95-Am-241 ENDF/B-VII.0 Processed by Red Cullen using PREPRO2007. 1 0 0 0 95241.0100 238.986000 2 1 0 49543 1451 1 0.0 0.0 0 0 0 69543 1451 2 1.00000000 30000000.0 0 0 10 79543 1451 3 120000.000 0.0 1 0 469 1159543 1451 4 95-Am-241 LANL EVAL-MAR06 Kawano,Chadwick 9543 1451 5 DIST-DEC06 9543 1451 6 ----ENDF/B-VII MATERIAL 9543 9543 1451 7 -----INCIDENT NEUTRON DATA 9543 1451 8 ------ENDF-6 FORMAT 9543 1451 9 9543 1451 10 **************************************************************** 9543 1451 11 9543 1451 12 P.Young [10/26/06] 9543 1451 13 Modified MF=13,MT=3 continuum x/s following the prescription by 9543 1451 14 H.Trellue and R.Little to correct problems in running MCNPX. Also 9543 1451 15 regridded MF=13,MT=3 summed x/s, added MF=15,MT=3 dummy spectrum 9543 1451 16 at 1.e-5 eV, and corrected gridding problems & inconsistencies 9543 1451 17 between MF=3 and MF=9. 9543 1451 18 9543 1451 19 **************************************************************** 9543 1451 20 Modification to ENDF/B-VI Rev. 2 9543 1451 21 9543 1451 22 MF=3 Neutron Cross Sections 9543 1451 23 MT=2 9543 1451 24 Adjusted to that cross sections sum to total. 9543 1451 25 MT=16,17 9543 1451 26 GNASH calclautions, and the parameters were adjusted to 9543 1451 27 reproduce the experiemtal data of Lougheed [Lo01], 9543 1451 28 Filatenkov [Fi99], and LANL C-INC data. 9543 1451 29 MT=18 9543 1451 30 The SOK code was used for evaluating the fission cross 9543 1451 31 section from 6 to 17 MeV. GNASH calculation was adopted 9543 1451 32 at high energies. 9543 1451 33 MT=102 9543 1451 34 Hauser-Feshbach statistical model calculations, and 9543 1451 35 renormalized to the experimental data of Gayther [Ga77], 9543 1451 36 and Wisshak [Wi80]. 9543 1451 37 MF=9 Multiplicities for production of radioactive elements 9543 1451 38 MT=102 9543 1451 39 Re-evaluated based on the GNASH calculation and 9543 1451 40 experimental data of Shinohara [Si97], and LANL C-INC. 9543 1451 41 9543 1451 42 Fi99 A.A. Filatenkov, RI-252, Khlopin Radium Institute (1999). 9543 1451 43 9543 1451 44 Ga77 D.B. Gayther, B.W. Thomas, Proc. 4th All Union Conf. 9543 1451 45 on Neutron Physics, Kiev, 1977, Vol.3, p.3 (1977). 9543 1451 46 9543 1451 47 Lo01 R.W. Lougheed, et al., UCRL-ID-145592, LLNL (2001). 9543 1451 48 9543 1451 49 Si97 N. Shinohara, et al., J. Nucl. Sci. Technol., 34, 7 (1997). 9543 1451 50 9543 1451 51 Wi80 K. Wisshak, F. Kaeppeler, Nucl. Sci. Eng., 76, 148 (1980). 9543 1451 52 9543 1451 53 **************************************************************** 9543 1451 54 EVALUATION OF n + 241Am REACTIONS 9543 1451 55 9543 1451 56 P. G. Young and D. G. Madland 9543 1451 57 9543 1451 58 Theoretical Division 9543 1451 59 Los Alamos National Laboratory 9543 1451 60 Los Alamos, NM 87545 9543 1451 61 February 23, 1994 9543 1451 62 9543 1451 63 I. SUMMARY 9543 1451 64 9543 1451 65 The cross section data file for neutron reactions with 241Am 9543 1451 66 has been reevaluated over the incident neutron energy range from 9543 1451 67 0.01 to 30 MeV. The evaluation is in ENDF-6 format. Details of 9543 1451 68 the analysis are given in the sections that follow. Some 9543 1451 69 general features of the work are: 9543 1451 70 9543 1451 71 1. The ENDF/B-VI n + 241Am resonance parameters were adopted at 9543 1451 72 neutron energies below 30 keV, suitably joined with the results 9543 1451 73 of the present analysis at 30 keV. 9543 1451 74 9543 1451 75 2. A coupled-channel optical model potential was developed from 9543 1451 76 analyses of nearby actinides that is consistent with 9543 1451 77 measurements of the n + 241Am neutron total cross section. This 9543 1451 78 potential was used to calculate the neutron total cross section, 9543 1451 79 elastic and inelastic scattering cross sections and angular 9543 1451 80 distributions, and reaction cross sections and transmission 9543 1451 81 coefficients for a theoretical analysis of the reaction 9543 1451 82 channels. The direct cross sections from the coupled-channel 9543 1451 83 analysis were combined with compound nucleus calculations at 9543 1451 84 lower energies and with preequilibrium theory calculations at 9543 1451 85 higher energies. Angular distributions for the first 40 excited 9543 1451 86 states of 241Am were obtained from the direct, compound-nucleus, 9543 1451 87 and preequilibrium calculations, and energy-angle correlated 9543 1451 88 distributions are provided for all continuum neutrons. 