92-U -241 ENDF/B-VII.0 Distributed by NNDC, Brookhaven Nat. Lab. 1 0 0 0 9.224100+4 2.389895+2 1 1 0 19246 1451 1 0.000000+0 1.000000+0 0 0 0 69246 1451 2 1.000000+0 3.000000+7 0 0 10 79246 1451 3 0.000000+0 0.000000+0 0 0 364 909246 1451 4 92-U -241 LANL EVAL-FEB05 P.G.Young, M.B.Chadwick 9246 1451 5 DIST-DEC06 9246 1451 6 ----ENDF/B-VII MATERIAL 9246 9246 1451 7 -----INCIDENT NEUTRON DATA 9246 1451 8 ------ENDF-6 FORMAT 9246 1451 9 9246 1451 10 **************************************************************** 9246 1451 11 9246 1451 12 MOD 1A - INCORPORATION OF REVISED DELAYED NEUTRON DATA 9246 1451 13 W. B. WILSON [2-28-05] 9246 1451 14 9246 1451 15 New DN 6-gp parameters from CINDER'90 summation calculations are 9246 1451 16 available. The CINDER calculations are based on a new CINDER 9246 1451 17 library in which beta-decay half-lives and beta-delayed neutron- 9246 1451 18 emission probablities are obtained from the evaluated experimental9246 1451 19 data file NuBase2003 (G. Audi, O. Bersillon, J. Blanchot, and 9246 1451 20 A. H. Wapstra, Nuclear Physics A729 (2003) p. 3-129), when avail- 9246 1451 21 able there. When experimental data are not available there they 9246 1451 22 are calculated in a model where allowed Gamow-Teller decays are 9246 1451 23 treated in a microscopic quasi-particle random-phase approximation9246 1451 24 (QRPA) and the first forbidden decays are treated in the statis- 9246 1451 25 tical gross theory (P. Moller, B. Pfeiffer, and K.-L. Kratz, Phys.9246 1451 26 Rev. C. 67 (2003) 055802). Further refinements are anticipated 9246 1451 27 before the final release of ENDF-7. 9246 1451 28 9246 1451 29 **************************************************************** 9246 1451 30 9246 1451 31 MOD 1 - PRELIMINARY EVALUATION OF n + 241U REACTIONS 9246 1451 32 9246 1451 33 P. G. Young and M. B. Chadwick 9246 1451 34 9246 1451 35 Theoretical Division 9246 1451 36 Los Alamos National Laboratory 9246 1451 37 Los Alamos, NM 87545 9246 1451 38 September, 2000 9246 1451 39 9246 1451 40 I. SUMMARY 9246 1451 41 9246 1451 42 The cross section data file for neutron reactions with 241U 9246 1451 43 has been evaluated over the incident neutron energy range from 9246 1451 44 10-5 eV to 30 MeV. This work utilizes results from a new 9246 1451 45 theoretical study, which includes a systematic analysis of 9246 1451 46 first-chance fission data from 232,233,234,235,236,238U + n 9246 1451 47 reactions. There are no experimental data for 241U. 9246 1451 48 9246 1451 49 Details of the present analysis are given in the sections 9246 1451 50 that follow. Some general features of the work are: 9246 1451 51 9246 1451 52 1. The ENDF/B-VI n + 237U resonance parameters were adopted for 9246 1451 53 n + 241U at neutron energies below 10 keV, as modified in the 9246 1451 54 Los Alamos 1998 evaluation of n + 237U reactions (Yo98). The 9246 1451 55 resonance analysis was suitably joined with the present analysis 9246 1451 56 at 10 keV. 9246 1451 57 9246 1451 58 2. A systematic analysis was performed of experimental fission 9246 1451 59 and radiative capture cross section data for uranium isotopes 9246 1451 60 between 232U and 238U. An isospin-dependent coupled-channel 9246 1451 61 optical model potential was developed for the uranium isotopes 9246 1451 62 and was used to calculate the n + 241U neutron total cross 9246 1451 63 section, elastic and inelastic scattering cross sections, 9246 1451 64 elastic scattering angular distributions, and reaction cross 9246 1451 65 sections. Transmission coefficients were obtained from the 9246 1451 66 optical model for theoretical calculations with reaction theory 9246 1451 67 codes. 9246 1451 68 9246 1451 69 3. Photon production data and fission neutron spectra were 9246 1451 70 taken from the existing ENDF/B-VI evaluation for n + 237U 9246 1451 71 reactions. Prompt ubar was estimated from systematics. 