17-Cl- 35 ENDF/B-VII.0 Processed by Red Cullen using PREPRO2007. 1 0 0 0 17035.0000 34.6684500 0 0 0 11725 1451 1 0.0 0.0 0 0 0 61725 1451 2 1.00000000 20000000.0 9 0 10 71725 1451 3 0.0 0.0 1 0 454 3221725 1451 4 17-Cl- 35 ORNL,LANL EVAL-OCT03 Sayer,Guber,Leal,Larson,Young+ 1725 1451 5 DIST-DEC06 1725 1451 6 ----ENDF/B-VII MATERIAL 1725 1725 1451 7 -----INCIDENT NEUTRON DATA 1725 1451 8 ------ENDF-6 FORMAT 1725 1451 9 ******************************************************************1725 1451 10 ORNL Resonance Parameter Evaluation, October, 2003. 1725 1451 11 R. O. Sayer, K. H. Guber, L. C. Leal, N. M. Larson, T. Rauscher 1725 1451 12 1725 1451 13 Our resonance parameter evaluation is described below. File 3 1725 1451 14 total [MT 1], elastic [MT 2], and capture [MT 102] cross section 1725 1451 15 values for T=0K for were computed from the resonance parameter 1725 1451 16 representation. For the energy range 0.00001 eV to 1.2 MeV, the 1725 1451 17 pointwise File 3 cross sections are based on the resonance 1725 1451 18 parameter files. Above 1.2 MeV, the current (February 2000) ENDF 1725 1451 19 cross sections are used. The CL35 file also contains (n,p) [MT 1725 1451 20 103,600] cross sections for T = 0K. For the energy range 0.00001 1725 1451 21 eV to 121 keV, the pointwise cross sections are based on the 1725 1451 22 resonance parameter file. Above 121 keV, the current (February 1725 1451 23 2000) ENDF cross sections are used. The last resonance with 1725 1451 24 non-zero proton width is at 103.5 keV. 1725 1451 25 1725 1451 26 We performed an evaluation [1] of Cl neutron cross sections in 1725 1451 27 the resolved resonance region with the multilevel Reich-Moore 1725 1451 28 R-matrix formalism. Resonance analyses were carried out with the 1725 1451 29 computer code SAMMY [3], which utilizes Bayes' method, a 1725 1451 30 generalized least squares technique. A recent modification of 1725 1451 31 SAMMY enabled us to calculate charged particle penetrabilities 1725 1451 32 for the proton exit channel. Our evaluation takes advantage of 1725 1451 33 recent high-resolution capture and transmission measurements at 1725 1451 34 the Oak Ridge Electron Linear Accelerator (ORELA) to extend the 1725 1451 35 resolved resonance energy range to 1.2 MeV with much more 1725 1451 36 accurate representation of the data than previous evaluations. 1725 1451 37 1725 1451 38 The total cross section data include measurements by Guber, et 1725 1451 39 al. [2] and Good, et al. [4], on the 80-m flight path at ORELA; 1725 1451 40 Cierjacks, et al. [5], on a 57-m flight path at the Karlsruhe 1725 1451 41 Isochronous Cyclotron; Singh, et al. [6] on the 200-m flight 1725 1451 42 path at the Columbia synchrocyclotron; Brugger, et al. [7], who 1725 1451 43 utilized a crystal spectrometer and also the MTR fast chopper 1725 1451 44 with a flight path of 45 m; Kiehn, et al. [8], with the 1725 1451 45 Rockefeller generator; and Newson, et al. [9], at the Duke Van 1725 1451 46 de Graaff facility. 1725 1451 47 1725 1451 48 Also included in the evaluation were the high resolution capture 1725 1451 49 cross section data (0.1 < En < 500 keV) of Guber, et al. [2] and 1725 1451 50 the older, low resolution capture data (0.02 < En < 1.0 keV) of 1725 1451 51 Kashukeev, et al. [10]. The 35Cl(n,p)35S cross section data of 1725 1451 52 Koehler [11] and Druyts, et al. [12] were also fit. The proton 1725 1451 53 widths are significant fractions of the total widths for 1725 1451 54 resonances at 398 and 4251 eV. 1725 1451 55 1725 1451 56 In order to give a proper treatment for charged particles in an 1725 1451 57 exit channel, an algorithm to calculate charged particle 1725 1451 58 penetrabilities (CPP) and shifts was incorporated in the SAMMY 1725 1451 59 code. The methodology for CPP computation has been given 1725 1451 60 previously [13]. Routines based on the CPP algorithm have been 1725 1451 61 developed and incorporated in a development version of the 1725 1451 62 nuclear data processing code NJOY [14] for use in preparing data 1725 1451 63 for criticality safety benchmark calculations. The nuclear 1725 1451 64 radii used for penetrabilities and shifts were computed 1725 1451 65 according to R = 1.23A**0.33333 + 0.8 fm, where A is the 1725 1451 66 nuclide mass. These values were 4.8222 and 4.8974 fm for 35Cl 1725 1451 67 and 37Cl, respectively. In the SAMMY analysis the radii used to 1725 1451 68 compute hard sphere phase shifts were allowed to vary, and 1725 1451 69 different radii were allowed for s- and p-waves. Final values 1725 1451 70 for 35Cl were R(L=0,1) = 3.6680, 4.8888 fm; final values for 37Cl 1725 1451 71 were R(L=0,1) = 3.3651,3.9565 fm. 1725 1451 72 1725 1451 73 Capture Cross Section Analysis 1725 1451 74 ------------------------------ 1725 1451 75 Guber, et al. [2] measured the neutron capture of chlorine up to 1725 1451 76 500 keV using a natural LiCl sample of thickness 0.09812 atoms/b 1725 1451 77 and the ORELA capture system, which had been re-engineered [20] 1725 1451 78 to minimize the amount of structural material surrounding the 1725 1451 79 sample and detectors. To calculate accurate correction factors 1725 1451 80 for experimental effects of the neutron capture data, reliable 1725 1451 81 neutron widths are needed since the sample was fairly thick. 