9543 1451 89 9543 1451 90 3. The evaluated fission and total cross sections were obtained 9543 1451 91 by adjusting the theoretical cross sections as needed to match 9543 1451 92 the available experimental data. 9543 1451 93 9543 1451 94 4. Nubar and the fission neutron spectra were obtained using 9543 1451 95 Madland-Nix theory. 9543 1451 96 9543 1451 97 II. THEORETICAL ANALYSIS 9543 1451 98 9543 1451 99 The primary goal of the theoretical analysis was to provide a 9543 1451 100 consistent set of data for all reactions over the energy range 9543 1451 101 30 keV to 30 MeV. In the case of n+241Am, there are reasonable 9543 1451 102 experimental data available for the neutron total and fission 9543 1451 103 cross sections. Therefore, the function of the theoretical 9543 1451 104 analysis was to provide the elastic, inelastic, (n,2n), (n,3n) 9543 1451 105 and (n,4n) cross sections, as well as the angular and energy 9543 1451 106 distributions of secondary neutrons. To accomplish this, a 9543 1451 107 theoretical analysis was performed, adjusting the relevant 9543 1451 108 parameters to match the total, fission, and (n,g) cross 9543 1451 109 sections. Additionally, a theoretical analysis was performed to 9543 1451 110 obtain the average neutron multiplicity from fission and the 9543 1451 111 energy spectra of fission neutrons as a function of incident 9543 1451 112 energy. 9543 1451 113 9543 1451 114 Coupled-channel deformed optical model calculations were 9543 1451 115 performed with the ECIS code (Ra70) over the incident neutron 9543 1451 116 energy range from 0.001 to 30 MeV. Hauser-Feshbach reaction 9543 1451 117 theory calculations were carried out with the LANL version of 9543 1451 118 the COMNUC code (Du70) at lower energies and the GNASH 9543 1451 119 statistical/preequilibrium code (Yo92) at higher energies to 9543 1451 120 obtain all partial reaction cross section data. Both reaction 9543 1451 121 theory codes used neutron transmission coefficients from the 9543 1451 122 optical model analysis. 9543 1451 123 9543 1451 124 A. Optical Model 9543 1451 125 9543 1451 126 The optical model potential was obtained by considering 9543 1451 127 several coupled-channel parameterizations developed from n + 9543 1451 128 235,238U and 239Pu experimental data (Ma78, Yo88, Yo92a). 9543 1451 129 Parameters were adjusted until a reasonable fit to experimental 9543 1451 130 data for the neutron total cross section of 241Am was obtained. 9543 1451 131 The lowest five members of the 5/2- ground state rotational band 9543 1451 132 were included in the calculations, that is, the 7/2-, 9/2-, 9543 1451 133 11/2- and 13/2- excited states at Ex = 41, 94, 159 and 235 keV 9543 1451 134 were coupled with the 5/2- ground state. 9543 1451 135 9543 1451 136 B. Reaction Theory Calculations 9543 1451 137 9543 1451 138 The Hauser-Feshbach statistical calculations were performed 9543 1451 139 with the COMNUC (Du70) and GNASH (Yo92b) codes. Both codes 9543 1451 140 include a double-humped fission barrier model, using uncoupled 9543 1451 141 oscillators for the barrier representation in GNASH and coupled 9543 1451 142 or uncoupled oscillators in COMNUC, as described by Arthur 9543 1451 143 (Ar82a). The COMNUC calculations include the possibility of 9543 1451 144 width-fluctuation corrections and corrections for class II 9543 1451 145 fluctuations (Ly74), which are needed at lower energies, whereas 9543 1451 146 GNASH provides the preequilibrium corrections that are required 9543 1451 147 at higher energies. Accordingly, COMNUC was used in the 9543 1451 148 calculations below about 2 MeV, utilizing a non-resonant model 9543 1451 149 and including class II fluctuations, and the GNASH code was 9543 1451 150 employed at higher energies using two uncoupled oscillators in 9543 1451 151 the fission calculations. 