17-Cl- 37 ENDF/B-VII.0 Processed by Red Cullen using PREPRO2007. 1 0 0 0 17037.0000 36.6483000 0 0 0 11731 1451 1 0.0 0.0 0 0 0 61731 1451 2 1.00000000 20000000.0 9 0 10 71731 1451 3 1200.00000 0.0 1 0 460 1561731 1451 4 17-Cl- 37 ORNL,LANL EVAL-OCT03 Sayer,Guber,Leal,Larson,Young+ 1731 1451 5 DIST-DEC06 1731 1451 6 ----ENDF/B-VII MATERIAL 1731 1731 1451 7 -----INCIDENT NEUTRON DATA 1731 1451 8 ------ENDF-6 FORMAT 1731 1451 9 ******************************************************************1731 1451 10 ORNL Resonance Parameter Evaluation, October, 2003. 1731 1451 11 R. O. Sayer, K. H. Guber, L. C. Leal, N. M. Larson, T. Rauscher 1731 1451 12 1731 1451 13 Our resonance parameter evaluation is described below. File 3 1731 1451 14 total [MT 1], elastic [MT 2], and capture [MT 102] cross section 1731 1451 15 values for T=0K for were computed from the resonance parameter 1731 1451 16 representation. For the energy range 0.00001 eV to 1.2 MeV, the 1731 1451 17 pointwise File 3 cross sections are based on the resonance 1731 1451 18 parameter files. Above 1.2 MeV, the current (February 2000) ENDF 1731 1451 19 cross sections are used. The CL35 file also contains (n,p) [MT 1731 1451 20 103,600] cross sections for T = 0K. For the energy range 0.00001 1731 1451 21 eV to 121 keV, the pointwise cross sections are based on the 1731 1451 22 resonance parameter file. Above 121 keV, the current (February 1731 1451 23 2000) ENDF cross sections are used. The last resonance with 1731 1451 24 non-zero proton width is at 103.5 keV. 1731 1451 25 1731 1451 26 We performed an evaluation [1] of Cl neutron cross sections in 1731 1451 27 the resolved resonance region with the multilevel Reich-Moore 1731 1451 28 R-matrix formalism. Resonance analyses were carried out with the 1731 1451 29 computer code SAMMY [3], which utilizes Bayes' method, a 1731 1451 30 generalized least squares technique. A recent modification of 1731 1451 31 SAMMY enabled us to calculate charged particle penetrabilities 1731 1451 32 for the proton exit channel. Our evaluation takes advantage of 1731 1451 33 recent high-resolution capture and transmission measurements at 1731 1451 34 the Oak Ridge Electron Linear Accelerator (ORELA) to extend the 1731 1451 35 resolved resonance energy range to 1.2 MeV with much more 1731 1451 36 accurate representation of the data than previous evaluations. 1731 1451 37 1731 1451 38 The total cross section data include measurements by Guber, et 1731 1451 39 al. [2] and Good, et al. [4], on the 80-m flight path at ORELA; 1731 1451 40 Cierjacks, et al. [5], on a 57-m flight path at the Karlsruhe 1731 1451 41 Isochronous Cyclotron; Singh, et al. [6] on the 200-m flight 1731 1451 42 path at the Columbia synchrocyclotron; Brugger, et al. [7], who 1731 1451 43 utilized a crystal spectrometer and also the MTR fast chopper 1731 1451 44 with a flight path of 45 m; Kiehn, et al. [8], with the 1731 1451 45 Rockefeller generator; and Newson, et al. [9], at the Duke Van 1731 1451 46 de Graaff facility. 1731 1451 47 1731 1451 48 Also included in the evaluation were the high resolution capture 1731 1451 49 cross section data (0.1 < En < 500 keV) of Guber, et al. [2] and 1731 1451 50 the older, low resolution capture data (0.02 < En < 1.0 keV) of 1731 1451 51 Kashukeev, et al. [10]. The 35Cl(n,p)35S cross section data of 1731 1451 52 Koehler [11] and Druyts, et al. [12] were also fit. The proton 1731 1451 53 widths are significant fractions of the total widths for 1731 1451 54 resonances at 398 and 4251 eV. 1731 1451 55 1731 1451 56 In order to give a proper treatment for charged particles in an 1731 1451 57 exit channel, an algorithm to calculate charged particle 1731 1451 58 penetrabilities (CPP) and shifts was incorporated in the SAMMY 1731 1451 59 code. The methodology for CPP computation has been given 1731 1451 60 previously [13]. Routines based on the CPP algorithm have been 1731 1451 61 developed and incorporated in a development version of the 1731 1451 62 nuclear data processing code NJOY [14] for use in preparing data 1731 1451 63 for criticality safety benchmark calculations. The nuclear 1731 1451 64 radii used for penetrabilities and shifts were computed 1731 1451 65 according to R = 1.23A**0.33333 + 0.8 fm, where A is the 1731 1451 66 nuclide mass. These values were 4.8222 and 4.8974 fm for 35Cl 1731 1451 67 and 37Cl, respectively. In the SAMMY analysis the radii used to 1731 1451 68 compute hard sphere phase shifts were allowed to vary, and 1731 1451 69 different radii were allowed for s- and p-waves. Final values 1731 1451 70 for 35Cl were R(L=0,1) = 3.6680, 4.8888 fm; final values for 37Cl 1731 1451 71 were R(L=0,1) = 3.3651,3.9565 fm. 1731 1451 72 1731 1451 73 Capture Cross Section Analysis 1731 1451 74 ------------------------------ 1731 1451 75 Guber, et al. [2] measured the neutron capture of chlorine up to 1731 1451 76 500 keV using a natural LiCl sample of thickness 0.09812 atoms/b 1731 1451 77 and the ORELA capture system, which had been re-engineered [20] 1731 1451 78 to minimize the amount of structural material surrounding the 1731 1451 79 sample and detectors. To calculate accurate correction factors 1731 1451 80 for experimental effects of the neutron capture data, reliable 1731 1451 81 neutron widths are needed since the sample was fairly thick. 