9246 1451 72 9246 1451 73 9246 1451 74 II. THEORETICAL ANALYSIS 9246 1451 75 9246 1451 76 The basic approach followed was to fit the available 9246 1451 77 experimental data for (n,f), (n,g), (n,xn), and other reactions 9246 1451 78 for the stable uranium isotopes using nuclear models, and to 9246 1451 79 then use reasonable extrapolations of the parameters to infer 9246 1451 80 cross sections for 241U. To perform the analysis, we utilized 9246 1451 81 the Hauser-Feshbach reaction theory code COMNUC, the Hauser- 9246 1451 82 Feshbach/preequilibrium reaction theory code GNASH, and the 9246 1451 83 coupled-channels optical model code ECIS. 9246 1451 84 9246 1451 85 A. Optical Model 9246 1451 86 9246 1451 87 The deformed optical model potential was obtained by 9246 1451 88 considering several coupled-channel parameterizations developed 9246 1451 89 from n + 235,238U and 239Pu experimental data , several of which 9246 1451 90 were used in ENDF/B-VI evaluations. The Harwell potential by 9246 1451 91 Madland and Young (Ma78), the Bruyeres-le-Chatel (BRC) potential 9246 1451 92 by Lagrange (Ha82), and a modified version of the BRC potential 9246 1451 93 by Arthur and Young (Yo88, Yo92a) were examined. Isospin 9246 1451 94 corrections were applied to all the potentials to adapt them for 9246 1451 95 the various U isotopes. Corrections from the measured to the 9246 1451 96 unmeasured cases were made in the deformation parameters b2 and 9246 1451 97 b4, using a simple model by D. Madland to calculate deformation 9246 1451 98 parameters for targets without experimental information from 9246 1451 99 deformations given in the extensive Nix-Moller mass analysis. 9246 1451 100 For the optical model potential, we chose to use an isospin 9246 1451 101 version of the BRC potential (Ha82), which was inferred from 9246 1451 102 Lagrange's results for individual nuclides. The lowest three 9246 1451 103 members of the 7/2+ ground state rotational band were included 9246 1451 104 in the calculations, that is, the 9/2+ and 11/2+ states at Ex = 9246 1451 105 56 and 123 keV were coupled with the 7/2+ ground state. All of 9246 1451 106 the potentials considered gave total and reaction cross sections 9246 1451 107 that were reasonably consistent, so the selection was based 9246 1451 108 mainly on the fact that the BRC potential gave better agreement 9246 1451 109 with fission cross sections for odd U isotopes (233,235U) at 9246 1451 110 lower energies. 9246 1451 111 9246 1451 112 B. Reaction Theory Calculations 9246 1451 113 9246 1451 114 The Hauser-Feshbach statistical calculations were performed 9246 1451 115 with the COMNUC (Du70) and GNASH (Yo92b) codes. Both codes 9246 1451 116 include a double-humped fission barrier model, using uncoupled 9246 1451 117 oscillators for the barrier representation in GNASH and coupled 9246 1451 118 or uncoupled oscillators in COMNUC, as described by Arthur 9246 1451 119 (Ar82a). The COMNUC calculations include the possibility of 9246 1451 120 width-fluctuation corrections and corrections for class II 9246 1451 121 fluctuations, which are needed at lower energies, whereas GNASH 9246 1451 122 provides the preequilibrium corrections that are required at 9246 1451 123 higher energies. Accordingly, COMNUC was used in the 9246 1451 124 calculations below about 0.5 MeV, utilizing a non-resonant model 9246 1451 125 and including class II fluctuations, and the GNASH code was 9246 1451 126 employed at higher energies using two uncoupled oscillators in 9246 1451 127 the fission calculations. 9246 1451 128 Each compound nucleus formed in the calculations is permitted 9246 1451 129 to decay through the fission channel, by neutron emission, and 9246 1451 130 by gamma-ray emission. Neutron transmission coefficients for 9246 1451 131 the Hauser-Feshbach calculations are obtained from the coupled- 9246 1451 132 channel optical model. Gamma ray transmission coefficients are 9246 1451 133 obtained from gamma-ray strength functions calculated with the 9246 1451 134 generalized Lorentzian model of Kopecky and Uhl (Ko90). 