1725 1451 82 Initial neutron widths were obtained by fitting the 1725 1451 83 transmission data; using these newly determined values, 1725 1451 84 corrections for self-shielding and multiple scattering were 1725 1451 85 calculated with SAMMY and used to determine capture widths. 1725 1451 86 Several iterations of fitting the transmission and capture data 1725 1451 87 were performed to obtain final resonance parameters for 0.1 < En 1725 1451 88 < 500 keV. From their resonance parameters, Guber, et al. [2], 1725 1451 89 calculated average cross sections that were rather different 1725 1451 90 from ENDF/B-VI. This difference is very likely the result of 1725 1451 91 underestimated neutron sensitivity in the older measurements as 1725 1451 92 well as an improved calculation of the weighting function. 1725 1451 93 1725 1451 94 In nuclides where the (n,gamma) cross section is small, the 1725 1451 95 direct capture (DC) is often a significant fraction of the cross 1725 1451 96 section. Guber, et al. [2] describe in detail the DC 1725 1451 97 calculations they performed for 35Cl and 37Cl using the code 1725 1451 98 TEDCA [21, 22]. They calculated that the effect of the DC 1725 1451 99 component was very small for 35Cl where the thermal capture 1725 1451 100 cross section is 43.6 b. However, for 37Cl approximately 0.31 b 1725 1451 101 of the thermal capture cross section of 0.433 b is due to direct 1725 1451 102 capture. We have deduced a set of resonance parameters, 1725 1451 103 including the external level parameters, that reproduce the 1725 1451 104 resonant part of the capture cross section. To this resonant 1725 1451 105 part, one must add the DC contribution to obtain the overall 1725 1451 106 capture cross section. The thermal value of the DC cross section 1725 1451 107 is 0.16 +- 0.05 b for 35Cl and 0.31 +- 0.16 b for 37Cl. 1725 1451 108 1725 1451 109 Thermal and Integral Quantities 1725 1451 110 ------------------------------- 1725 1451 111 The following table gives a comparison of our elastic, capture, 1725 1451 112 (n,p), and total cross sections for En = 0.0253 eV and T = 0K 1725 1451 113 with the corresponding ENDF/B-VI quantities, which are based 1725 1451 114 principally on the compilation of Mughabghab [15]. The capture 1725 1451 115 cross section values include the DC contribution. Also given is 1725 1451 116 the resonance capture integral, I-gamma. 1725 1451 117 1725 1451 118 Cl Thermal Cross Sections and Resonance Integrals for T = 0K 1725 1451 119 Nuclide Quantity ENDF/B-VI (b) Present Evaluation (b) 1725 1451 120 ------- ------- -------------- ---------------------- 1725 1451 121 35Cl total 64.70 +- 0.50 64.75 1725 1451 122 elastic 20.60 +- 0.30 20.67 1725 1451 123 capture 43.60 +- 0.40 43.60 1725 1451 124 (n,p) 0.48 +- 0.14 0.480 1725 1451 125 I-gamma 17.80 +- 2.00 18.19 1725 1451 126 1725 1451 127 37Cl total 1.583 +- 0.050 1.581 1725 1451 128 elastic 1.150 +- 0.050 1.148 1725 1451 129 capture 0.433 +- 0.006 0.433 1725 1451 130 I-gamma 0.204 +- 0.040 0.198 1725 1451 131 1725 1451 132 The new ORELA measurements and the older KFK measurements enabled 1725 1451 133 us to extend the resonance parameter representation to 1.2 MeV; 1725 1451 134 the ENDF/B-VI representation above 226 keV, based on calculations 1725 1451 135 utilizing Hauser-Feshbach statistical theory, is inadequate. 1725 1451 136 1725 1451 137 SUMMARY AND CONCLUSIONS 1725 1451 138 ----------------------- 1725 1451 139 The Cl data used in this evaluation include recent ORELA 1725 1451 140 high-resolution capture and transmission measurements as well as 1725 1451 141 several older data sets. Since the 35Cl(n,p)35S reaction yields 1725 1451 142 a significant contribution to the total cross section from 1725 1451 143 thermal energies up to about 10 keV, the 35Cl(n,p) data of 1725 1451 144 Koehler [11] and Druyts, et al. [12] were fit to obtain proton 1725 1451 145 width values for several resonances. The proton widths are 1725 1451 146 significant fractions of the total widths for resonances at 398 1725 1451 147 and 4251 eV. When uncertainties are considered, there is good 1725 1451 148 agreement between our resonance parameter calculations and 1725 1451 149 experiment for natCl total cross sections up to 1200 keV, for 1725 1451 150 35Cl(n,p) cross sections up to 100 keV, and for natCl capture 1725 1451 151 cross sections up to 500 keV. Our thermal elastic, capture, 1725 1451 152 (n,p), and total cross sections are in good agreement with the 1725 1451 153 corresponding ENDF/B-VI quantities, which are based primarily on 1725 1451 154 the compilation of Mughabghab [15]. 