1731 1451 82 Initial neutron widths were obtained by fitting the 1731 1451 83 transmission data; using these newly determined values, 1731 1451 84 corrections for self-shielding and multiple scattering were 1731 1451 85 calculated with SAMMY and used to determine capture widths. 1731 1451 86 Several iterations of fitting the transmission and capture data 1731 1451 87 were performed to obtain final resonance parameters for 0.1 < En 1731 1451 88 < 500 keV. From their resonance parameters, Guber, et al. [2], 1731 1451 89 calculated average cross sections that were rather different 1731 1451 90 from ENDF/B-VI. This difference is very likely the result of 1731 1451 91 underestimated neutron sensitivity in the older measurements as 1731 1451 92 well as an improved calculation of the weighting function. 1731 1451 93 1731 1451 94 In nuclides where the (n,gamma) cross section is small, the 1731 1451 95 direct capture (DC) is often a significant fraction of the cross 1731 1451 96 section. Guber, et al. [2] describe in detail the DC 1731 1451 97 calculations they performed for 35Cl and 37Cl using the code 1731 1451 98 TEDCA [21, 22]. They calculated that the effect of the DC 1731 1451 99 component was very small for 35Cl where the thermal capture 1731 1451 100 cross section is 43.6 b. However, for 37Cl approximately 0.31 b 1731 1451 101 of the thermal capture cross section of 0.433 b is due to direct 1731 1451 102 capture. We have deduced a set of resonance parameters, 1731 1451 103 including the external level parameters, that reproduce the 1731 1451 104 resonant part of the capture cross section. To this resonant 1731 1451 105 part, one must add the DC contribution to obtain the overall 1731 1451 106 capture cross section. The thermal value of the DC cross section 1731 1451 107 is 0.16 +- 0.05 b for 35Cl and 0.31 +- 0.16 b for 37Cl. 1731 1451 108 1731 1451 109 Thermal and Integral Quantities 1731 1451 110 ------------------------------- 1731 1451 111 The following table gives a comparison of our elastic, capture, 1731 1451 112 (n,p), and total cross sections for En = 0.0253 eV and T = 0K 1731 1451 113 with the corresponding ENDF/B-VI quantities, which are based 1731 1451 114 principally on the compilation of Mughabghab [15]. The capture 1731 1451 115 cross section values include the DC contribution. Also given is 1731 1451 116 the resonance capture integral, I-gamma. 1731 1451 117 1731 1451 118 Cl Thermal Cross Sections and Resonance Integrals for T = 0K 1731 1451 119 Nuclide Quantity ENDF/B-VI (b) Present Evaluation (b) 1731 1451 120 ------- ------- -------------- ---------------------- 1731 1451 121 35Cl total 64.70 +- 0.50 64.75 1731 1451 122 elastic 20.60 +- 0.30 20.67 1731 1451 123 capture 43.60 +- 0.40 43.60 1731 1451 124 (n,p) 0.48 +- 0.14 0.480 1731 1451 125 I-gamma 17.80 +- 2.00 18.19 1731 1451 126 1731 1451 127 37Cl total 1.583 +- 0.050 1.581 1731 1451 128 elastic 1.150 +- 0.050 1.148 1731 1451 129 capture 0.433 +- 0.006 0.433 1731 1451 130 I-gamma 0.204 +- 0.040 0.198 1731 1451 131 1731 1451 132 The new ORELA measurements and the older KFK measurements enabled 1731 1451 133 us to extend the resonance parameter representation to 1.2 MeV; 1731 1451 134 the ENDF/B-VI representation above 226 keV, based on calculations 1731 1451 135 utilizing Hauser-Feshbach statistical theory, is inadequate. 1731 1451 136 1731 1451 137 SUMMARY AND CONCLUSIONS 1731 1451 138 ----------------------- 1731 1451 139 The Cl data used in this evaluation include recent ORELA 1731 1451 140 high-resolution capture and transmission measurements as well as 1731 1451 141 several older data sets. Since the 35Cl(n,p)35S reaction yields 1731 1451 142 a significant contribution to the total cross section from 1731 1451 143 thermal energies up to about 10 keV, the 35Cl(n,p) data of 1731 1451 144 Koehler [11] and Druyts, et al. [12] were fit to obtain proton 1731 1451 145 width values for several resonances. The proton widths are 1731 1451 146 significant fractions of the total widths for resonances at 398 1731 1451 147 and 4251 eV. When uncertainties are considered, there is good 1731 1451 148 agreement between our resonance parameter calculations and 1731 1451 149 experiment for natCl total cross sections up to 1200 keV, for 1731 1451 150 35Cl(n,p) cross sections up to 100 keV, and for natCl capture 1731 1451 151 cross sections up to 500 keV. Our thermal elastic, capture, 1731 1451 152 (n,p), and total cross sections are in good agreement with the 1731 1451 153 corresponding ENDF/B-VI quantities, which are based primarily on 1731 1451 154 the compilation of Mughabghab [15]. 1731 1451 155 1731 1451 156 Our evaluation fits the data much better than does ENDF/B-VI. 1731 1451 157 This new representation should be particularly applicable to 1731 1451 158 improvement of the reliability of criticality safety 1731 1451 159 calculations for systems where Cl is present. 