9543 1451 152 9543 1451 153 Each compound nucleus formed in the calculations is permitted 9543 1451 154 to decay through the fission channel, by neutron emission, and 9543 1451 155 by gamma-ray emission. Neutron transmission coefficients for 9543 1451 156 the Hauser-Feshbach calculations are obtained from the coupled- 9543 1451 157 channel optical model. Gamma ray transmission coefficients are 9543 1451 158 obtained from gamma-ray strength functions calculated with the 9543 1451 159 generalized Lorentzian model of Kopecky and Uhl (Ko90). 9543 1451 160 Transmission coefficients for fission are calculated from the 9543 1451 161 fission model summarized here and detailed in Yo92b. 9543 1451 162 9543 1451 163 Gilbert and Cameron (Gi70) phenomenological level density 9543 1451 164 functions were used to represent continuum levels at ground- 9543 1451 165 state deformations, appropriately matched to available 9543 1451 166 experimental structure data at lower excitation energies. 9543 1451 167 Multiplicative factors were applied to the level density 9543 1451 168 functions to account for enhancements in the fission transition 9543 1451 169 state densities at the fission barriers due to increased 9543 1451 170 asymmetry conditions, and the continuum level densities were 9543 1451 171 matched to the discrete fission transition states at each 9543 1451 172 barrier. The discrete fission transition state spectra were 9543 1451 173 calculated from bandhead information taken from calculations and 9543 1451 174 compilations by Britt (Br82) and by Nagel (Na91). 9543 1451 175 9543 1451 176 9543 1451 177 III. DESCRIPTION OF EVALUATED DATA BASE 9543 1451 178 9543 1451 179 A. Total Cross Section 9543 1451 180 9543 1451 181 The evaluated total cross section below 30 keV is obtained 9543 1451 182 from the resonance parameter evaluation in ENDF/B-VI, suitably 9543 1451 183 matched to the results of the current analysis at 30 keV. From 9543 1451 184 30 keV to 30 MeV, the coupled-channel deformed optical model 9543 1451 185 calculations described above were modified to agree with the 9543 1451 186 experimental data of Phillips (Ph70). 9543 1451 187 9543 1451 188 B. Elastic Cross Section 9543 1451 189 9543 1451 190 The elastic cross section at all energies is obtained from 9543 1451 191 the difference of the total and nonelastic cross sections. 9543 1451 192 Below 30 keV it comes from the ENDF/B-VI resonance parameters 9543 1451 193 and at higher energies it is mainly determined by the coupled- 9543 1451 194 channel optical model calculations. Angular distributions for 9543 1451 195 elastic neutrons were obtained at all energies from the coupled- 9543 1451 196 channel calculations and are given as Legendre expansions. 9543 1451 197 9543 1451 198 C. Fission Cross Section 9543 1451 199 9543 1451 200 The fission cross section was obtained by adjusting the 9543 1451 201 results of the theoretical analysis to optimize agreement with 9543 1451 202 experimental data. At most energies the adjustment was less 9543 1451 203 than a few percent. Above 8 MeV, the theoretical values were 9543 1451 204 used directly. Neutrons from fission are assumed to isotropic 9543 1451 205 in the laboratory system. 9543 1451 206 9543 1451 207 D. Radiative Capture Cross Section 9543 1451 208 9543 1451 209 The radiative capture cross section is calculated using the 9543 1451 210 generalized Lorentzian model of Ko90. The normalization of the 9543 1451 211 strength function was set by requiring the calculated (n,g) 9543 1451 212 cross section be consistent with measured values for 241Am. 9543 1451 213 9543 1451 214 E. Inelastic Neutron Cross Sections 9543 1451 215 9543 1451 216 Discrete (n,n') cross sections are included for the lowest 40 9543 1451 217 excited states of 241Am. The first, second, third, and fifth 9543 