451 781 there is little to distinguish the performance of the present 825 1451 782 file compared to the previous ENDF file and JENDL-3.2. 825 1451 783 825 1451 784 ***************************************************************** 825 1451 785 825 1451 786 REFERENCES 825 1451 787 825 1451 788 [Aj86] F. Ajzenberg-Selove, Nucl.Phys. A460, 1 (1986) 825 1451 789 [Aj91] F. Ajzenberg-Selove, Nucl.Phys. A523, 1 (1991) 825 1451 790 [Ba63] R.W. Bauer et al., Nucl.Phys. 47, 241 (1963) 825 1451 791 [Ba73] J.K. Bair and F.X. Haas, Phys.Rev.C 7, 1356 (1973) 825 1451 792 (n,a0) cross sect. obtained by detailed balance from this ref. 825 1451 793 [Ba85] M. Baba et al., Nuclear Data for Basic and Applied Sci., 825 1451 794 Proc. Conf., Santa Fe, NM, May 1985, Vol.1 (Gordon and Breach, 825 1451 795 1986) p.223 825 1451 796 [Be67] P.L. Beach et al., Phys.Rev. 156, 1201 (1967) 825 1451 797 [Be70] P. Bertin, report CEA-R-4047 (1970) 825 1451 798 [Bo63] M. 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Kalbach, Los Alamos National Laboratory report 825 1451 853 LA-10248-MS (1985) 825 1451 854 [Ka88] C. Kalbach, Phys.Rev.C 37, 2350 (1988); see also 825 1451 855 C. Kalbach and F. M. Mann, Phys.Rev.C 23, 112 (1981) 825 1451 856 [Ke93] S.Kellogg, reported by C.R.Brune et al., Phys. Rev. C 48, 825 1451 857 3119 (1993). Data renormalized substantially. 825 1451 858 [Ki72] W.E. Kinney and F.G. Perey, report ORNL-4780 (1972) 825 1451 859 [Ko90] J. Kopecky and M. Uhl, Phys.Rev.C 41, 1941 (1990) 825 1451 860 [La60] R.O. Lane et.al., Argonne report ANL-6172 (1960) 825 1451 861 [La80] D. Larson et al., Symp. on Neutron Cross Sections from 10 825 1451 862 to 50 MeV, BNL, May 1980, report BNL-NCS-51243, Vol. 1 (1980) 825 1451 863 p.277 and private communication (1989) 825 1451 864 [Le68] B. Leroux et al., Nucl.Phys. A116, 196 (1968) 825 1451 865 [Li66] D. Lister and A. Sayres, Phys.Rev. 143, 745 (1966) 825 1451 866 [Lu70] B. Lundberg et al., Phys.Scripta 2, 273 (1970) 825 1451 867 [Ma62] J.P. Martin and M.S. Zucker, B.Am.Phys.Soc. 7, 72 (1962) 825 1451 868 [Ma68] D.R. Maxson and R.D. Murphy, Nucl.Phys. A110, 555 (1968) 825 1451 869 [Mc66a] W.J. McDonald et al., Nucl.Phys. 75, 353 (1966) 825 1451 870 [Mc66b] W.N. McDicken and W. Jack, Nucl.Phys. 88, 457 (1966) 825 1451 871 [Ne72] D.O. Nellis and P.S. Buchanan, report DNA-2716 (1972) 825 1451 872 [Ne90] R. Nelson et al., LANL, private communication, 1990 825 1451 873 [Ne99] R.O. Nelson and A. Michaudon, Los Alamos report LA-UR-99- 825 1451 874 4170 (1999). 825 1451 875 [No78] C. Nordborg et al., Nucl.Sci.Eng. 66, 75 (1978) 825 1451 876 [Ok55] A. Okazaki, Phys.Rev. 99, 55 (1955) 825 1451 877 [Ol90] N. Olsson et al., Nucl.Phys.A 509, 161 (1990) 825 1451 878 [Or70] V.J. Orphan et al., Nucl.Sci.Eng. 42, 352 (1970) 825 1451 879 [Pe72] F.G. Perey et al., report ORNL-4823 [ENDF-178] (1972) 825 1451 880 [Pe85] J.S. Petler et al., Phys.Rev.C 32, 673 (1985) 825 1451 881 [Ph61] D.D. Phillips, private communication to BNL (1961) 825 1451 882 [Sa97] T. Sanami and M. Baba, Trieste Conf.