1731 1451 160 1731 1451 161 The present ENDF format does not allow for a resonance parameter 1731 1451 162 representation of charged particle cross sections. A proposal is 1731 1451 163 in preparation for a new ENDF format which will permit the full 1731 1451 164 generality of the Reich-Moore theory, including charged particle 1731 1451 165 penetrabilities. The parametric representation (File 2) will be 1731 1451 166 made available when the new ENDF format is approved. 1731 1451 167 1731 1451 168 REFERENCES 1731 1451 169 ---------- 1731 1451 170 [1] R. O. Sayer, K. H. Guber, L. C. Leal, N. M. Larson, 1731 1451 171 and T. Rauscher, ORNL/TM-2003/50, March, 2003. 1731 1451 172 [2] K. H. Guber, R. O. Sayer, T. E. Valentine, L. C. Leal, 1731 1451 173 R. R. Spencer, J. A. Harvey, P. E. Koehler, and T. Rauscher, 1731 1451 174 Phys. Rev. C65, 058801 (2002). 1731 1451 175 [3] N. M. Larson, ORNL/TM-9179/R5 (2000). 1731 1451 176 [4] W. M. Good, J. A. Harvey, and N. W. Hill, ORNL-4937, 1731 1451 177 p. 198 (1973); J. A. Harvey, private communication. 1731 1451 178 [5] S. Cierjacks, P.Forti, D. Kopsch, L. Kropp, J. Nebe, and H. 1731 1451 179 Unseld, "High Resolution Total Neutron Cross Sections for Na, 1731 1451 180 Cl, K, V, MN and Co between 0.5 and 30 MEV", 1731 1451 181 KFK-1000, (1969). 1731 1451 182 [6] U. N. Singh, H. I. Liou, G. Hacken, M. Slagowitz, F. Rahn, 1731 1451 183 J. Rainwater, W. Makofske, and J. Garg, "Neutron Resonance 1731 1451 184 Spectroscopy: Chlorine", Phys. Rev. C10, 2138 (1974). 1731 1451 185 [7] R. M. Brugger, et al., Phys. Rev. 104, 1054 (1956). 1731 1451 186 [8] R. M. Kiehn, et al., Phys. Rev. 91, 66 (1953). 1731 1451 187 [9] H. W. Newson, et al., Phys. Rev. 105, 198 (1957). 1731 1451 188 [10] N. T. Kashukeev, Yu. P. Popov, and F. L. Shapiro, 1731 1451 189 J. Nucl. Energy 14, 76 (1961). 1731 1451 190 [11] P. E. Koehler, Phys. Rev. C44, 1675 (1991). 1731 1451 191 [12] S. Druyts, C. Wagemans, and P. Geltenbort, 1731 1451 192 Nucl. Phys. A574, 291 (1994). 1731 1451 193 [13] R. O. Sayer, ORNL/TM-2000/212 (2000). 1731 1451 194 [14] R. E. MacFarlane and D. W. Muir, LA-12740-M (1994). 1731 1451 195 [15] S. F. Mughabghab, M. Divadeenam, N. E. Holden, Neutron Cross 1731 1451 196 Sections, Vol. 1, Part A, Academic Press, Inc. (1981). 1731 1451 197 [16] G. H. E. Sims and D. G. Juhnke, Phys. Rev. 165, 1184 (1968). 1731 1451 198 [17] I. G. Schroder, M. McKeown, and G. Schar -Goldhaber, 1731 1451 199 J. Inorg. Nucl. Chem. 31, 3721 (1969). 1731 1451 200 [18] Y. M. Gledenov, V. I. Salatski, P. V. Sedyshev, P. J. 1731 1451 201 Szalanski, J. Andrzejewski, and A. Zak, Proc. Int. Conf. on 1731 1451 202 Nuclear Data for Science and Technology, 1731 1451 203 Trieste, p. 511 (1997). 1731 1451 204 [19] Y. M. Gledenov, L. B. Mitsina, M. Mitukov, Y. P. Popov, J. 1731 1451 205 Rigol, V. I. Salatski, and F. Van Zuan, Joint Institute for 1731 1451 206 Nuclear Research, Communications P3-89-351, 1731 1451 207 Dubna, USSR (1989). 1731 1451 208 [20] P. E. Koehler, et al., Phys. Rev. C54, 1463 (1996). 1731 1451 209 [21] H. Krauss, K. Grun, T. Rauscher, and H. Oberhummer, 1992, 1731 1451 210 TU Wien (Vienna, Austria), code TEDCA (unpublished). 1731 1451 211 [22] T. Rauscher, R. Bieber, H. Oberhummer, K.-L. Kratz, 1731 1451 212 J. Dobaczewski, P. Moller, and M. M. Sharma, 1731 1451 213 Phys.Rev. C57, 2031 (1998). 1731 1451 214 [23] R. L. Macklin, Phys. Rev. C29, 1996 (1984). 1731 1451 215 [24] C. E. Porter and R. G. Thomas, Phys. Rev. 104, 483 (1956). 1731 1451 216 [25] E. P. Wigner, Can. Math. Congr. Proc., Toronto, 1731 1451 217 p 174 (1957); Ann. Math 67, 325 (1958). 1731 1451 218 **************************************************************** 1731 1451 219 1731 1451 220 ENDF/B-VI MOD 1 Evaluation, February 2000, P.G. Young, 1731 1451 221 R.E. MacFarlane, L.C. Liu (LANL) 1731 1451 222 1731 1451 223 NEUTRON ENERGIES BELOW 202 keV ---------------------------------- 1731 1451 224 1731 1451 225 The resolved resonance parameter data of the JENDL3.2 1731 1451 226 evaluation by Watanabe (Wa94) was adopted. The description of 1731 1451 227 those data in the JENDL3.2 evaluation is repeated below. 1731 1451 228 1731 1451 229 MF=2 RESONANCE PARAMETERS(BELOW 202.0KEV) 1731 1451 230 MT=151 RESOLVED RESONANCE PARAMETERS 1731 1451 231 Resolved resonance parameters for MLBW formula with varying 1731 1451 232 scattering radius. Negative energy level data were adjusted 1731 1451 233 to reproduce 2200m/s cross sections. 1731 1451 234 Evaluation was mainly based on macklin's data [1] and 1731 1451 235 Mughabghab's compilation [2]. 1731 1451 236 1731 1451 237 Calculated 2200-m/s cross section and res. integrals (barns) 1731 1451 238 2200 m/s Res. Integ. 1731 1451 239 Total 1.583 - 1731 1451 240 Elastic 1.15 - 1731 1451 241 Capture 0.433 0.204 1731 1451 242 1731 1451 243 MF=12 PHOTON MULTIPLICITIES 1731 1451 244 The spectrum of gamma rays from radiative capture is based 1731 1451 245 upon a new evaluation by A. Adams and S.C. Frankle [Ad98]. 