1451 218 excited states are members of the K = 5/2 ground-state 9543 1451 219 rotational band and include coupled-channel as well as compound 9543 1451 220 nucleus contributions. The remaining discrete-state cross 9543 1451 221 sections through the 40th excited state are combinations of 9543 1451 222 compound nucleus and preequilibrium contributions and were 9543 1451 223 calculated with the GNASH code. Angular distributions for all 9543 1451 224 the discrete inelastic neutrons are appropriate combinations of 9543 1451 225 the compound nucleus, direct reaction, and preequilibrium 9543 1451 226 contributions and are represented by Legendre expansions. 9543 1451 227 9543 1451 228 The inelastic data corresponding to excitation energies in 9543 1451 229 241Am above 0.508 MeV are given as energy-angle correlated 9543 1451 230 continuous spectra and were calculated with the GNASH code. The 9543 1451 231 results are given in File 6 of the ENDF/B-formatted evaluation 9543 1451 232 (ENDF-6 format) and utilize systematics by Kalbach (Ka88) for 9543 1451 233 angular distribution information, parameterized in terms of 9543 1451 234 preequilibrium ratios calculated in GNASH. 9543 1451 235 9543 1451 236 F. Cross Sections for 241Am(n,xn) Reactions 9543 1451 237 9543 1451 238 The 241Am(n,2n), (n,3n), and (n,4n) cross sections result 9543 1451 239 entirely from the theoretical analysis and GNASH calculations. 9543 1451 240 Energy-angle correlated distributions are given for all the 9543 1451 241 241Am(n,xn) reactions, making use of Kalbach's systematics 9543 1451 242 (Ka88) and the ENDF-6 File 6 representation. 9543 1451 243 9543 1451 244 G. Nubar 9543 1451 245 9543 1451 246 The evaluation of delayed nubar was carried over directly 9543 1451 247 from the ENDF/B-VI evaluation of 241Am. The prompt nubar 9543 1451 248 evaluation was obtained using Madland-Nix theory. 9543 1451 249 9543 1451 250 H. Fission Neutron Spectra 9543 1451 251 9543 1451 252 The fission neutron spectra was determined using Madland-Nix 9543 1451 253 theory and are consistent with nubar. 9543 1451 254 9543 1451 255 9543 1451 256 **************************************************************** 9543 1451 257 9543 1451 258 REFERENCES 9543 1451 259 9543 1451 260 Ar82 E. D. Arthur, "Use of the Statistical Model for the 9543 1451 261 Calculation of Compound Nucleus Contributions to Inelastic 9543 1451 262 Scattering on Actinide Nuclei," Proc. of OECD/NEA Specialists' 9543 1451 263 Meeting on Fast Neutron Scattering on Actinide Nuclei, (Paris, 9543 1451 264 November, 1981), NEANDC-158 "U" (1982) p. 145. 9543 1451 265 9543 1451 266 Ba74 B. B. Back, O. Hansen, H. C. Britt, and J. D. Garrett, 9543 1451 267 "Fission of Doubly Even Actinide Nuclei Induced by Direct 9543 1451 268 Reactions, " Phys. Rev. C 9, 1924 (1974). 9543 1451 269 9543 1451 270 Br82 H. C. Britt, personal communication, 1982. 9543 1451 271 9543 1451 272 Du70 C. L. Dunford, "A Unified Model for Analysis of Compound 9543 1451 273 Nucleus Reactions,"AI-AEC-12931, Atomics Int. (1970). 9543 1451 274 9543 1451 275 Gi65 A. Gilbert and A. G. W. Cameron, "A Composite Nuclear- 9543 1451 276 Level Density Formula with Shell Corrections," Can. J. Phys. 43, 9543 1451 277 1446 (1965). 9543 1451 278 9543 1451 279 Ka88 C. Kalbach, "Systematics of Continuum Angular 9543 1451 280 Distributions: Extensions to Higher Energies," Phys. Rev. C37, 9543 1451 281 2350 (1988); C. Kalbach and F. M. Mann, "Phenomenology of 9543 1451 282 Continuum Angular Distributions. I. Systematics and 9543 1451 283 Parameterization," Phys. Rev. C 23, 112 (1981). 9543 1451 284 9543 1451 285 Ko90 J. Kopecky and M.Uhl, "Test of Gamma-Ray Strength 9543 1451 286 Functions in Nuclear Reaction Model Calculations," Phys. Rev. C 9543 1451 287 42, 1941 (1990). 9543 1451 288 9543 1451 289 Ra70 J. Raynal, "Optical-Model and Coupled-Channel Calculations 9543 1451 290 in Nuclear Physics," IAEA SMR-9/8, Int. At. En. Agency (1970). 