(1997)p.616 825 1451 883 [Sc72] R.A. Schrack, Bull.Am.Phy.Soc. 17, 555 [HE1] (1972) 825 1451 884 [Sc77] I. Schouky et al., report KFK-2503 825 1451 885 [Si68] I. Sick et al., Helv.Phys.Acta 41, 573 (1968) 825 1451 886 [Su94] T.S. Subramanian et al., Phys. Rev. C 34, 1580 (1986), and 825 1451 887 private communication to Chadwick (1994). 825 1451 888 [Wa57] R.B.Walton et al., Phys. Rev. 107, 1065 (1957) 825 1451 889 [Yo01] P.G. Young, G.M. Hale, and M.B. Chadwick, LANL report to 825 1451 890 be issued (2001). 825 1451 891 [Yo92] P.G. Young, E.D. Arthur, and M.B. Chadwick, Los Alamos 825 1451 892 report LA-12343-MS (1992) 825 1451 893 825 1451 894 825 1451 895 ************************ C O N T E N T S *********************** 825 1451 896 ***************** Program LINEAR (VERSION 2007-1) *************** 825 1451 897 For All Data Greater than 1.0000E-10 barns in Absolute Value 825 1451 898 Data Linearized Using Energy Dependent Uncertainty 825 1451 899 Energy Accuracy 825 1451 900 (eV) (per-cent) 825 1451 901 ----------- ----------- 825 1451 902 0.0 .010000000 825 1451 903 1.00000000 .010000000 825 1451 904 10.0000000 .100000000 825 1451 905 2.00000E+9 .100000000 825 1451 906 ***************** Program SIGMA1 (VERSION 2007-1) *************** 825 1451 907 Data Doppler Broadened to 1200.00000 Kelvin 825 1451 908 for All Data Greater than 1.0000E-10 barns in Absolute Value 825 1451 909 Data Linearized Using Energy Dependent Uncertainty 825 1451 910 Energy Accuracy 825 1451 911 (eV) (per-cent) 825 1451 912 ----------- ----------- 825 1451 913 0.0 .010000000 825 1451 914 1.00000000 .010000000 825 1451 915 10.0000000 .100000000 825 1451 916 2.00000E+9 .100000000 825 1451 917 ***************** Program SIGMA1 (VERSION 2007-1) *************** 825 1451 918 Data Doppler Broadened to 12000.0000 Kelvin 825 1451 919 for All Data Greater than 1.0000E-10 barns in Absolute Value 825 1451 920 Data Linearized Using Energy Dependent Uncertainty 825 1451 921 Energy Accuracy 825 1451 922 (eV) (per-cent) 825 1451 923 ----------- ----------- 825 1451 924 0.0 .010000000 825 1451 925 1.00000000 .010000000 825 1451 926 10.0000000 .100000000 825 1451 927 2.00000E+9 .100000000 825 1451 928 ***************** Program FIXUP (Version 2007-1) **************** 825 1451 929 Corrected ZA/AWR in All Sections-----------------------------Yes 825 1451 930 Corrected Thresholds-----------------------------------------No 825 1451 931 Extended Cross Sections to 20 MeV----------------------------No 825 1451 932 Allow Cross Section Deletion---------------------------------Yes 825 1451 933 Allow Cross Section Reconstruction---------------------------Yes 825 1451 934 Make All Cross Sections Non-Negative-------------------------Yes 825 1451 935 Delete Energies Not in Ascending Order-----------------------Yes 825 1451 936 Deleted Duplicate Points-------------------------------------Yes 825 1451 937 Check for Ascending MAT/MF/MT Order--------------------------Yes 825 1451 938 Check for Legal MF/MT Numbers--------------------------------Yes 825 1451 939 Allow Creation of Missing Sections---------------------------No 825 1451 940 Allow Insertion of Energy Points-----------------------------No 