1731 1451 246 1731 1451 247 NEUTRON ENERGIES ABOVE 202 keV ---------------------------------- 1731 1451 248 1731 1451 249 SUMMARY 1731 1451 250 This evaluation is based primarily on a theoretical analysis 1731 1451 251 between neutron energies of 100 keV and 20 MeV that is optimized 1731 1451 252 to the somewhat limited available experimental data. Elastic 1731 1451 253 and inelastic scattering angular distributions (through MT=76) 1731 1451 254 and the radiative capture cross section (MF=3, MT=102) 1731 1451 255 are taken from the JENDL3.2 evaluation [Wa94]. 1731 1451 256 The theoretical calculations utilize Hauser-Feshbach 1731 1451 257 statistical theory with corrections for width fluctuations, 1731 1451 258 preequilibrium and direct reaction processes. Spherical optical 1731 1451 259 model calculations are used to obtain the neutron total cross 1731 1451 260 section and neutron, proton, deuteron, triton, and alpha 1731 1451 261 transmission coefficients. 1731 1451 262 Cross sections and spectra for individual reactions are 1731 1451 263 included for exiting neutron, proton, deuteron, alpha, and 1731 1451 264 gamma-ray reactions. Multiplicities, angular distributions, and 1731 1451 265 emission energy spectra are given for gamma rays, particles, and 1731 1451 266 recoil nuclei emitted in the dominant reactions, utilizing File 1731 1451 267 6 of the ENDF/B-6 format [Ro91]. Energy-angle-correlated 1731 1451 268 spectra are given for all outgoing particles and photons, and 1731 1451 269 residual nuclei energy distributions are included. 1731 1451 270 1731 1451 271 THEORY 1731 1451 272 HAUSER-FESHBACH STATISTICAL THEORY CALCULATIONS. The GNASH 1731 1451 273 code [Yo92] was used for all Hauser-Feshbach statistical theory 1731 1451 274 calculations. Preequilibrium corrections were performed in the 1731 1451 275 course of the GNASH calculations using the exciton model of 1731 1451 276 Kalbach [Ka77,Ka85]. Discrete level data from nuclear data 1731 1451 277 sheets were matched to continuum level densities using the 1731 1451 278 formulation of Gilbert and Cameron [Gi65] and pairing and shell 1731 1451 279 parameters from the Cook [Co67] analysis. Neutron and charged- 1731 1451 280 particle transmission coefficients were obtained from the 1731 1451 281 optical potentials, as discussed below. Gamma-ray transmission 1731 1451 282 coefficients were calculated using the Kopecky-Uhl model [Ko90]. 1731 1451 283 Calculations were performed for all significant reactions 1731 1451 284 producing neutrons, protons, deuterons, alpha particles, and 1731 1451 285 gamma rays for incident neutrons between 100 keV and 20 MeV. 1731 1451 286 The angular distribution systematics by Kalbach [Ka88] were 1731 1451 287 used to describe the angular distributions for all continuum 1731 1451 288 particles. 1731 1451 289 1731 1451 290 OPTICAL MODEL POTENTIALS. For incident and exiting neutrons, 1731 1451 291 a phenomenological optical model potential by Arthur and Young 1731 1451 292 [Ar80], based on an analysis of n + Fe and p + Fe reactions, was 1731 1451 293 utilized for the neutron transmission coefficients, whereas the 1731 1451 294 potential of Watanabe [Wa94] was used to calculate the neutron 1731 1451 295 total cross section. The two differenct potentials were used 1731 1451 296 because on the one hand the Watanabe potential agreed well with 1731 1451 297 total cross section measurements, whereas the Arthur potential 1731 1451 298 appears to give a better reaction cross section, which is very 1731 1451 299 important for Hauser-Feshbach calculations. The SCAT2 optical 1731 1451 300 model code [Be92] was used for all calculations. 1731 1451 301 To obtain transmission coefficients for charged particle 1731 1451 302 reactions, the Beccetti-Greenlees potential [Be71] was used for 1731 1451 303 protons, the Perey and Perey [Pe63] potential for deuterons, the 1731 1451 304 Beccetti-Greenlees potential [Be69] for tritons,and the potential 1731 1451 305 of MacFadden [Mc66] was used for alpha particles. 1731 1451 306 1731 1451 307 DIRECT REACTIONS: Energy-dependent cross sections of 1731 1451 308 inelastic neutrons from 37Cl(n,n') direct reactions were 1731 1451 309 obtained using DWUCK calculations and deformation parameters 1731 1451 310 estimated from systematics using the compilations of Raman et 1731 1451 311 al. [Ra89] and Spear [Sp89]. 