9543 1451 291 9543 1451 292 Yo88 P. G. Young and E. D. Arthur, "Calculation of 235U(n,n') 9543 1451 293 Cross Sections for ENDF/B-VI," Int. Conf. on Nucl. Data for 9543 1451 294 Science and Technology, Mito, Japan, May 30 - June 3, 1988 (Ed. 9543 1451 295 S. Igarasi, Saikon Publ. Co., Ltd., 1988) p. 603. 9543 1451 296 9543 1451 297 Yo92a P. G. Young and E. D. Arthur, "Theoretical Analyses of 9543 1451 298 (n,xn) Reactions on 235U, 238U, 237Np, and 239Pu for ENDF/B-VI," 9543 1451 299 Proc. Int. Conf. on Nuclear Data for Science and Technology, 9543 1451 300 Julich, Germany, 13-17 May 1991 (LA-UR-91-1424), [Ed. S. M. 9543 1451 301 Qaim, Springer-Verlag, Germany (1992)], p. 894. 9543 1451 302 9543 1451 303 Yo92b P. G. Young, E. D. Arthur, and M. B. Chadwick, 9543 1451 304 "Comprehensive Nuclear Model Calculations: Introduction to the 9543 1451 305 Theory and Use of the GNASH Code," Los Alamos National 9543 1451 306 Laboratory report LA-12343-MS (1992). 9543 1451 307 9543 1451 308 **************************************************************** 9543 1451 309 *****************************************************************9543 1451 310 9543 1451 311 THE COMMENTS BELOW PERTAIN TO THE PARTS OF THE ENDF/B-VI 9543 1451 312 EVALUATION THAT ARE UTILIZED HERE. 9543 1451 313 9543 1451 314 *****************************************************************9543 1451 315 REVISION 1 CHANGES 9543 1451 316 ENERGY RELEASE PER FISSION FROM ENDF/B-V ADDED 9543 1451 317 9543 1451 318 * * * * * * *9543 1451 319 HISTORY 9543 1451 320 THE ORIGINAL EVALUATION WAS PERFORMED BY 9543 1451 321 GU FUHUA, YU BAOSHENG, ZHOU DELIN, ZHUANG YOUXIANG 9543 1451 322 SHI XIANGJUN, YAN SHIWEI, WANG CUILAN, ZHANG JENGSHANG 9543 1451 323 UNDER THE CONTRACTS BETWEEN IAEA/NDS AND IAE,1985. 1| AND 9543 1451 324 REVISED BY 9543 1451 325 ZHOU DELIN, YU BAOSHENG, LIU TONG 9543 1451 326 SHI XIANGJUN, YAN SHIWEI 9543 1451 327 1988. 2| THE CAPTURE CROSS SECTIONS AND RESONANCE PARAMETERS 9543 1451 328 HAVE BEEN REVIEWED AND REEVALUATED BY ZHOU DELIN ET AL.1988 3|.9543 1451 329 MF=1, GENERAL INFORMATION 9543 1451 330 MT=451, COMMENTS AND DICTIONARY 9543 1451 331 MT=452, TOTAL NUMBER OF NEUTRONS PER FISSION 9543 1451 332 IT IS THE SUM OF DELAY NEUTRONS (MT=455) AND PROMPT 9543 1451 333 NEUTRONS PER FISSION (MT=456). 9543 1451 334 MT=455, T.R.ENGLAND +,LA-11151,LA-11534,LAURA-88-4118 9543 1451 335 MF=2, MT=151, RESONANCE PARAMETERS 9543 1451 336 RESOLVED RESONANCE PARAMETERS FOR SLBW FORMULA IN 1.0E-5 TO 9543 1451 337 1.5E+2 EV RESONANCE ENERGY REGION 9543 1451 338 RESOLVED PARAMETERS WERE RECOMMENDED AS FOLLOWING: 9543 1451 339 IT WAS NOTICED THAT THE PARAMETERS OF THE FIRST SEVERAL WELL 9543 1451 340 DEFINED RESONANCES (0.308, 0,576, 1.276, 1.928, 2.372, 2.358 9543 1451 341 EV, FOR EXAMPLE) GIVEN BY DERRIEN ET AL. 5| (TRANSMISSION), 9543 1451 342 KALEBIN ET AL. 6| (TRANSMISSION) AS WELL AS WESTON ET AL. 7| 9543 1451 343 (ABSORPTION, NOMALIZED TO THERMAL CAPTURE CROSS SECTION OF 582 9543 1451 344 B) RESPECTIVELY ARE IN EXCELLENT AGREEMENT WITH EACH OTHER. 9543 1451 345 THIS FACT MEANS THAT THE RESONANCE PARAMETERS FOR THE FULL 9543 1451 346 RESONANCE ENERGY REGION CAN BE COMBINED BY AVERAGING WEIGHTED 9543 1451 347 WITH RANDOM ERROR ONLY WITHOUT TAKING THE 8% SYSTEMATIC ERROR 9543 1451 348 IN ABSORPTION MEASUREMENT 7| INTO ACCOUNT. SO THAT THE 9543 1451 349 RECOMMENDED VALUES FOR MOST RESONANCES WERE AVERAGED IN EQUAL 9543 1451 350 WEIGHT EXCEPT THOSE FOR WHICH THE RANDOM ERRORS OF WESTON ET 9543 1451 351 AL.'S MEASUREMENT OR/AND THE ERRORS OF KALEBIN ET AL.'S 9543 1451 352 MEASUREMENT ARE MUCH LARGER THAN DERRIEN ET AL.'S, IN SUCH 9543 1451 353 CASES THE AVERAGE WERE MADE WITH UNEQUAL WEIGHTS PROPERLY. 9543 1451 354 UNRESOLVED RESONANCE PARAMETERS IN 1.5E+2 EV TO 30 KEV ENERGY 9543 1451 355 REGION 9543 1451 356 KIKUCH'S PARAMETERS 4| WERE USED AS INPUT DATA AND ADJUSTED 9543 1451 357 TO FIT THE CAPTURE CROSS SECTIONS (EVALUATED ON THE BASES OF 9543 1451 358 WESTON ET AL.'S, VANPRAET ET AL.'S 8|, WISSHAK ET AL.'S 9| 9543 1451 359 AND DERRIEN ET AL.'S MEASUREMENTS) AND FISSION CROSS SECTION 9543 1451 360 OF DABBS 10| (AVERAGED IN PROPER ENERGY RANGE) THEN THE 9543 1451 361 RECOMMENDED UNRESOLVED RESONANCE PARAMETERS WERE OBTAINED. 