1725 1451 155 1725 1451 156 Our evaluation fits the data much better than does ENDF/B-VI. 1725 1451 157 This new representation should be particularly applicable to 1725 1451 158 improvement of the reliability of criticality safety 1725 1451 159 calculations for systems where Cl is present. 1725 1451 160 1725 1451 161 The present ENDF format does not allow for a resonance parameter 1725 1451 162 representation of charged particle cross sections. A proposal is 1725 1451 163 in preparation for a new ENDF format which will permit the full 1725 1451 164 generality of the Reich-Moore theory, including charged particle 1725 1451 165 penetrabilities. The parametric representation (File 2) will be 1725 1451 166 made available when the new ENDF format is approved. 1725 1451 167 1725 1451 168 REFERENCES 1725 1451 169 ---------- 1725 1451 170 [1] R. O. Sayer, K. H. Guber, L. C. Leal, N. M. Larson, 1725 1451 171 and T. Rauscher, ORNL/TM-2003/50, March, 2003. 1725 1451 172 [2] K. H. Guber, R. O. Sayer, T. E. Valentine, L. C. Leal, 1725 1451 173 R. R. Spencer, J. A. Harvey, P. E. Koehler, and T. Rauscher, 1725 1451 174 Phys. Rev. C65, 058801 (2002). 1725 1451 175 [3] N. M. Larson, ORNL/TM-9179/R5 (2000). 1725 1451 176 [4] W. M. Good, J. A. Harvey, and N. W. Hill, ORNL-4937, 1725 1451 177 p. 198 (1973); J. A. Harvey, private communication. 1725 1451 178 [5] S. Cierjacks, P.Forti, D. Kopsch, L. Kropp, J. Nebe, and H. 1725 1451 179 Unseld, "High Resolution Total Neutron Cross Sections for Na, 1725 1451 180 Cl, K, V, MN and Co between 0.5 and 30 MEV", 1725 1451 181 KFK-1000, (1969). 1725 1451 182 [6] U. N. Singh, H. I. Liou, G. Hacken, M. Slagowitz, F. Rahn, 1725 1451 183 J. Rainwater, W. Makofske, and J. Garg, "Neutron Resonance 1725 1451 184 Spectroscopy: Chlorine", Phys. Rev. C10, 2138 (1974). 1725 1451 185 [7] R. M. Brugger, et al., Phys. Rev. 104, 1054 (1956). 1725 1451 186 [8] R. M. Kiehn, et al., Phys. Rev. 91, 66 (1953). 1725 1451 187 [9] H. W. Newson, et al., Phys. Rev. 105, 198 (1957). 1725 1451 188 [10] N. T. Kashukeev, Yu. P. Popov, and F. L. Shapiro, 1725 1451 189 J. Nucl. Energy 14, 76 (1961). 1725 1451 190 [11] P. E. Koehler, Phys. Rev. C44, 1675 (1991). 1725 1451 191 [12] S. Druyts, C. Wagemans, and P. Geltenbort, 1725 1451 192 Nucl. Phys. A574, 291 (1994). 1725 1451 193 [13] R. O. Sayer, ORNL/TM-2000/212 (2000). 1725 1451 194 [14] R. E. MacFarlane and D. W. Muir, LA-12740-M (1994). 1725 1451 195 [15] S. F. Mughabghab, M. Divadeenam, N. E. Holden, Neutron Cross 1725 1451 196 Sections, Vol. 1, Part A, Academic Press, Inc. (1981). 1725 1451 197 [16] G. H. E. Sims and D. G. Juhnke, Phys. Rev. 165, 1184 (1968). 1725 1451 198 [17] I. G. Schroder, M. McKeown, and G. Schar -Goldhaber, 1725 1451 199 J. Inorg. Nucl. Chem. 31, 3721 (1969). 1725 1451 200 [18] Y. M. Gledenov, V. I. Salatski, P. V. Sedyshev, P. J. 1725 1451 201 Szalanski, J. Andrzejewski, and A. Zak, Proc. Int. Conf. on 1725 1451 202 Nuclear Data for Science and Technology, 1725 1451 203 Trieste, p. 511 (1997). 1725 1451 204 [19] Y. M. Gledenov, L. B. Mitsina, M. Mitukov, Y. P. Popov, J. 1725 1451 205 Rigol, V. I. Salatski, and F. Van Zuan, Joint Institute for 1725 1451 206 Nuclear Research, Communications P3-89-351, 1725 1451 207 Dubna, USSR (1989). 1725 1451 208 [20] P. E. Koehler, et al., Phys. Rev. C54, 1463 (1996). 1725 1451 209 [21] H. Krauss, K. Grun, T. Rauscher, and H. Oberhummer, 1992, 1725 1451 210 TU Wien (Vienna, Austria), code TEDCA (unpublished). 1725 1451 211 [22] T. Rauscher, R. Bieber, H. Oberhummer, K.-L. Kratz, 1725 1451 212 J. Dobaczewski, P. Moller, and M. M. Sharma, 1725 1451 213 Phys.Rev. C57, 2031 (1998). 1725 1451 214 [23] R. L. Macklin, Phys. Rev. C29, 1996 (1984). 1725 1451 215 [24] C. E. Porter and R. G. Thomas, Phys. Rev. 104, 483 (1956). 1725 1451 216 [25] E. P. Wigner, Can. Math. Congr. Proc., Toronto, 1725 1451 217 p 174 (1957); Ann. Math 67, 325 (1958). 1725 1451 218 **************************************************************** 1725 1451 219 1725 1451 220 ENDF/B-VI MOD 1 Evaluation, February 2000, P.G. Young, 1725 1451 221 R.E. MacFarlane, L.C. Liu (LANL) 1725 1451 222 1725 1451 223 NEUTRON ENERGIES BELOW 226 keV 1725 1451 224 1725 1451 225 The resolved resonance parameter data of the JENDL3.2 1725 1451 226 evaluation by Watanabe (Wa94) was adopted. The description of 1725 1451 227 those data in the JENDL3.2 evaluation is repeated below. 1725 1451 228 1725 1451 229 MF=2 RESONANCE PARAMETERS 1725 1451 230 MT=151 RESOLVED RESONANCE PARAMETERS(BELOW 226KEV) 1725 1451 231 Resolved resonance parameters for MLBW formula. 1725 1451 232 Negative energy level parameters were adjusted to reproduce 1725 1451 233 2200m/s cross sections. 1725 1451 234 Evaluation was mainly based on Macklin's data [1] and 1725 1451 235 Mughabghab's compilation [2]. 1725 1451 236 Below 226 keV, (n,p) and (n,alpha) cross sections were given 1725 1451 237 as background total cross section. 