1731 1451 312 1731 1451 313 EVALUATED DATA 1731 1451 314 1731 1451 315 CALCULATIONAL RESULTS. The MF=3 cross sections and MF=6 1731 1451 316 energy/angle distributions that are based completely on 1731 1451 317 calculations are: 1731 1451 318 1731 1451 319 MT = 16: (n,2n) Reaction 1731 1451 320 MT = 17: (n,3n) Reaction 1731 1451 321 MT = 22: (n,nalpha) Reaction 1731 1451 322 MT = 28: (n,np) Reaction 1731 1451 323 MT = 32: (n,nd) Reaction 1731 1451 324 MT = 51-80: (n,n') Discrete Level Reactions 1731 1451 325 MT = 91: (n,n') Continuum Reaction 1731 1451 326 MT = 103: (n,p) Reaction 1731 1451 327 MT = 104: (n,d) Reaction 1731 1451 328 MT = 105: (n,t) Reaction 1731 1451 329 MT = 107: (n,alpha) Reaction 1731 1451 330 MT = 649: (n,p) Continuum Reaction 1731 1451 331 MT = 650-669: (n,d) Discrete Level Reactions 1731 1451 332 MT = 699: (n,d) Continuum Reaction 1731 1451 333 MT = 700-730: (n,t) Discrete Level Reactions 1731 1451 334 MT = 749: (n,t) Continuum Reaction 1731 1451 335 MT = 800-824: (n,alpha) Discrete Level Reactions 1731 1451 336 MT = 849: (n,alpha) Continuum Reaction 1731 1451 337 1731 1451 338 Additionally, (n,gamma) cross sections (multiplicities) 1731 1451 339 included in MF=12 and energy distributions in MF=15 are taken 1731 1451 340 from the GNASH calculations. In addition to the usual Hauser- 1731 1451 341 Feshbach cross section component obtained using the Kopecky-Uhl 1731 1451 342 gamma-ray strength function, a semidirect component is included 1731 1451 343 in GNASH that enhances the cross section and hardens the 1731 1451 344 spectrum near En = 10-18 MeV. 1731 1451 345 Discrete (n,n') cross sections and angular distributions were 1731 1451 346 calculated using a combination of the GNASH and COMNUC [Du70] 1731 1451 347 codes for compound nucleus reactions. Preequilibrium components 1731 1451 348 were included in the (n,n') reactions at higher energies to 1731 1451 349 approximate direct reaction effects (in an average manner) for 1731 1451 350 discrete states not included in the DWUCK calculations. Cross 1731 1451 351 sections for a total of 30 excited states are included for 37Cl. 1731 1451 352 Discrete gamma-ray cross sections that exceed 1 mb are included 1731 1451 353 explicitly in the MF=6 distributions for all reactions. The 1731 1451 354 elastic angular distributions are included in in MF =4; the 1731 1451 355 (n,n') angular distributions and (n,n'gamma) multiplicities are 1731 1451 356 included in MF=6. 1731 1451 357 Cross sections (MF=3) for approximately 20 or more discrete 1731 1451 358 states are included for charged-particle reactions. Again, 1731 1451 359 multiplicities for (n,x gamma) reactions are included in MF=6. 1731 1451 360 Kalbach systematics (Ka88) are used to specify all continuum 1731 1451 361 particle angular distributions in MF=6. All continuum photon 1731 1451 362 angular distributions are assumed isotropic. Residual nucleus 1731 1451 363 recoil energy spectra are included in MF=6 for all reactions. 1731 1451 364 1731 1451 365 USE OF EXPERIMENTAL DATA. The available experimental data for 1731 1451 366 37Cl is somewhat limited. Data that were useful for the 1731 1451 367 evaluation are measurements of the neutron total cross section 1731 1451 368 for natural Cl; measurements of (n,gamma) cross sections for 1731 1451 369 35Cl and 37Cl at lower energies; and a few measurements above 1731 1451 370 12 MeV of (n,p) and (n,alpha) cross sections. 1731 1451 371 The only adjustment made to the calculated cross sections on 1731 1451 372 the basis of the experimental data was to fine tune the 1731 1451 373 normalization of the gamma-ray strength function calculations 1731 1451 374 using the radiative capture measurement. The final 1731 1451 375 normalization that was determined is approximately a factor of 2 1731 1451 376 higher than the value we have established from systematics in 1731 1451 377 other analyses. 1731 1451 378 1731 1451 379 **************************************************************** 1731 1451 380 1731 1451 381 REFERENCES 1731 1451 382 1731 1451 383 [Ad98] A. Adams and S.C. Frankle, LANL Group X-CI, personal 1731 1451 384 communication (1998). 1731 1451 385 [Ar80] E.D.Arthur and P.G. Young, "Evaluation of Neutron Cross 1731 1451 386 Sections to 40 MeV for 54,56Fe," Proc. Sym Neutron Cross 1731 1451 387 Sections from 10 to 50 MeV, BNL, 12-14 May 1980, p. 731. 1731 1451 388 [Be92] O. Bersillon, "SCAT2 - A Spherical Optical Model Code," 1731 1451 389 in Proc. ICTP Workshop on Computation and Analysis of Nuclear 1731 1451 390 Data Relevant to Nuclear Energy and Safety, 10 February-13 1731 1451 391 March, 1992, Trieste, Italy, to be published in World 1731 1451 392 |Scientific Press, and Progress Report of the Nuclear Physics 1731 1451 393 Division, Bruyeres-le-Chatel 1977, CEA-N-2037 (1978) p.111. 1731 1451 394 [Be71] F.D. Becchetti, Jr., and G.W. Greenlees in "Polarization 1731 1451 395 Phenomena in Nuclear Reactions," (Ed: H.H.Barschall and 1731 1451 396 W.Haeberli, The University of Wisconsin Press, 1971) p.682. 1731 1451 397 [Co67] J.L. Cook, H. Ferguson, and A.R. Musgrove, Aust.J.Phys. 1731 1451 398 20, 477 (1967). 1731 1451 399 [Du70] C.L. Dunford, "A Unified Model for Analysis of Compound 1731 1451 400 Nucleus Reactions," Atomics International report AI-AEC-12931 1731 1451 401 (1970). 1731 1451 402 [Gi65] A. Gilbert and A.G.W. Cameron, Can.J.Phys. 43, 1446 1731 1451 403 (1965). 1731 1451 404 [Ka77] C. Kalbach, Z.Phys.A 283, 401 (1977). 1731 1451 405 [Ka85] C. Kalbach, "PRECO-D2: Program for Calculating 1731 1451 406 Preequilibrium and Direct Reaction Double Differential Cross 1731 1451 407 Sections," Los Alamos National Laboratory report LA-10248-MS 1731 1451 408 (1985). 