9543 1451 362 THERMAL ENERGY CROSS SECTIONS 9543 1451 363 FISSION CROSS SECTION THE VALUE OF 3.15 B WAS ADOPTED. 9543 1451 364 CAPTURE CROSS SECTION 620+-13 B, THE WEIGHTED AVERAGED VALUE 9543 1451 365 OF THE FOLLOWING DATA WAS ADOPTED: 9543 1451 366 .KALEBIN: 625+-20 (=640-3.15-11.5, TRANSMISSION); 9543 1451 367 .DOVBENKO ET AL.: 654+-104 (CAPTURE) 11|; 9543 1451 368 .HARBOUR ET AL.: 612+-25 (CAPTURE, DEDUCED RESULT TAKEN FROM 9543 1451 369 AN ANALYSIS BY STORY, 1978. QUOTTED FROM LYNN ET AL.) 12|; 9543 1451 370 .POMERANCE: 625+-35 (QUOTED FROM LYNN ET AL.) 12|; 9543 1451 371 .WISSHAK ET AL.: 625+-35 (ISOMERIC RATIO, INDIRECTLY) 13|; 9543 1451 372 .WESTON ET AL.: 582+-50 (ABSORPTION, A RELATIVE MEASUREMENT 9543 1451 373 NORMALIZED TO THERMAL CAPTURE CROSS SECTION OF 582 B. IT MAY 9543 1451 374 BE CONSIDERED TO NORMALIZE TO DERRIEN'S MEASUREMENT AT FIRST 9543 1451 375 SEVERAL RESONANCES EQUIVALENTLY. THEN THE 8% SYSTEMATIC 9543 1451 376 UNCERTAINTY IN THE ENERGY REGION OF >0.2 EV MUST BE ADDED TO 9543 1451 377 THERMAL VALUE) 3|. 9543 1451 378 MF=4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS 9543 1451 379 MT=18 ANGULAR DISTRIBUTIONS OF FISSION NEUTRONS 9543 1451 380 ASSUMED ISOTROPIC IN THE LABORATORY SYSTEM. 9543 1451 381 MF=9 9543 1451 382 MT=102 9543 1451 383 THE DATA OF ISOMERIC RATIO HAVE BEEN REVISED BASED ON THE NEW 9543 1451 384 EVALUATION 2! AND THE SHAPE OF THE THEORETICAL CALCULATION OF 9543 1451 385 13! . 9543 1451 386 MF=12,13,14,15 9543 1451 387 THE DATA CALCULATED BY R. HOWERTON (P.C.) FROM MF=2,3,5. 9543 1451 388 MF=32,33 9543 1451 389 THE FILE 32 AND 33 OF ENDF/B-V, REV.2 ARE ADOPTED. BUT THE 9543 1451 390 THE COVARIANCES OF MT=151 OF FILE 32 AND THE COVARIANCES OF 9543 1451 391 MT=18 OF FILE 33 HAVE BEEN MODIFIED PRELIMINARYLY TO MATCH 9543 1451 392 THE PRESENT EVALUATIONS. 9543 1451 393 9543 1451 394 REFERENCES 9543 1451 395 1| GU FUHUA ET AL., NEUTRON DATA EVALUATION FOR AM-241, 9543 1451 396 1985.(UNPUBLISHED). 9543 1451 397 2| THOU DELIN ET AL., NEUTRON DATA EVALUATION FOR AM-241, 9543 1451 398 1988. (UNPUBLISHED). 9543 1451 399 3| ZHOU DELIN , ON THE CAPTURE DATA EVALUATION FOR 9543 1451 400 AM-241, 1988. (TO BE PUBLISHED). 9543 1451 401 4| KIKUCH Y., JAERI-M 82-096, 1982. 9543 1451 402 5| DERRIEN H. ET AL., WASH75 P.637, 1975. 9543 1451 403 6| KALEBIN S. ET AL., A.E. 40, 373 (1976). 9543 1451 404 7| WESTON L. ET AL., NUCL. SCI. ENG., 61, 356 (1976). 9543 1451 405 8| VANPRAET . ET AL., SANTA FE(85), P.493, 1985. 9543 1451 406 9| WISSHAK K. ET AL., NUCL. SCI. ENG., 76, 148 (1980). 9543 1451 407 10| DABBS J. ET AL., NUCL. SCI. ENG., 83, 22 (1983). 9543 1451 408 11| DOVBENKO A. ET AL., LA-TR-71-74, 1971. 9543 1451 409 12| LYNN J. ET AL., PROGRESS IN NUCLEAR ENERGY, V.5, 9543 1451 410 P.255, 1980. 9543 1451 411 HARBOUR R. ET AL., NUCL. SCI. ENG., 50, 364 (1973). 9543 1451 412 POMERANCE H. ORNL-1879, P.50, 1955. 9543 1451 413 13| WISSHAK K. ET AL., NUCL. SCI. ENG., 81, 396 (1982). 9543 1451 414 **************************************************************** 9543 1451 415 ***************** Program LINEAR (VERSION 2007-1) ***************9543 1451 416 For All Data Greater than 1.0000E-10 barns in Absolute Value 9543 1451 417 Data Linearized Using Energy Dependent Uncertainty 9543 1451 418 Energy Accuracy 9543 1451 419 (eV) (per-cent) 9543 1451 420 ----------- ----------- 9543 1451 421 0.0 .010000000 9543 1451 422 1.00000000 .010000000 9543 1451 423 10.0000000 .100000000 9543 1451 424 2.00000E+9 .100000000 9543 1451 425 ***************** Program RECENT (VERSION 2007-1) ***************9543 1451 426 for All Data Greater than 1.0000E-10 barns in Absolute Value 9543 1451 427 Data Linearized Using Energy Dependent Uncertainty 9543 1451 428 Energy Accuracy 9543 1451 429 (eV) (per-cent) 9543 1451 430 ----------- ----------- 9543 1451 431 0.0 .010000000 9543 1451 432 1.00000000 .010000000 9543 1451 433 10.0000000 .100000000 9543 1451 434 