1725 1451 238 1725 1451 239 Calculated 2200-m/s cross sections and res. integrals (barns) 1725 1451 240 2200 m/s Res. Integ. 1725 1451 241 Total 64.2 - 1725 1451 242 Elastic 20.6 - 1725 1451 243 Capture 43.6 17.8 1725 1451 244 1725 1451 245 MF=12 PHOTON MULTIPLICITIES 1725 1451 246 The spectrum of gamma rays from radiative capture is based 1725 1451 247 upon a new evaluation by A. Adams and S.C. Frankle (Ad98). 1725 1451 248 1725 1451 249 1725 1451 250 NEUTRON ENERGIES ABOVE 226 keV 1725 1451 251 1725 1451 252 SUMMARY 1725 1451 253 This evaluation is based primarily on a theoretical analysis 1725 1451 254 between neutron energies of 100 keV and 20 MeV that is optimized 1725 1451 255 to the somewhat limited available experimental data. Elastic 1725 1451 256 and inelastic scattering angular distributions (through MT=70) 1725 1451 257 are taken from the JENDL3.2 evaluation [Wa94]. Also, the MF3, 1725 1451 258 MT102 data of JENDL below 4 MeV were adopted. 1725 1451 259 The theoretical calculations utilize Hauser-Feshbach 1725 1451 260 statistical theory with corrections for width fluctuations, 1725 1451 261 preequilibrium and direct reaction processes. Spherical optical 1725 1451 262 model calculations are used to obtain the neutron total cross 1725 1451 263 section and neutron, proton, deuteron, triton, and alpha 1725 1451 264 transmission coefficients. 1725 1451 265 Cross sections and spectra for individual reactions are 1725 1451 266 included for exiting neutron, proton, deuteron, alpha, and 1725 1451 267 gamma-ray reactions. Multiplicities, angular distributions, and 1725 1451 268 emission energy spectra are given for gamma rays, particles, and 1725 1451 269 recoil nuclei emitted in the dominant reactions, utilizing File 1725 1451 270 6 of the ENDF/B-6 format [Ro91]. Energy-angle-correlated 1725 1451 271 spectra are given for all outgoing particles and photons, and 1725 1451 272 residual nuclei energy distributions are included. 1725 1451 273 1725 1451 274 THEORY 1725 1451 275 1725 1451 276 HAUSER-FESHBACH STATISTICAL THEORY CALCULATIONS. The GNASH 1725 1451 277 code [Yo92] was used for all Hauser-Feshbach statistical theory 1725 1451 278 calculations. Preequilibrium corrections were performed in the 1725 1451 279 course of the GNASH calculations using the exciton model of 1725 1451 280 Kalbach [Ka77,Ka85]. Discrete level data from nuclear data 1725 1451 281 sheets were matched to continuum level densities using the 1725 1451 282 formulation of Gilbert and Cameron [Gi65] and pairing and shell 1725 1451 283 parameters from the Cook [Co67] analysis. Neutron and charged- 1725 1451 284 particle transmission coefficients were obtained from the 1725 1451 285 optical potentials, as discussed below. Gamma-ray transmission 1725 1451 286 coefficients were calculated using the Kopecky-Uhl model [Ko90]. 1725 1451 287 Calculations were performed for all significant reactions 1725 1451 288 producing neutrons, protons, deuterons, alpha particles, and 1725 1451 289 gamma rays for incident neutrons between 100 keV and 20 MeV. 1725 1451 290 The angular distribution systematics by Kalbach [Ka88] were 1725 1451 291 used to describe the angular distributions for all continuum 1725 1451 292 particles. 1725 1451 293 1725 1451 294 OPTICAL MODEL POTENTIALS. For incident and exiting neutrons, 1725 1451 295 a phenomenological optical model potential by Arthur and Young 1725 1451 296 [Ar80], based on an analysis of n + Fe and p + Fe reactions, was 1725 1451 297 utilized for the neutron transmission coefficients, whereas the 1725 1451 298 potential of Watanabe [Wa94] was used to calculate the neutron 1725 1451 299 total cross section. The two differenct potentials were used 1725 1451 300 because on the one hand the Watanabe potential agreed well with 1725 1451 301 total cross section measurements, whereas the Arthur potential 1725 1451 302 appears to give a better reaction cross section, which is very 1725 1451 303 important for Hauser-Feshbach calculations. The SCAT2 optical 1725 1451 304 model code [Be92] was used for all calculations. 1725 1451 305 To obtain transmission coefficients for charged particle 1725 1451 306 reactions, the Beccetti-Greenlees potential [Be71] was used for 1725 1451 307 protons, the Perey and Perey [Pe63] potential for deuterons, the 1725 1451 308 Beccetti-Greenlees potential [Be69] for tritons,and the 1725 1451 309 potential of MacFadden [Mc66] was used for alpha particles. 1725 1451 310 1725 1451 311 DIRECT REACTIONS: Energy-dependent cross sections of 1725 1451 312 inelastic neutrons from 35Cl(n,n') direct reactions were 1725 1451 313 obtained using DWUCK calculations and deformation parameters 1725 1451 314 estimated from systematics using the compilations of Raman et 1725 1451 315 al. [Ra89] and Spear [Sp89]. 