1731 1451 409 [Ka88] C.Kalbach, Phys.Rev.C 37, 2350 (1988); see also 1731 1451 410 C. Kalbach and F. M. Mann, Phys.Rev.C 23, 112 (1981). 1731 1451 411 [Ko90] J.Kopecky and M.Uhl, Phys.Rev.C 42, 1941 (1990). 1731 1451 412 [Mc66] L. McFadden and G.R. Satchler, Nucl. Phys. 84, 177 (1966).1731 1451 413 [Pe63a] F.G. Perey, Phys. Rev. 131, 745 (1963). 1731 1451 414 [Pe63b] C.M. Perey and F.G. Perey, Phys. Rev. 132, 755 (1963). 1731 1451 415 [Pe72] F.G. Perey, et al., Oak Ridge report ORNL-4823 (1972). 1731 1451 416 [Ra89] S. Raman et al., At.Nucl.Data Tables 42, 1 (1989). 1731 1451 417 [Ro91] P. Rose, "ENDF-102: Data Formats and Procedures for the 1731 1451 418 Evaluated Nuclear Data File, ENDF-6," Brookhaven National 1731 1451 419 Laboratory informal report BNL-NCS-44945 [ENDF-102, Rev. 10/91]1731 1451 420 (1991). 1731 1451 421 [Sp89] R.H. Spear, At.Nucl.Data Tables 42, 55 (1989). 1731 1451 422 [Wa94] T. Watanabe, JENDL-3.2 Evaluation (1994). 1731 1451 423 [Yo92] P.G. Young, E.D. Arthur, and M.B. Chadwick, Los Alamos 1731 1451 424 report LA-12343-MS (1992). 1731 1451 425 1731 1451 426 ************************ C O N T E N T S *********************** 1731 1451 427 ***************** Program LINEAR (VERSION 2007-1) ***************1731 1451 428 For All Data Greater than 1.0000E-10 barns in Absolute Value 1731 1451 429 Data Linearized Using Energy Dependent Uncertainty 1731 1451 430 Energy Accuracy 1731 1451 431 (eV) (per-cent) 1731 1451 432 ----------- ----------- 1731 1451 433 0.0 .010000000 1731 1451 434 1.00000000 .010000000 1731 1451 435 10.0000000 .100000000 1731 1451 436 2.00000E+9 .100000000 1731 1451 437 ***************** Program SIGMA1 (VERSION 2007-1) ***************1731 1451 438 Data Doppler Broadened to 1200.00000 Kelvin 1731 1451 439 for All Data Greater than 1.0000E-10 barns in Absolute Value 1731 1451 440 Data Linearized Using Energy Dependent Uncertainty 1731 1451 441 Energy Accuracy 1731 1451 442 (eV) (per-cent) 1731 1451 443 ----------- ----------- 1731 1451 444 0.0 .010000000 1731 1451 445 1.00000000 .010000000 1731 1451 446 10.0000000 .100000000 1731 1451 447 2.00000E+9 .100000000 1731 1451 448 ***************** Program FIXUP (Version 2007-1) ****************1731 1451 449 Corrected ZA/AWR in All Sections-----------------------------Yes 1731 1451 450 Corrected Thresholds-----------------------------------------No 1731 1451 451 Extended Cross Sections to 20 MeV----------------------------No 1731 1451 452 Allow Cross Section Deletion---------------------------------Yes 1731 1451 453 Allow Cross Section Reconstruction---------------------------Yes 1731 1451 454 Make All Cross Sections Non-Negative-------------------------Yes 1731 1451 455 Delete Energies Not in Ascending Order-----------------------Yes 1731 1451 456 Deleted Duplicate Points-------------------------------------Yes 1731 1451 457 Check for Ascending MAT/MF/MT Order--------------------------Yes 1731 1451 458 Check for Legal MF/MT Numbers--------------------------------Yes 1731 1451 459 Allow Creation of Missing Sections---------------------------No 1731 1451 460 Allow Insertion of Energy Points-----------------------------No 1731 1451 461 Create Uniform Energy Grid-----------------------------------No 1731 1451 462 Delete Section if Cross Section =0 at All Energies-----------Yes 1731 1451 463 **************** Program DICTIN (VERSION 2007-1) ****************1731 1451 464 1 451 620 11731 1451 465 2 151 4 11731 1451 466 3 1 7740 11731 1451 467 3 2 2788 11731 1451 468 3 4 32 01731 1451 469 3 16 9 01731 1451 470 3 17 4 01731 1451 471 3 22 10 01731 1451 472 3 28 11 01731 1451 473 3 32 6 01731 1451 474 3 51 16 01731 1451 475 3 52 16 01731 1451 476 3 53 16 01731 1451 477 3 54 14 01731 1451 478 3 55 13 01731 1451 479 3 56 14 01731 1451 480 3 57 14 01731 1451 481 3 58 14 01731 1451 482 3 59 15 01731 1451 483 3 60 14 01731 1451 484 3 61 14 01731 1451 485 3 62 14 01731 1451 486 3 63 15 01731 1451 487 3 64 15 01731 1451 488 3 65 16 01731 1451 489 3 66 17 01731 1451 490 3 67 16 01731 1451 491 3 68 16 01731 1451 492 3 69 16 01731 1451 493 3 70 16 01731 1451 494 3 71 16 01731 1451 495 3 72 15 01731 1451 496 3 73 15 01731 1451 497 3 74 14 01731 1451 498 3 75 14 01731 1451 499 3 76 14 01731 1451 500 3 77 13 01731 1451 501 3 91 13 01731 1451 502 3 102 5253 11731 1451 503 3 103 11 01731 1451 504 3 104 21 01731 1451 505 3 105 21 01731 1451 506 3 107 21 01731 1451 507 3 649 11 01731 1451 508 3 650 14 01731 1451 509 3 651 11 01731 1451 510 3 652 13 01731 1451 511 3 653 12 01731 1451 512 3 654 12 01731 1451 513 3 655 11 01731 1451 514 3 656 11 01731 1451 515 3 657 11 01731 1451 516 3 658 10 01731 1451 517 3 659 10 01731 1451 518 3 660 9 01731 1451 519 3 661 9 01731 1451 520 3 699 8 01731 1451 521 3 700 13 01731 1451 522 3 701 11 01731 1451 523 3 702 12 01731 1451 524 3 703 12 01731 1451 525 3 704 11 01731 1451 526 3 705 11 01731 1451 527 3 706 10 01731 1451 528 3 707 10 01731 1451 529 3 708 10 01731 1451 530 3 709 