2.00000E+9 .100000000 9543 1451 435 ***************** Program SIGMA1 (VERSION 2007-1) ***************9543 1451 436 Data Doppler Broadened to 1200.00000 Kelvin 9543 1451 437 for All Data Greater than 1.0000E-10 barns in Absolute Value 9543 1451 438 Data Linearized Using Energy Dependent Uncertainty 9543 1451 439 Energy Accuracy 9543 1451 440 (eV) (per-cent) 9543 1451 441 ----------- ----------- 9543 1451 442 0.0 .010000000 9543 1451 443 1.00000000 .010000000 9543 1451 444 10.0000000 .100000000 9543 1451 445 2.00000E+9 .100000000 9543 1451 446 ***************** Program SIGMA1 (VERSION 2007-1) ***************9543 1451 447 Data Doppler Broadened to 120000.000 Kelvin 9543 1451 448 for All Data Greater than 1.0000E-10 barns in Absolute Value 9543 1451 449 Data Linearized Using Energy Dependent Uncertainty 9543 1451 450 Energy Accuracy 9543 1451 451 (eV) (per-cent) 9543 1451 452 ----------- ----------- 9543 1451 453 0.0 .010000000 9543 1451 454 1.00000000 .010000000 9543 1451 455 10.0000000 .100000000 9543 1451 456 2.00000E+9 .100000000 9543 1451 457 ***************** Program FIXUP (Version 2007-1) ****************9543 1451 458 Corrected ZA/AWR in All Sections-----------------------------Yes 9543 1451 459 Corrected Thresholds-----------------------------------------No 9543 1451 460 Extended Cross Sections to 20 MeV----------------------------No 9543 1451 461 Allow Cross Section Deletion---------------------------------Yes 9543 1451 462 Allow Cross Section Reconstruction---------------------------Yes 9543 1451 463 Make All Cross Sections Non-Negative-------------------------Yes 9543 1451 464 Delete Energies Not in Ascending Order-----------------------Yes 9543 1451 465 Deleted Duplicate Points-------------------------------------Yes 9543 1451 466 Check for Ascending MAT/MF/MT Order--------------------------Yes 9543 1451 467 Check for Legal MF/MT Numbers--------------------------------Yes 9543 1451 468 Allow Creation of Missing Sections---------------------------No 9543 1451 469 Allow Insertion of Energy Points-----------------------------No 9543 1451 470 Create Uniform Energy Grid-----------------------------------No 9543 1451 471 Delete Section if Cross Section =0 at All Energies-----------Yes 9543 1451 472 **************** Program DICTIN (VERSION 2007-1) ****************9543 1451 473 1 451 588 39543 1451 474 1 452 5 49543 1451 475 1 455 7 49543 1451 476 1 456 5 49543 1451 477 1 458 5 49543 1451 478 2 151 378 49543 1451 479 3 1 751 49543 1451 480 3 2 213 49543 1451 481 3 4 92 49543 1451 482 3 16 12 49543 1451 483 3 17 10 49543 1451 484 3 18 334 49543 1451 485 3 19 334 19543 1451 486 3 19 334 19543 1451 487 3 51 69 49543 1451 488 3 52 20 49543 1451 489 3 53 22 49543 1451 490 3 54 25 49543 1451 491 3 55 21 49543 1451 492 3 56 24 49543 1451 493 3 57 25 49543 1451 494 3 58 23 49543 1451 495 3 59 23 49543 1451 496 3 60 22 49543 1451 497 3 61 22 49543 1451 498 3 62 24 49543 1451 499 3 63 23 49543 1451 500 3 64 24 49543 1451 501 3 65 20 49543 1451 502 3 66 21 49543 1451 503 3 67 22 49543 1451 504 3 68 24 49543 1451 505 3 69 22 49543 1451 506 3 70 22 49543 1451 507 3 71 22 49543 1451 508 3 72 22 49543 1451 509 3 73 22 49543 1451 510 3 74 23 49543 1451 511 3 75 21 49543 1451 512 3 76 21 49543 1451 513 3 77 21 49543 1451 514 3 78 22 49543 1451 515 3 79 22 49543 1451 516 3 80 20 49543 1451 517 3 81 20 49543 1451 518 3 82 21 49543 1451 519 3 83 20 49543 1451 520 3 84 21 49543 1451 521 3 85 20 49543 1451 522 3 86 19 49543 1451 523 3 87 18 49543 1451 524 3 88 19 49543 1451 525 3 89 20 49543 1451 526 3 90 17 49543 1451 527 3 91 18 49543 1451 528 3 102 324 49543 1451 529 4 2 107 49543 1451 530 4 18 2 49543 1451 531 4 51 105 49543 1451 532 4 52 103 49543 1451 533 4 53 101 49543 1451 534 4 54 52 49543 1451 535 4 55 101 49543 1451 536 4 56 52 49543 1451 537 4 57 52 49543 1451 538 4 58 52 49543 1451 539 4 59 52 49543 1451 540 4 60 52 49543 1451 541 4 61 50 49543 1451 542 4 62 50 49543 1451 543 4 63 50 49543 1451 544 4 64 50 49543 1451 545 4 65 50 49543 1451 546 4 66 50 49543 1451 547 4 67 50 49543 