9246 1451 135 Transmission coefficients for fission are calculated from the 9246 1451 136 fission model summarized here and detailed in Yo92b. 9246 1451 137 Gilbert and Cameron (Gi70) phenomenological level density 9246 1451 138 functions were used to represent continuum levels at ground- 9246 1451 139 state deformations, appropriately matched to available 9246 1451 140 experimental structure data at lower excitation energies. 9246 1451 141 Multiplicative factors were applied to the level density 9246 1451 142 functions to account for enhancements in the fission transition 9246 1451 143 state densities at the fission barriers due to increased 9246 1451 144 asymmetry conditions, and the continuum level densities were 9246 1451 145 matched to the discrete fission transition states at each 9246 1451 146 barrier. The discrete fission transition state spectra were 9246 1451 147 calculated from bandhead information taken from calculations and 9246 1451 148 compilations by Britt (Br82). 9246 1451 149 Initial values of fission barrier parameters were taken from 9246 1451 150 the work of Britt (Br82,Ba74), and we used default level density 9246 1451 151 parameters of Gilbert and Cameron for all ground state nuclei. 9246 1451 152 We only modified the Britt-Back parameters in very simple ways 9246 1451 153 in order to facilitate extrapolation of the parameters. Our 9246 1451 154 modifications were limited to minor adjustments of the fission 9246 1451 155 barrier heights, the pairing energy at the fission barriers 9246 1451 156 (although we usually used the Gilbert-Cameron values), and the 9246 1451 157 level matching of the temperature region of the continuum level 9246 1451 158 densities at the fission saddles. 9246 1451 159 We fit the experimental (n,f) and (n,g) cross sections for 9246 1451 160 all stable isotopes over the energy region of first-chance 9246 1451 161 fission using the COMNUC model code. Experimental data exists 9246 1451 162 for targets of 232U, 233U, 234U, 235U, 236U, and 238U, which 9246 1451 163 allowed us to infer fission barrier parameters and gamma-ray 9246 1451 164 strength functions for the compound systems of 233U, 234U, 235U, 9246 1451 165 236U, 237U, and 239U. Using the parameters determined from the 9246 1451 166 first-chance fission fitting without modification, we performed 9246 1451 167 GNASH calculations over the entire energy region of each target 9246 1451 168 nucleus. We carried the calculations to 30 MeV, which involve 9246 1451 169 first-, second-, third-, fourth-, and fifth-chance fission 9246 1451 170 processes. These comparisons provide a necessary test of the 9246 1451 171 reliability of our calculations, in that no adjustments are made 9246 1451 172 past the first-chance fission results. 9246 1451 173 9246 1451 174 III. DESCRIPTION OF EVALUATED DATA BASE 9246 1451 175 9246 1451 176 A. Total Cross Section 9246 1451 177 9246 1451 178 The evaluated total cross section below 10 keV is obtained 9246 1451 179 from the n + 237U resonance parameter evaluation in ENDF/B-VI, 9246 1451 180 as modified in a recent Los Alamos evaluation (Yo98). From 10 9246 1451 181 keV to 30 MeV, the coupled-channel deformed optical model 9246 1451 182 calculations described above are used directly. 9246 1451 183 9246 1451 184 B. Elastic Cross Section 9246 1451 185 9246 1451 186 The elastic cross section at all energies is obtained from 9246 1451 187 the difference of the total and nonelastic cross sections. Below 9246 1451 188 10 keV it comes from the resonance parameters and at higher 9246 1451 189 energies it is determined by the coupled-channel optical model 9246 1451 190 calculations. Angular distributions for elastic neutrons were 9246 1451 191 obtained at all energies from the ECIS coupled-channel 9246 1451 192 calculations combined with the COMNUC compound-elastic 9246 1451 193 calculations (see above) and are given as Legendre expansions. 