10 01731 1451 531 3 710 10 01731 1451 532 3 711 9 01731 1451 533 3 712 9 01731 1451 534 3 713 8 01731 1451 535 3 714 8 01731 1451 536 3 715 7 01731 1451 537 3 749 7 01731 1451 538 3 800 16 01731 1451 539 3 801 16 01731 1451 540 3 802 14 01731 1451 541 3 803 14 01731 1451 542 3 804 13 01731 1451 543 3 805 11 01731 1451 544 3 849 11 01731 1451 545 4 2 208 11731 1451 546 6 16 1034 11731 1451 547 6 17 64 11731 1451 548 6 22 1281 11731 1451 549 6 28 1439 11731 1451 550 6 32 253 11731 1451 551 6 51 206 11731 1451 552 6 52 200 11731 1451 553 6 53 162 11731 1451 554 6 54 186 11731 1451 555 6 55 185 11731 1451 556 6 56 152 11731 1451 557 6 57 153 11731 1451 558 6 58 181 11731 1451 559 6 59 152 11731 1451 560 6 60 181 11731 1451 561 6 61 148 11731 1451 562 6 62 171 11731 1451 563 6 63 31 11731 1451 564 6 64 31 11731 1451 565 6 65 29 11731 1451 566 6 66 31 11731 1451 567 6 67 31 11731 1451 568 6 68 35 11731 1451 569 6 69 29 11731 1451 570 6 70 31 11731 1451 571 6 71 29 11731 1451 572 6 72 29 11731 1451 573 6 73 31 11731 1451 574 6 74 29 11731 1451 575 6 75 29 11731 1451 576 6 76 33 11731 1451 577 6 77 22 11731 1451 578 6 91 1792 11731 1451 579 6 649 1400 11731 1451 580 6 650 13 11731 1451 581 6 651 22 11731 1451 582 6 652 22 11731 1451 583 6 653 22 11731 1451 584 6 654 22 11731 1451 585 6 655 22 11731 1451 586 6 656 24 11731 1451 587 6 657 22 11731 1451 588 6 658 24 11731 1451 589 6 659 22 11731 1451 590 6 660 24 11731 1451 591 6 661 24 11731 1451 592 6 699 523 11731 1451 593 6 700 13 11731 1451 594 6 701 22 11731 1451 595 6 702 22 11731 1451 596 6 703 22 11731 1451 597 6 704 26 11731 1451 598 6 705 26 11731 1451 599 6 706 30 11731 1451 600 6 707 26 11731 1451 601 6 708 34 11731 1451 602 6 709 32 11731 1451 603 6 710 34 11731 1451 604 6 711 34 11731 1451 605 6 712 26 11731 1451 606 6 713 36 11731 1451 607 6 714 24 11731 1451 608 6 715 28 11731 1451 609 6 749 338 11731 1451 610 6 800 13 11731 1451 611 6 801 22 11731 1451 612 6 802 22 11731 1451 613 6 803 24 11731 1451 614 6 804 24 11731 1451 615 6 805 30 11731 1451 616 6 849 1160 11731 1451 617 12 102 341 01731 1451 618 14 102 1 11731 1451 619 15 102 672 11731 1451 620 1731 1 0 621 1731 0 0 622 17037.0000 36.6483000 0 0 1 01731 2151 623 17037.0000 1.00000000 0 0 1 01731 2151 624 1.00000E-5 1200000.00 0 0 0 01731 2151 625 1.50000000 .488561000 0 0 0 01731 2151 626 1731 2 0 627 1731 0 0 628 17037.0000 36.6483000 0 0 0 01731 3 1 629 0.0 0.0 0 0 1 232111731 3 1 630 23211 2 1731 3 1 631 1.00000E-5 43.5498868 1.02999E-5 42.9119457 1.06087E-5 42.28356781731 3 1 632 1.09269E-5 41.6641265 1.12544E-5 41.0541596 1.15920E-5 40.45280201731 3 1 633 1.19395E-5 39.8605892 1.22976E-5 39.2767620 1.26662E-5 38.70181441731 3 1 634 1.30462E-5 38.1349346 1.34372E-5 37.5768239 1.38403E-5 37.02649441731 3 1 635 1.42552E-5 36.4846355 1.46827E-5 35.9504181 1.51229E-5 35.42429581731 3 1 636 1.55765E-5 34.9055786 1.60434E-5 34.3948792 1.65246E-5 33.89132621731 3 1 637 1.70199E-5 33.3954871 1.75304E-5 32.9066644 1.80559E-5 32.42524711731 3 1 638 1.85975E-5 31.9506567 1.91550E-5 31.4833120 1.97295E-5 31.02258521731 3 1 639 2.03209E-5 30.5688599 2.09305E-5 30.1215237 2.15579E-5 29.68109231731 3 1 640 2.22045E-5 29.2468310 2.28701E-5 28.8192342 2.35561E-5 28.39763511731 3 1 641 2.42622E-5 27.9825333 2.49899E-5 27.5732690 2.57390E-5 27.17025921731 3 1 642 2.65110E-5 26.7729567 2.73057E-5 26.3817028 2.81247E-5 25.99600861731 3 1 643 2.89678E-5 25.6161758 2.98367E-5 25.2417208 3.07311E-5 24.87300971731 3 1 644 3.16528E-5 24.5095122 3.26017E-5 24.1515559 3.35795E-5 23.79867711731 3 1 645 3.45861E-5 23.4511845 3.56235E-5 23.1086094 3.66913E-5 22.77128421731 3 1 646 3.77919E-5 22.4387199 3.89247E-5 22.1112614 4.00923E-5 21.78841531731 3 1 647 4.12941E-5 21.4705397 4.25327E-5 21.1571367 4.38076E-5 20.84856011731 3 1 648 4.51216E-5 20.5443370 4.64742E-5 20.2447793 4.78681E-5 19.94946631731 3 1 649 4.93030E-5 19.6586704 5.07818E-5 19.3720047 5.23041E-5 19.08972161731 3 1 650 5.38729E-5 18.8114450 5.54878E-5 18.5374362 5.71521E-5 18.26731501731 3 1 651 5.88653E-5 18.0013320 6.06310E-5 17.7391160 6.24484E-5 17.48094091731 3 1 652 6.43215E-5 17.2264237 6.62496E-5 16.9758086 6.82368E-5 16.72874711731 3 1 653 7.02822E-5 16.4854941 7.23903E-5 16.2456873 7.45603E-5 16.00956921731 3 1 654 7.67967E-5 15.7767992 7.90987E-5 15.5476184 8.14712E-5 15.32169311731 3 1 655 8.39134E-5 15.0992383 8.64304E-5 14.8799455 8.90212E-5 14.66403741731 3 1 656 9.16913E-5 14.4511992 9.44399E-5 14.2416356 9.72725E-5 14.03506031731 3 1 657 1.00188E-4 13.8316641 1.03193E-4 13.6311990 1.06287E-4 13.43376481731 3 1 658 1.09475E-4 13.2391645 1.12756E-4 13.0475901 1.16139E-4 12.85871041731 3 1 659 1.19620E-4 12.6728028 1.23208E-4 12.4895123 1.26901E-4 12.30907551731 3 1 660 1.30707E-4 12.1312253 1.34626E-4 11.9560905 1.38664E-4 11.78345761731 3 1 661 1.42820E-4 11.6135392 1.47104E-4 11.4460285 1.51513E-4 11.28112261731 3 1 662 1.56058E-4 11.1185766 1.60736E-4 10.9585499 1.65557E-4 10.80082691731 3 1 663 1.70520E-4 10.6455395 1.75635E-4 10.4924774 1.80899E-4 10.34181751731 3 1 664 1.86325E-4 10.1933234 