1451 548 4 68 50 49543 1451 549 4 69 48 49543 1451 550 4 70 48 49543 1451 551 4 71 48 49543 1451 552 4 72 48 49543 1451 553 4 73 48 49543 1451 554 4 74 48 49543 1451 555 4 75 48 49543 1451 556 4 76 48 49543 1451 557 4 77 48 49543 1451 558 4 78 48 49543 1451 559 4 79 48 49543 1451 560 4 80 36 49543 1451 561 4 81 36 49543 1451 562 4 82 36 49543 1451 563 4 83 36 49543 1451 564 4 84 36 49543 1451 565 4 85 36 49543 1451 566 4 86 36 49543 1451 567 4 87 36 49543 1451 568 4 88 36 49543 1451 569 4 89 36 49543 1451 570 4 90 36 49543 1451 571 5 18 25 49543 1451 572 5 455 579 49543 1451 573 6 16 687 49543 1451 574 6 17 350 49543 1451 575 6 37 104 49543 1451 576 6 91 1297 49543 1451 577 8 102 27 49543 1451 578 9 102 26 49543 1451 579 12 18 4 49543 1451 580 12 102 4 49543 1451 581 13 3 423 49543 1451 582 14 3 1 49543 1451 583 14 18 1 49543 1451 584 14 102 1 49543 1451 585 15 3 379 49543 1451 586 15 18 81 49543 1451 587 15 102 51 49543 1451 588 9543 1 0 589 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1892 12.7896831 10.8396088 13.0808128 11.5033088 13.2640674 12.04591829543 3 2 1893 13.4499075 12.6763302 14.0231590 14.8071761 14.2079581 15.42539239543 3 2 1894 14.3993047 15.9661740 14.5654508 16.3318856 14.7466000 16.60686759543 3 2 1895 15.0507585 16.7723790 15.4112242 16.5485740 15.6577503 16.20825169543 3 2 1896 17.0942309 13.6206165 17.9499847 12.3637317 18.7150350 11.47309569543 3 2 1897 19.4130480 10.8773660 19.8534939 10.5933930 20.3952607 10.32084549543 3 2 1898 20.8777650 10.1471621 21.6070490 10.0474044 21.9922915 10.09903949543 3 2 1899 22.6546887 10.3741346 24.3709520 11.5463268 25.1175325 11.81345569543 3 2 1900 25.5539784 11.8513489 26.0442199 11.8098853 27.8280263 11.40795099543 3 2 1901 28.6005983 11.3119376 29.2641321 11.2931751 30.4302030 11.31274529543 3 2 1902 31.1105653 11.2757404 32.8413312 10.9420813 33.2756940 10.90565939543 3 2 1903 33.9308034 11.0115293 34.2861818 11.1750575 34.6596598 11.43459839543 3 2 1904 35.0325683 11.7778020 36.4428766 13.4453574 36.8711440 13.88513039543 3 2 1905 37.5422480 14.3347967 38.0473476 14.4412905 38.4363233 14.39080109543 3 2 1906 39.2500583 13.9926959 41.0745279 12.5694099 41.7796377 12.09156099543 3 2 1907 42.4795871 11.7132050 43.1835879 11.4241403 44.6193977 11.05389179543 3 2 1908 45.9613514 10.9377842 46.6307429 10.9742185 47.3510954 11.08674709543 3 2 1909 49.3338865 11.6124825 50.0190701 11.7457632 50.6411512 11.79374579543 3 2 1910 52.8870059 11.6160891 53.7219992 11.7199643 54.5373165 12.04486689543 3 2 1911 56.1602164 13.0293809 56.6853169 13.2644653 57.4352027 13.39774319543 3 2 1912 58.3142415 13.2372647 59.5733177 12.7406379 60.3204978 12.59616789543 3 2 1913 60.9642797 12.7076518 61.6336228 13.1042399 62.3949539 13.86958049543 3 2 1914 63.7375737 15.5516891 64.2428102 16.0859694 64.9740244 16.58611739543 3 2 1915 65.5552966 16.7018410 66.2630001 16.5146476 67.1887784 15.87567019543 3 2 1916 68.5726053 14.6690486 69.9086456 13.7348443 71.8633257 12.81121169543 3 2 1917 73.0119816 12.3751166 74.0239711 12.0709175 75.5226086 11.84130609543 3 2 1918 76.0955892 11.8237183 78.6939293 11.9030437 82.6642686 11.80339419543 3 2 1919 87.3277134 11.9848992 88.6189480 12.1323564 90.3214763 12.53115719543 3 2 1920 93.2126120 13.6922224 94.0133659 13.9427487 95.2637252 14.09529099543 3 2 1921 96.6869644 13.9210199 98.0388477 13.6621738 98.6055229 13.61929139543 3 2 1922 99.1721982 13.6523660 99.7388734 13.7769596 100.328451 14.00877929543 3 2 1923 100.998342 14.3879858 103.259290 16.0691496 103.993681 16.52343029543 3 2 1924 105.147287 16.9461434 105.775937 17.0046357 106.479758 16.93308069543 3 2 1925 107.166025 16.7456662 108.165981 16.3268958 111.022359 14.86787129543 3 2 1926 112.345277 14.2649207 113.775518 13.7122658 115.714228 13.18612329543 3 2 1927 117.465044 13.0081711 117.570123 13.0075291 118.628542 13.06140349543 3 2 1928 122.542611 13.6317404 123.161864 13.6508141 124.071112 13.60469199543 3 2 1929 127.816220 13.0125324 128.172004 12.9991963 128.950525 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