825 1451 941 Create Uniform Energy Grid-----------------------------------No 825 1451 942 Delete Section if Cross Section =0 at All Energies-----------Yes 825 1451 943 **************** Program DICTIN (VERSION 2007-1) **************** 825 1451 944 1 451 1087 3 825 1451 945 2 151 4 3 825 1451 946 3 1 889 3 825 1451 947 3 2 507 3 825 1451 948 3 4 97 3 825 1451 949 3 5 9 3 825 1451 950 3 16 14 3 825 1451 951 3 22 23 3 825 1451 952 3 23 22 3 825 1451 953 3 28 25 3 825 1451 954 3 32 12 3 825 1451 955 3 41 11 3 825 1451 956 3 44 10 3 825 1451 957 3 45 11 3 825 1451 958 3 51 41 3 825 1451 959 3 52 72 3 825 1451 960 3 53 69 3 825 1451 961 3 54 73 3 825 1451 962 3 55 59 3 825 1451 963 3 56 24 3 825 1451 964 3 57 23 3 825 1451 965 3 91 26 3 825 1451 966 3 102 198 3 825 1451 967 3 103 60 3 825 1451 968 3 104 51 3 825 1451 969 3 105 37 3 825 1451 970 3 107 362 3 825 1451 971 3 108 26 3 825 1451 972 3 112 17 3 825 1451 973 3 600 41 3 825 1451 974 3 601 32 3 825 1451 975 3 602 47 3 825 1451 976 3 603 49 3 825 1451 977 3 650 24 3 825 1451 978 3 651 21 3 825 1451 979 3 652 19 3 825 1451 980 3 653 16 3 825 1451 981 3 654 19 3 825 1451 982 3 655 16 3 825 1451 983 3 656 18 3 825 1451 984 3 657 12 3 825 1451 985 3 658 16 3 825 1451 986 3 659 12 3 825 1451 987 3 660 15 3 825 1451 988 3 661 16 3 825 1451 989 3 662 14 3 825 1451 990 3 663 16 3 825 1451 991 3 664 14 3 825 1451 992 3 665 12 3 825 1451 993 3 666 12 3 825 1451 994 3 667 13 3 825 1451 995 3 668 15 3 825 1451 996 3 669 13 3 825 1451 997 3 700 24 3 825 1451 998 3 701 24 3 825 1451 999 3 702 16 3 825 1451 1000 3 703 13 3 825 1451 1001 3 704 16 3 825 1451 1002 3 705 13 3 825 1451 1003 3 706 15 3 825 1451 1004 3 707 14 3 825 1451 1005 3 708 11 3 825 1451 1006 3 709 14 3 825 1451 1007 3 749 6 3 825 1451 1008 3 800 304 3 825 1451 1009 3 801 90 3 825 1451 1010 3 802 79 3 825 1451 1011 3 803 94 3 825 1451 1012 4 2 3867 3 825 1451 1013 4 51 84 3 825 1451 1014 4 52 84 3 825 1451 1015 4 53 66 3 825 1451 1016 4 54 64 3 825 1451 1017 4 55 50 3 825 1451 1018 4 56 2 3 825 1451 1019 4 57 2 3 825 1451 1020 4 600 2 3 825 1451 1021 4 601 2 3 825 1451 1022 4 602 2 3 825 1451 1023 4 603 2 3 825 1451 1024 4 650 2 3 825 1451 1025 4 651 2 3 825 1451 1026 4 652 2 3 825 1451 1027 4 653 2 3 825 1451 1028 4 654 2 3 825 1451 1029 4 655 2 3 825 1451 1030 4 656 2 3 825 1451 1031 4 657 2 3 825 1451 1032 4 658 2 3 825 1451 1033 4 659 2 3 825 1451 1034 4 660 2 3 825 1451 1035 4 661 2 3 825 1451 1036 4 662 2 3 825 1451 1037 4 663 2 3 825 1451 1038 4 664 2 3 825 1451 1039 4 665 2 3 825 1451 1040 4 666 2 3 825 1451 1041 4 667 2 3 825 1451 1042 4 668 2 3 825 1451 1043 4 669 2 3 825 1451 1044 4 700 2 3 825 1451 1045 4 701 2 3 825 1451 1046 4 702 2 3 825 1451 1047 4 703 2 3 825 1451 1048 4 704 2 3 825 1451 1049 4 705 2 3 825 1451 1050 4 706 2 3 825 1451 1051 4 707 2 3 825 1451 1052 4 708 2 3 825 1451 1053 4 709 2 3 825 1451 1054 4 800 2188 3 825 1451 1055 4 801 2 3 825 1451 1056 4 802 2 3 825 1451 1057 4 803 2 3 825 1451 1058 6 5 4784 3 825 1451 1059 6 16 522 3 825 1451 1060 6 22 2279 3 825 1451 1061 6 23 915 3 825 1451 1062 6 28 1451 3 825 1451 1063 6 32 476 3 825 