1725 1451 316 1725 1451 317 EVALUATED DATA 1725 1451 318 1725 1451 319 CALCULATIONAL RESULTS. The MF=3 cross sections and MF=6 1725 1451 320 energy/angle distributions that are based completely on 1725 1451 321 calculations are: 1725 1451 322 1725 1451 323 MT = 16: (n,2n) Reaction 1725 1451 324 MT = 22: (n,nalpha) Reaction 1725 1451 325 MT = 28: (n,np) Reaction 1725 1451 326 MT = 32: (n,nd) Reaction 1725 1451 327 MT = 51-80: (n,n') Discrete Level Reactions 1725 1451 328 MT = 91: (n,n') Continuum Reaction 1725 1451 329 MT = 103: (n,p) Reaction 1725 1451 330 MT = 104: (n,d) Reaction 1725 1451 331 MT = 105: (n,t) Reaction 1725 1451 332 MT = 107: (n,alpha) Reaction 1725 1451 333 MT = 111: (n,2p) Reaction 1725 1451 334 MT = 112: (n,palpha) Reaction 1725 1451 335 MT = 600-619: (n,p) Discrete Level Reactions 1725 1451 336 MT = 649: (n,p) Continuum Reaction 1725 1451 337 MT = 650-669: (n,d) Discrete Level Reactions 1725 1451 338 MT = 699: (n,d) Continuum Reaction 1725 1451 339 MT = 700-730: (n,t) Discrete Level Reactions 1725 1451 340 MT = 749: (n,t) Continuum Reaction 1725 1451 341 MT = 800-824: (n,alpha) Discrete Level Reactions 1725 1451 342 MT = 849: (n,alpha) Continuum Reaction 1725 1451 343 1725 1451 344 Additionally, (n,gamma) cross sections (multiplicities) 1725 1451 345 included in MF=12 and energy distributions in MF=15 are taken 1725 1451 346 from the GNASH calculations. In addition to the usual Hauser- 1725 1451 347 Feshbach cross section component obtained using the Kopecky-Uhl 1725 1451 348 gamma-ray strength function, a semidirect component is included 1725 1451 349 in GNASH that enhances the cross section and hardens the 1725 1451 350 spectrum near En = 10-18 MeV. 1725 1451 351 Discrete (n,n') cross sections and angular distributions were 1725 1451 352 calculated using a combination of the GNASH and COMNUC [Du70] 1725 1451 353 codes for compound nucleus reactions. Preequilibrium components 1725 1451 354 were included in the (n,n') reactions at higher energies to 1725 1451 355 approximate direct reaction effects (in an average manner) for 1725 1451 356 discrete states not included in the DWUCK calculations. Cross 1725 1451 357 sections for a total of 30 excited states are included for 35Cl. 1725 1451 358 Discrete gamma-ray cross sections that exceed 1 mb are included 1725 1451 359 explicitly in the MF=6 distributions for all reactions. The 1725 1451 360 elastic angular distributions are included in in MF =4; the 1725 1451 361 (n,n') angular distributions and (n,n'gamma) multiplicities are 1725 1451 362 included in MF=6. 1725 1451 363 Cross sections (MF=3) for approximately 20 or more discrete 1725 1451 364 states are included for charged-particle reactions. Again, 1725 1451 365 multiplicities for (n,x gamma) reactions are included in MF=6. 1725 1451 366 Kalbach systematics (Ka88) are used to specify all continuum 1725 1451 367 particle angular distributions in MF=6. All continuum photon 1725 1451 368 angular distributions are assumed isotropic. Residual nucleus 1725 1451 369 recoil energy spectra are included in MF=6 for all reactions. 1725 1451 370 1725 1451 371 USE OF EXPERIMENTAL DATA. The available experimental data for 1725 1451 372 35Cl is somewhat limited. Data that were useful for the 1725 1451 373 evaluation are measurements of the neutron total cross section 1725 1451 374 for natural Cl; measurements of (n,gamma) cross sections for 1725 1451 375 35Cl and 37Cl at lower energies; and a few isolated 1725 1451 376 measurements near 14 MeV of (n,2n) or (n,x) reactions leading to 1725 1451 377 radioactive products. 1725 1451 378 The only adjustment made to the calculated cross sections on 1725 1451 379 the basis of the experimental data was to fine tune the 1725 1451 380 normalization of the gamma-ray strength function calculations 1725 1451 381 using the radiative capture measurement. The final 1725 1451 382 normalization that was determined is near the middle of the 1725 1451 383 range of adjustment that we have established from systematics in 1725 1451 384 other analyses. 1725 1451 385 1725 1451 386 **************************************************************** 1725 1451 387 1725 1451 388 REFERENCES 1725 1451 389 1725 1451 390 [Ad98] A. Adams and S.C. Frankle, LANL Group X-CI, personal 1725 1451 391 communication (1998). 1725 1451 392 [Ar80] E.D. Arthur and P.G. Young, Proc. Sym. on Neutron Cross 1725 1451 393 Sections from 10 to 50 MeV, 12-14 May 1980, Brookhaven 1725 1451 394 National Laboratory [Eds. M.R. Bhat and S. Pearlstein], 1725 1451 395 report BNL-NCS-51245 (1980) p.731. 1725 1451 396 [Be92] O. Bersillon, "SCAT2 - A Spherical Optical Model Code," 1725 1451 397 in Proc. ICTP Workshop on Computation and Analysis of Nuclear 1725 1451 398 Data Relevant to Nuclear Energy and Safety, 10 February-13 1725 1451 399 March, 1992, Trieste, Italy, to be published, World Scientific 1725 1451 400 Press, and Progress Report of the Nuclear Physics Division, 1725 1451 401 Bruyeres-le-Chatel 1977, CEA-N-2037 (1978) p. 111 1725 1451 402 [Be71] F.D. Becchetti, Jr., and G.W. Greenlees, Polarization 1725 1451 403 Phenomena in Nuclear Reactions, Proc. Conf. [Ed: H.H.Barschall 1725 1451 404 and W.Haeberli] (The University of Wisconsin Press, 1971) 1725 1451 405 p.682. 