1.91911E-4 10.0471185 1.97667E-4 9.903028051731 3 1 665 2.03592E-4 9.76118488 2.09699E-4 9.62138193 2.15985E-4 9.483766481731 3 1 666 2.22463E-4 9.34813683 2.29132E-4 9.21462063 2.36004E-4 9.083043811731 3 1 667 2.43079E-4 8.95351184 2.50370E-4 8.82585910 2.57875E-4 8.700211551731 3 1 668 2.65610E-4 8.57637929 2.73572E-4 8.45449800 2.81777E-4 8.334387251731 3 1 669 2.90224E-4 8.21615596 2.98929E-4 8.09964849 3.07890E-4 7.984976591731 3 1 670 3.17125E-4 7.87197124 3.26631E-4 7.76075723 3.36428E-4 7.651161731731 3 1 671 3.46513E-4 7.54330121 3.56906E-4 7.43701872 3.67605E-4 7.332417721731 3 1 672 3.78631E-4 7.22934996 3.89981E-4 7.12792155 4.01678E-4 7.027981541731 3 1 673 4.13719E-4 6.92963300 4.26128E-4 6.83273171 4.38901E-4 6.737531751731 3 1 674 4.40762E-4 6.72397059 4.52066E-4 6.64368766 4.55898E-4 6.617079671731 3 1 675 4.65617E-4 6.55130130 4.71554E-4 6.51202169 4.79583E-4 6.460240741731 3 1 676 4.87748E-4 6.40876813 4.93959E-4 6.37059797 5.04498E-4 6.307294851731 3 1 677 5.08775E-4 6.28224868 5.21824E-4 6.20756750 5.24026E-4 6.195280051731 3 1 678 5.39744E-4 6.10957163 5.55923E-4 6.02551373 5.58280E-4 6.013542611731 3 1 679 5.72598E-4 5.94266923 5.77452E-4 5.91918216 5.89762E-4 5.861126201731 3 1 680 5.97283E-4 5.82645757 6.07452E-4 5.78076630 6.17794E-4 5.735351501731 3 1 681 6.25661E-4 5.70167475 6.39010E-4 5.64583152 6.44427E-4 5.623739121731 3 1 682 6.60955E-4 5.55787307 6.63744E-4 5.54703663 6.83653E-4 5.471459981731 3 1 683 7.04146E-4 5.39735402 7.07131E-4 5.38680368 7.25267E-4 5.324333381731 3 1 684 7.31415E-4 5.30363615 7.47007E-4 5.25247681 7.56533E-4 5.221933171731 3 1 685 7.69413E-4 5.18167953 7.82513E-4 5.14167401 7.92477E-4 5.112012301731 3 1 686 8.09386E-4 5.06283332 8.16247E-4 5.04337982 8.37182E-4 4.985390161731 3 1 687 8.40715E-4 4.97584891 8.65932E-4 4.90932631 8.91889E-4 4.844114981731 3 1 688 8.95669E-4 4.83483509 9.18641E-4 4.77987526 9.26428E-4 4.761671731731 3 1 689 9.46178E-4 4.71667474 9.58243E-4 4.68981912 9.74558E-4 4.654422541731 3 1 690 9.91151E-4 4.61925463 .001003771 4.59318210 .001025188 4.549963321731 3 1 691 .001033879 4.53286624 .001060395 4.48192046 .001064871 4.473536201731 3 1 692 .001096811 4.41510888 .001129689 4.35785003 .001134477 4.349703771731 3 1 693 .001163573 4.30146205 .001173437 4.28548648 .001198452 4.246002011731 3 1 694 .001213734 4.22244264 .001234399 4.19139147 .001255416 4.160550681731 3 1 695 .001271402 4.13768464 .001298529 4.09979526 .001309537 4.084806741731 3 1 696 .001343122 4.04015862 .001348791 4.03281117 .001389247 3.981623501731 3 1 697 .001430892 3.93147504 .001436956 3.92434368 .001473810 3.882107781731 3 1 698 .001486304 3.86812615 .001517989 3.83356937 .001537346 3.812957441731 3 1 699 .001563521 3.78579116 .001590141 3.75881992 .001610389 3.738822311731 3 1 700 .001644749 3.70569811 .001658691 3.69259541 .001701232 3.653576111731 3 1 701 .001708412 3.64716346 .001759655 3.60250438 .001765606 3.597440991731 3 1 702 .001812403 3.55868934 .001826240 3.54750470 .001866765 3.515579481731 3 1 703 .001888956 3.49851748 .001922723 3.47321174 .001953826 3.450465161731 3 1 704 .001980394 3.43155449 .002029453 3.39748445 .002039758 3.390528911731 3 1 705 .002100939 3.35024691 .002108044 3.34568148 .002163917 3.310804911731 3 1 706 .002189641 3.29513761 .002228823 3.27195002 .002274436 3.245617961731 3 1 707 .002295634 3.23372466 .002362473 3.19715110 .002364490 3.196078221731 3 1 708 .002435368 3.15931716 .002453961 3.14990988 .002508415 3.123139891731 3 1 709 .002548947 3.10370628 .002583608 3.08755522 .002647657 3.058454161731 3 1 710 .002661102 3.05251576 .002740871 3.01816998 .002750140 3.014277601731 3 1 711 .002823082 2.98451555 .002856641 2.97116399 .002907706 2.951418921731 3 1 712 .002967214 2.92898837 .002994921 2.91883576 .003082121 2.887694791731 3 1 713 .003084697 2.88680026 .003177221 2.85549471 .003201421 2.847512751731 3 1 714 .003272461 2.82473918 .003325398 2.80820045 .003370617 2.794465891731 3 1 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1.84730968 .014143550 1.840752491731 3 1 741 .014335873 1.83534671 .014765869 1.82364267 .015131654 1.813997391731 3 1 742 .015208491 1.81204415 .015664661 1.80081909 .016134225 1.789629841731 3 1 743 .016188790 1.78837022 .016618162 1.77882462 .017116308 1.768104811731 3 1 744 .017393190 1.76233511 .017629702 1.75758716 .018158171 1.747322631731 3 1 745 .018686861 1.73738343 .018702814 1.73709436 .019263450 1.727269801731 3 1 746 .019841246 1.71747423 .020161848 1.71221396 .020436008 1.707880601731 3 1 747 .021048973 1.69851217 .021679938 1.68918386 .021753258 1.688134921731 3 1 748 .022330215 1.68018660 .022999587 1.67127118 .023569760 1.663926381731 3 1 749 .023689445 1.66243604 .024399561 1.65389066 .025204987 1.644549851731 3 1 750 .025268741 1.64382228 .025300000 1.64347291 .026058858 1.635309031731 3 1 751 .026840000 1.62718874 .027645049 1.61909922 .028473738 1.611364231731 3 1 752 .029327791 1.60366367 .030206922 1.59600404 .030334954 1.594925741731 3 1 753 .031112960 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