1451 1064 6 41 258 3 825 1451 1065 6 44 246 3 825 1451 1066 6 45 275 3 825 1451 1067 6 91 2341 3 825 1451 1068 6 108 798 3 825 1451 1069 6 112 454 3 825 1451 1070 6 749 320 3 825 1451 1071 12 102 16 3 825 1451 1072 13 4 1251 3 825 1451 1073 13 16 134 3 825 1451 1074 13 22 51 3 825 1451 1075 13 103 286 3 825 1451 1076 13 104 1540 3 825 1451 1077 13 105 472 3 825 1451 1078 13 107 1161 3 825 1451 1079 14 4 933 3 825 1451 1080 14 16 17 3 825 1451 1081 14 22 187 3 825 1451 1082 14 102 1 3 825 1451 1083 14 103 554 3 825 1451 1084 14 104 242 3 825 1451 1085 14 105 1 3 825 1451 1086 14 107 400 3 825 1451 1087 825 1 0 1088 825 0 0 1089 8016.00000 15.8575100 0 0 1 0 825 2151 1090 8016.00000 1.00000000 0 0 1 0 825 2151 1091 1.00000E-5 20000000.0 0 0 0 0 825 2151 1092 0.0 .556256300 0 0 0 0 825 2151 1093 825 2 0 1094 825 0 0 1095 8016.00000 15.8575100 0 0 0 0 825 3 1 1096 0.0 0.0 0 0 1 2656 825 3 1 1097 2656 2 825 3 1 1098 1.00000E-5 351.019584 1.02999E-5 345.872082 1.06087E-5 340.801663 825 3 1 1099 1.09269E-5 335.803270 1.12544E-5 330.881242 1.15920E-5 326.028596 825 3 1 1100 1.19395E-5 321.249658 1.22976E-5 316.538300 1.26662E-5 311.898507 825 3 1 1101 1.30462E-5 307.323728 1.34372E-5 302.819622 1.38403E-5 298.378221 825 3 1 1102 1.42552E-5 294.005081 1.46827E-5 289.693518 1.51229E-5 285.447189 825 3 1 1103 1.55765E-5 281.260526 1.60434E-5 277.138474 1.65246E-5 273.073999 825 3 1 1104 1.70199E-5 269.071684 1.75304E-5 265.125896 1.80559E-5 261.239776 825 3 1 1105 1.85975E-5 257.408656 1.91550E-5 253.635915 1.97295E-5 249.916485 825 3 1 1106 2.03209E-5 246.253462 2.09305E-5 242.641905 2.15579E-5 239.085974 825 3 1 1107 2.22045E-5 235.579740 2.28701E-5 232.127193 2.35561E-5 228.722949 825 3 1 1108 2.42622E-5 225.371044 2.49899E-5 222.066149 2.57390E-5 218.811630 825 3 1 1109 2.65110E-5 215.603070 2.73057E-5 212.443225 2.81247E-5 209.328146 825 3 1 1110 2.89678E-5 206.260270 2.98367E-5 203.235693 3.07311E-5 200.257368 825 3 1 1111 3.16528E-5 197.321015 3.26017E-5 194.429278 3.35795E-5 191.578412 825 3 1 1112 3.45861E-5 188.770912 3.56235E-5 186.002989 3.66913E-5 183.277332 825 3 1 1113 3.77919E-5 180.589987 3.89247E-5 177.943741 4.00923E-5 175.334609 825 3 1 1114 4.12941E-5 172.765485 4.25327E-5 170.232342 4.38076E-5 167.738042 825 3 1 1115 4.51216E-5 165.278762 4.64742E-5 162.857024 4.78681E-5 160.469425 825 3 1 1116 4.93030E-5 158.118170 5.07818E-5 155.800129 5.23041E-5 153.517343 825 3 1 1117 5.38729E-5 151.266771 5.54878E-5 149.050527 5.71521E-5 146.865537 825 3 1 1118 5.88653E-5 144.713824 6.06310E-5 142.592389 6.24484E-5 140.503446 825 3 1 1119 6.43215E-5 138.443898 6.62496E-5 136.415720 6.82368E-5 134.416091 825 3 1 1120 7.02822E-5 132.447076 7.23903E-5 130.505740 7.45603E-5 128.594049 825 3 1 1121 7.67967E-5 126.709244 7.90987E-5 124.853278 8.14712E-5 123.023447 825 3 1 1122 8.39134E-5 121.221495 8.64304E-5 119.444922 8.90212E-5 117.695532 825 3 1 1123 9.16913E-5 115.970774 9.44399E-5 114.272309 9.72725E-5 112.597814 825 3 1 1124 1.00188E-4 110.948839 1.03193E-4 109.323371 1.06287E-4 107.722220 825 3 1 1125 1.09475E-4 106.143789 1.12756E-4 104.589636 1.16139E-4 