1725 1451 406 [Co67] J.L. Cook, H. Ferguson, and A.R. deL Musgrove, Aust.J. 1725 1451 407 Phys. 20, 477 (1967) 1725 1451 408 [Du70] C.L. Dunford, "A Unified Model for Analysis of Compound 1725 1451 409 Nucleus Reactions," Atomics International report AI-AEC-12931 1725 1451 410 (1970). 1725 1451 411 [Gi65] A. Gilbert and A.G.W. Cameron, Can. J. Phys. 43, 1446 1725 1451 412 (1965). 1725 1451 413 [Ka77] C. Kalbach, Z.Phys.A 283, 401 (1977) 1725 1451 414 [Ka85] C. Kalbach, Los Alamos National Laboratory report 1725 1451 415 LA-10248-MS (1985) 1725 1451 416 [Ka88] C. Kalbach, Phys.Rev.C 37, 2350 (1988); see also 1725 1451 417 see also C. Kalbach and F.M. Mann, Phys.Rev.C 23, 112 (1981). 1725 1451 418 [Ko90] J. Kopecky and M. Uhl, Phys.Rev. C 41, 1941 (1990) 1725 1451 419 [Mc66] L. McFadden and G.R. Satchler, Nucl.Phys. 84, 177 (1966). 1725 1451 420 [Pe63a] C.M. Perey and F.G. Perey, Phys.Rev. 132, 755 (1963) 1725 1451 421 [Pe63b] F.G. Perey, Phys.Rev. 131, 745 (1963) 1725 1451 422 [Pe72] F.G. Perey, et al., report ORNL-4823 (1972) 1725 1451 423 [Ra89] S. Raman et al., At. & Nucl. Data Tab. 42, 1 (1989). 1725 1451 424 [Ro91] P. Rose, Brookhaven National Laboratory informal report 1725 1451 425 BNL-NCS-44945 [ENDF-102, Rev. 10/91] (1991) 1725 1451 426 [Sp89] R.H. Spear, At. & Nucl. Data Tab. 42, 55 (1989). 1725 1451 427 [Wa94] T. Watanabe, JENDL-3.2 Evaluation (1994). 1725 1451 428 [Yo92] P.G. Young, E.D. Arthur, and M.B. Chadwick, Los Alamos 1725 1451 429 report LA-12343-MS (1992) 1725 1451 430 1725 1451 431 ************************ C O N T E N T S *********************** 1725 1451 432 ***************** Program LINEAR (VERSION 2007-1) ***************1725 1451 433 For All Data Greater than 1.0000E-10 barns in Absolute Value 1725 1451 434 Data Linearized Using Energy Dependent Uncertainty 1725 1451 435 Energy Accuracy 1725 1451 436 (eV) (per-cent) 1725 1451 437 ----------- ----------- 1725 1451 438 0.0 .010000000 1725 1451 439 1.00000000 .010000000 1725 1451 440 10.0000000 .100000000 1725 1451 441 2.00000E+9 .100000000 1725 1451 442 ***************** Program FIXUP (Version 2007-1) ****************1725 1451 443 Corrected ZA/AWR in All Sections-----------------------------Yes 1725 1451 444 Corrected Thresholds-----------------------------------------No 1725 1451 445 Extended Cross Sections to 20 MeV----------------------------No 1725 1451 446 Allow Cross Section Deletion---------------------------------Yes 1725 1451 447 Allow Cross Section Reconstruction---------------------------Yes 1725 1451 448 Make All Cross Sections Non-Negative-------------------------Yes 1725 1451 449 Delete Energies Not in Ascending Order-----------------------Yes 1725 1451 450 Deleted Duplicate Points-------------------------------------Yes 1725 1451 451 Check for Ascending MAT/MF/MT Order--------------------------Yes 1725 1451 452 Check for Legal MF/MT Numbers--------------------------------Yes 1725 1451 453 Allow Creation of Missing Sections---------------------------No 1725 1451 454 Allow Insertion of Energy Points-----------------------------No 1725 1451 455 Create Uniform Energy Grid-----------------------------------No 1725 1451 456 Delete Section if Cross Section =0 at All Energies-----------Yes 1725 1451 457 **************** Program DICTIN (VERSION 2007-1) ****************1725 1451 458 1 451 780 11725 1451 459 2 151 4 11725 1451 460 3 1 6702 11725 1451 461 3 2 3607 11725 1451 462 3 4 37 01725 1451 463 3 16 8 01725 1451 464 3 22 11 01725 1451 465 3 28 10 01725 1451 466 3 32 6 01725 1451 467 3 51 17 01725 1451 468 3 52 16 01725 1451 469 3 53 15 01725 1451 470 3 54 15 01725 1451 471 3 55 15 01725 1451 472 3 56 14 01725 1451 473 3 57 15 01725 1451 474 3 58 14 01725 1451 475 3 59 14 01725 1451 476 3 60 14 01725 1451 477 3 61 14 01725 1451 478 3 62 13 01725 1451 479 3 63 15 01725 1451 480 3 64 16 01725 1451 481 3 65 15 01725 1451 482 3 66 16 01725 1451 483 3 67 16 01725 1451 484 3 68 16 01725 1451 485 3 69 16 01725 1451 486 3 70 13 01725 1451 487 3 71 15 01725 1451 488 3 72 14 01725 1451 489 3 73 14 01725 1451 490 3 74 15 01725 1451 491 3 75 14 01725 1451 492 3 76 14 01725 1451 493 3 77 14 01725 1451 494 3 78 14 01725 1451 495 3 79 13 01725 1451 496 3 80 13 01725 1451 497 3 91 13 01725 1451 498 3 102 6415 11725 1451 499 3 103 839 11725 1451 500 3 104 41 01725 1451 501 3 105 39 01725 1451 502 3 107 109 11725 1451 503 3 111 9 01725 1451 504 3 112 10 01725 1451 505 3 600 805 11725 1451 506 3 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9.16126148 54972.0200 8.60832179 54974.5900 8.111396611725 3 1 1854 54977.7500 7.56874044 54980.9100 7.09138851 54984.0700 6.669138931725 3 1 1855 54987.2300 6.29485915 54990.2700 5.97355974 54993.3200 5.685507941725 3 1 