103.057073 825 3 1 1126 1.19620E-4 101.548352 1.23208E-4 100.060593 1.26901E-4 98.5957142 825 3 1 1127 1.30707E-4 97.1515492 1.34626E-4 95.7291437 1.38664E-4 94.3267642 825 3 1 1128 1.42820E-4 92.9461386 1.47104E-4 91.5847727 1.51513E-4 90.2442698 825 3 1 1129 1.56058E-4 88.9226398 1.60736E-4 87.6211784 1.65557E-4 86.3381325 825 3 1 1130 1.70520E-4 85.0745750 1.75635E-4 83.8287969 1.80899E-4 82.6022361 825 3 1 1131 1.86325E-4 81.3929701 1.91911E-4 80.2020037 1.97667E-4 79.0279134 825 3 1 1132 2.03592E-4 77.8717826 2.09699E-4 76.7319238 2.15985E-4 75.6095385 825 3 1 1133 2.22463E-4 74.5029821 2.29132E-4 73.4132967 2.36004E-4 72.3390620 825 3 1 1134 2.43079E-4 71.2811399 2.50370E-4 70.2381783 2.57875E-4 69.2112070 825 3 1 1135 2.65610E-4 68.1986744 2.73572E-4 67.2016909 2.81777E-4 66.2187812 825 3 1 1136 2.90224E-4 65.2508374 2.98929E-4 64.2965862 3.07890E-4 63.3569435 825 3 1 1137 3.17125E-4 62.4305256 3.26631E-4 61.5183561 3.36428E-4 60.6190187 825 3 1 1138 3.46513E-4 59.7334700 3.56906E-4 58.8604225 3.67605E-4 58.0007272 825 3 1 1139 3.78631E-4 57.1531667 3.89981E-4 56.3186150 4.01678E-4 55.4958311 825 3 1 1140 4.13719E-4 54.6856649 4.26128E-4 53.8869298 4.38901E-4 53.1004516 825 3 1 1141 4.52066E-4 52.3250833 4.65617E-4 51.5615911 4.79583E-4 50.8089026 825 3 1 1142 4.93959E-4 50.0677400 5.08775E-4 49.3370713 5.24026E-4 48.6175944 825 3 1 1143 5.39744E-4 47.9083034 5.55923E-4 47.2098882 5.72598E-4 46.5213590 825 3 1 1144 5.89762E-4 45.8433925 6.07452E-4 45.1750170 6.25661E-4 44.5169143 825 3 1 1145 6.44427E-4 43.8681285 6.63744E-4 43.2292958 6.83653E-4 42.5995211 825 3 1 1146 7.04146E-4 41.9794126 7.25267E-4 41.3680902 7.47007E-4 40.7661738 825 3 1 1147 7.69413E-4 40.1727975 7.92477E-4 39.5885202 8.16247E-4 39.0125496 825 3 1 1148 8.40715E-4 38.4454234 8.65932E-4 37.8863513 8.91889E-4 37.3358858 825 3 1 1149 9.18641E-4 36.7932309 9.46178E-4 36.2589383 9.74558E-4 35.7322340 825 3 1 1150 .001003771 35.2136410 .001033879 34.7024209 .001064871 34.1990810 825 3 1 1151 .001096811 33.7028965 .001129689 33.2143728 .001163573 32.7328000 825 3 1 1152 .001198452 32.2586562 .001234399 31.7912712 .001271402 31.3310970 825 3 1 1153 .001309537 30.8774814 .001348791 30.4308851 .001389247 29.9906610 825 3 1 1154 .001430892 29.5572344 .001473810 29.1300058 .001517989 28.7093823 825 3 1 1155 .001563521 28.2947700 .001610389 27.8865881 .001658691 27.4842444 825 3 1 1156 .001708412 27.0881332 .001759655 26.6976982 .001812403 26.3133204 825 3 1 1157 .001866765 25.9344508 .001922723 25.5614728 .001980394 25.1938427 825 3 1 1158 .002039758 24.8319338 .002100939 24.4752250 .002163917 24.1240659 825 3 1 1159 .002228823 23.7779588 .002295634 23.4372509 .002364490 23.1014493 825 3 1 1160 .002435368 22.7708885 .002508415 22.4450988 .002583608 22.1243965 825 3 1 1161 .002661102 21.8083283 .002740871 21.4972099 .002823082 21.1905910 825 3 1 1162 .002907706 20.8887805 .002994921 20.5913449 .003084697 20.2985762 825 3 1 1163 .003177221 20.0100600 .003272461 19.7260813 .003370617 19.4462336 825 3 1 1164 .003471655 19.1707948 .003575785 18.8993706 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