1856 54996.3600 5.42638171 54999.4000 5.19249180 55005.7200 4.774160751725 3 1 1857 55012.0400 4.42946650 55018.8300 4.12205837 55025.6100 3.865705591725 3 1 1858 55032.8700 3.63546927 55040.1200 3.44118570 55048.0800 3.260613761725 3 1 1859 55056.0400 3.10705449 55064.7000 2.96451626 55073.3600 2.842508301725 3 1 1860 55082.9600 2.72640180 55092.5600 2.62656161 55103.0900 2.532099491725 3 1 1861 55113.6200 2.45043785 55125.3200 2.37185480 55137.0200 2.303706361725 3 1 1862 55150.1300 2.24175726 55163.2300 2.17989087 55177.9800 2.127212821725 3 1 1863 55192.7300 2.07456298 55209.1100 2.03013087 55225.4900 1.985720391725 3 1 1864 55243.7500 1.94791666 55262.0000 1.91015046 55282.6000 1.877502741725 3 1 1865 55303.1900 1.84488431 55326.1300 1.81877816 55349.0700 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1891 57822.4900 29.7240673 57827.9300 28.4525465 57833.3800 26.84826021725 3 1 1892 57848.0900 21.8836209 57855.4400 19.4040722 57862.7900 17.18289481725 3 1 1893 57868.7800 15.5621264 57874.7700 14.1156526 57880.7600 12.83371751725 3 1 1894 57886.7500 11.7034236 57892.7400 10.7096830 57898.7300 9.835252531725 3 1 1895 57904.7300 9.06569817 57910.7100 8.38804822 57918.0700 7.662862941725 3 1 1896 57925.4200 7.03813280 57932.7700 6.49751556 57940.1200 6.027502351725 3 1 1897 57947.2100 5.63124581 57954.2900 5.28229377 57968.4400 4.699272451725 3 1 1898 57983.1500 4.22021033 57997.8600 3.83736379 58013.6500 3.506444161725 3 1 1899 58029.4400 3.23849707 58046.3300 3.00514888 58063.2100 2.813883441725 3 1 1900 58081.7300 2.64135077 58100.2500 2.49899417 58120.3900 2.370713501725 3 1 1901 58140.5500 2.26408284 58162.8800 2.16570032 58185.2100 2.083622191725 3 1 1902 58209.7100 2.00828062 58234.2200 1.94511296 58261.4500 1.886180341725 3 1 1903 58288.6800 1.83662984 58319.1800 1.78992929 58349.6800 1.753839881725 3 1 1904 58383.9900 1.71333671 58418.3100 1.68444825 58456.4300 1.652434241725 3 1 1905 58494.5500 1.62948108 58537.0300 1.60395951 58579.5200 1.585557831725 3 1 1906 58627.4400 1.56484967 58675.3700 1.54984184 58728.7400 1.533166031725 3 1 1907 58782.1100 1.52100300 58842.0200 1.50737752 58901.9300 1.498020241725 3 1 1908 58967.2900 1.48783308 59032.6400 1.47766524 59103.4400 1.470490781725 3 1 1909 59174.2400 1.46332974 59255.9400 1.45507961 59337.6300 1.449595841725 3 1 1910 59430.2100 1.44339214 59522.8000 1.43719725 59626.2800 1.432812381725 3 1 1911 59729.7600 1.42843513 59844.1300 1.42360437 59958.5000 1.418779741725 3 1 1912 60028.3500 1.41711779 60115.0400 1.41505652 60256.9800 1.411687141725 3 1 1913 60398.9200 1.40832305 60527.3400 1.40528345 60655.7700 1.404188311725 3 1 1914 60770.6700 1.40321158 60885.5700 1.40223782 60986.9600 1.401381241725 3 1 1915 61088.3400 1.40250371 61176.2100 1.40347936 61264.0800 1.404457581725 3 1 1916 61345.1900 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5.107593361725 3 1 1929 62663.8800 5.48131339 62671.3100 5.90573528 62678.7400 6.388618621725 3 1 1930 62686.1800 6.93889734 62693.6100 7.56486942 62701.0500 8.276001161725 3 1 1931 62708.4800 9.08051308 62715.9200 9.98287938 62725.0400 11.22324321725 3 1 1932 62734.1700 12.5883891 62752.4200 15.4135935 62759.1800 16.32937631725 3 1 1933 62765.9300 17.0641449 62772.6900 17.5471852 62779.4500 17.72586631725 3 1 1934 62786.2100 17.5801575 62792.9700 17.1268168 62799.7300 16.41629691725 3 1 1935 62806.4900 15.5179270 62824.7400 12.7326776 62833.8600 11.34098511725 3 1 1936 62842.9900 10.0938858 62850.4200 9.18475469 62857.8600 8.373095411725 3 1 1937 62865.2900 7.65488008 62872.7300 7.02205243 62880.1600 6.465509501725 3 1 1938 62887.6000 5.97670988 62895.0300 5.54697866 62902.4700 5.168305971725 3 1 1939 62911.5900 4.76392698 62920.7100 4.41589268 62929.8400 4.114822961725 3 1 1940 62938.9600 3.85335499 62947.7500 3.63313317 62956.5400 3.439343611725 3 1 1941 62974.1100 3.11596595 62992.3600 2.85069992 63010.6100 2.638964261725 3 1 1942 63030.2100 2.45621873 63049.8100 2.30851774 63070.7700 2.179985771725 3 1 1943 63091.7200 2.07476153 63114.7000 1.97994224 63137.6800 1.901777161725 3 1 1944 63162.6900 1.83139901 63187.7000 1.77293940 63215.4100 1.719014921725 3 1 1945 63243.1200 1.67403634 63273.5400 1.63272893 63303.9500 1.600970021725 3 1 1946 63337.7500 1.56569881 63371.5400 1.54066904 63409.3900 1.512653701725 3 1 1947 63447.2500 1.49262616 63489.8300 1.47011894 63532.4100 1.453883311725 3 1 1948 63579.7200 1.43585745 63627.0400 1.42267854 63679.7600 1.408006021725 3 1 1949 63732.4800 1.39709963 63791.9600 1.38480300 63851.4400 1.376020501725 3 1 1950 63917.6800 1.36624632 63983.9100 1.35647902 64058.2600 1.348719101725 3 1 1951 64132.6100 1.34096349 64213.7200 1.33250665 64294.8300 1.326618871725 3 1 1952 64382.6900 1.32024408 64470.5600 1.31387107 64571.9500 1.306520051725 3 1 1953 64673.3400 1.29917123 64866.2700 1.28519234 65022.0400 1.273909411725 3 1 1954 65177.8200 1.26262833 65341.5400 1.25077452 65505.2600 1.238922841725 3 1 1955 65647.1600 1.22664175 65789.0500 1.21436303 65920.0200 1.203030771725 3 1 1956 66051.0100 1.18869717 66171.0700 1.17556118 66291.1300 1.162426981725 3 1 1957 66398.0900 1.14799520 66505.0600 1.13356420 66601.1200 1.118277941725 3 1 1958 66697.1600 1.10299745 66782.3000 1.08713550 66867.4400 1.071276731725 3 1 1959 66943.8400 1.05480549 67020.2400 1.03833828 67089.0100 1.021021881725 3 1 1960 67157.7700 1.00371320 67218.8900 .988333226 67280.0200 .9709545551725 3 1 1961 67334.5900 .955447857 67389.1600 .939949549 67438.2800 .9260081681725 3 1 1962 67487.4000 .912077711 67532.1500 .899398656 67576.9000 .8899109951725 3 1 1963 67617.2900 .881363792 67657.6700 .877860604 67676.2300 .8762584511725 3 1 1964 67694.7800 .878291026 67731.8900 .882378560 67765.7300 .8946633891725 3 1 1965 67799.5600 .916830951 67831.2200 .950333129 67862.8700 1.001458351725 3 1 1966 67892.3400 1.07163740 67921.8100 1.17301024 67936.0000 1.236750261725 3 1 1967 67950.1900 1.31285675 67964.3800 1.40384288 67978.5700 1.512883151725 3 1 1968 67993.3000 1.64924957 68008.0400 1.81451848 68022.7700 2.015422141725 3 1 1969 68037.5100 2.26041239 68049.5200 2.49991253 68061.5200 2.782611311725 3 1 1970 68073.5200 3.11661391 68085.5300 3.51209933 68097.5400 3.980139011725 3 1 1971 68109.5500 4.53338691 68121.5500 5.18539136 68133.5500 5.948955171725 3 1 1972 68148.2900 7.05553939 68163.0300 8.35599539 68177.7700 9.829781041725 3 1 1973 68192.5000 11.4147852 68203.4100 12.5885398 68214.3300 13.68998221725 3 1 1974 68225.2400 14.6412732 68236.1600 15.3707431 68247.0700 15.82683371725 3 1 1975 68257.9800 15.9891693 68268.9000 15.8712594 68279.8100 15.51406861725 3 1 1976 68294.5500 14.7525878 68309.2900 13.8026160 68324.0200 12.78933211725 3 1 1977 68338.7600 11.7755607 68350.7700 10.9975868 68362.7700 10.27343731725 3 1 1978 68374.7700 9.60765304 68386.7800 9.00120306 68398.7900 8.451802611725 3 1 1979 68410.8000 7.95556265 68422.8000 7.50790590 68434.8000 7.104358811725 3 1 1980 68449.5400 6.66206853 68464.2700 6.27112661 68479.0200 5.924400511725 3 1 1981 68493.7500 5.61627816 68507.9400 5.35098998 68522.1200 5.112508951725 3 1 1982 68536.3100 4.89740761 68550.5100 4.70264841 68579.9800 4.353290341725 3 1 1983 68609.4500 4.06390377 68641.1000 3.80485873 68672.7500 3.587877191725 3 1 1984 68706.5900 3.39233476 68740.4200 3.22660715 68777.5300 3.072037021725 3 1 1985 68814.6400 2.94017560 68855.0300 2.81728222 68895.4100 2.711703651725 3 1 1986 68940.1600 2.61095976 68984.9100 2.52404171 69034.0300 2.441508901725 3 1 1987 69083.1500 2.36993410 69137.7300 2.30533434 69192.3000 2.240754861725 3 1 1988 69253.4200 2.18590114 69314.5500 2.13104504 69383.3000 2.084101201725 3 1 1989 69452.0700 2.03714893 69528.4800 1.99728219 69604.8800 1.957424671725 3 1 1990 69690.0200 1.92329087 69775.1500 1.88916420 69871.2000 1.857557361725 3 1 1991 69967.2500 1.83155726 70074.2200 1.80260350 70181.1800 1.780161571725 3 1 1992 70301.2400 1.75497290 70421.3100 1.73534621 70552.2900 1.713937561725 3 1 1993 70683.2700 1.69712049 70825.1600 1.67890370 70967.0500 1.664507441725 3 1 1994 71130.7700 1.64789717 71294.5000 1.63549915 71480.0500 1.621449601725 3 1 1995 71665.6000 1.60740066 72080.3700 1.58525599 72309.5800 1.573019351725 3 1 1996 72538.7900 1.56432205 73062.7000 1.54444403 73652.1000 1.528431821725 3 1 1997 73979.5500 1.51953660 74306.9900 1.51327176 74817.2700 1.503509791725 3 1 1998 74956.4300 1.50084807 75101.2200 1.49807957 75153.2300 1.497085641725 3 1 1999 75205.2500 1.49609215 75257.2700 1.49509993 75283.2800 1.494604701725 3 1 2000 75309.2900 1.49411056 75322.2900 1.49386419 75335.3000 1.493618231725 3 1 2001 75348.3000 1.49337328 75361.3000 1.49312949 75374.3000 1.492887361725 3 1 2002 75380.8100 1.49276699 75387.3100 1.49264759 75393.8100 1.492529171725 3 1 2003 75400.3100 1.49241202 75406.8200 1.49229635 75413.3200 1.492183071725 3 1 2004 75419.8200 1.49207280 75423.0700 1.49201914 75426.3300 1.491966571725 3 1 2005 75429.5800 1.49191566 75432.8300 1.49186657 75436.0800 1.491819721725 3 1 2006 75439.3300 1.49177565 75442.5800 1.49173508 75445.8300 1.491698951725 3 1 2007 75449.0900 1.49166850 75452.3400 1.49164577 75455.5900 1.491633281725 3 1 2008 75457.2100 1.49163211 75458.8400 1.49163491 75460.4600 1.491642851725 3 1 2009 75462.0900 1.49165657 75463.7100 1.49167773 75465.3400 1.491707601725 3 1 2010 75467.0200 1.49175057 75468.5300 1.49180150 75470.0400 1.491867511725 3 1 2011 75471.3700 1.49194134 75472.7000 1.49203370 75473.8900 1.492136911725 3 1 2012 75475.0900 1.49226356 75476.1500 1.49240123 75477.2100 1.492568751725 3 1 2013 75478.1400 1.49274581 75479.0700 1.49295844 75479.9100 1.493190491725 3 1 2014 75480.7600 1.49346879 75481.5100 1.49376506 75482.2700 1.494123321725 3 1 2015 75482.9300 1.49449820 75483.5900 1.49494468 75484.1600 1.495399101725 3 1 2016 75484.7400 1.49594382 75485.2700 1.49653699 75485.8000 1.497242851725 3 1 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