9246 1451 194 9246 1451 195 C. Fission Cross Section 9246 1451 196 9246 1451 197 The fission cross section is calculated from the resonance 9246 1451 198 parameters below 10 keV, as described earlier. At higher 9246 1451 199 energies the fission cross section is based on the theoretical 9246 1451 200 analysis described above. 9246 1451 201 9246 1451 202 D. Radiative Capture Cross Section 9246 1451 203 9246 1451 204 Below 10 keV, the capture cross section is based on the 9246 1451 205 resonance parameters. At higher energies the cross section is 9246 1451 206 calculated using the generalized Lorentzian model of Ko90. The 9246 1451 207 normalization of the strength function was set by requiring the 9246 1451 208 calculated (n,g) cross section be consistent with measured 9246 1451 209 values for 235U, similar to our n + 237U evaluation 9246 1451 210 9246 1451 211 E. Inelastic Neutron Cross Sections 9246 1451 212 9246 1451 213 Discrete (n,n') cross sections are included for the lowest 2 9246 1451 214 rotational levels of 241U (MT=51,52)and for 25 (representative) 9246 1451 215 collective levels (MT=53-77). Because the structure of 241U is 9246 1451 216 unknown, the rotational states were estimated from a rotational 9246 1451 217 model. The two excited states are members of the K = 7/2 ground- 9246 1451 218 state rotational band; the cross sections and angular 9246 1451 219 distributions include direct components from the ECIS 9246 1451 220 calculations as well as compound nucleus contributions from the 9246 1451 221 COMNUC calculations. The other collective levels (MT=53-78) are 9246 1451 222 based on calculations for 235U (MT=53-58) and 238U (MT=59-77), 9246 1451 223 with the assumption that similar states exist for 241U. The 9246 1451 224 angular distributions of all excited levels are represented by 9246 1451 225 Legendre expansions. 9246 1451 226 The (n,n'continuum) inelastic data (resulting from compound 9246 1451 227 nucleus and preequilibrium reactions at excitation energies in 9246 1451 228 241U above 0.123 MeV) are given as energy-angle correlated 9246 1451 229 continuous spectra and were calculated with the GNASH code. The 9246 1451 230 results are given in File 6 of the ENDF/B-formatted evaluation 9246 1451 231 (ENDF-6 format) and utilize systematics by Kalbach (Ka88) for 9246 1451 232 angular distribution information, parameterized in terms of 9246 1451 233 preequilibrium ratios calculated in GNASH. 9246 1451 234 9246 1451 235 F. Cross Sections for 241U(n,xn) Reactions 9246 1451 236 9246 1451 237 The 241U(n,2n), (n,3n), and (n,4n) cross sections result 9246 1451 238 entirely from the theoretical analysis and GNASH calculations. 9246 1451 239 Energy-angle correlated distributions are given for all the 9246 1451 240 241U(n,xn) reactions, making use of Kalbach's systematics (Ka88) 9246 1451 241 and the ENDF/B-6 File 6 representation. 9246 1451 242 9246 1451 243 G. Nubar 9246 1451 244 9246 1451 245 The evaluation of delayed nubar were carried over directly 9246 1451 246 from the ENDF/B-VI evaluation of 237U. The prompt nubar 9246 1451 247 evaluation is based on the systematics of Manero and Konshin 9246 1451 248 (Ma72), updated using experimental values for targets of 235U 9246 1451 249 and 238U . 9246 1451 250 9246 1451 251 H. Fission Neutron Spectra 9246 1451 252 9246 1451 253 The fission neutron spectra in the revised evaluation is 9246 1451 254 carried over directly from the 237U evaluation in ENDF/B-VI. A 9246 1451 255 maxwellian representation is used for the spectrum shape, with 9246 1451 256 energy-dependent temperature parameters based on systematics. 9246 1451 257 9246 1451 258 9246 1451 259 IV. CONCLUSIONS 9246 1451 260 9246 1451 261 The new analysis of n + 241U nuclear data should provide an 9246 1451 262 approximate representation of most reactions over the incident 9246 1451 263 energy range 10 keV to 30 MeV. This evaluation is regarded as 9246 1451 264 preliminary until some of our assumptions concerning structure 9246 1451 265 and fission barriers can be better assessed. Theoretical 9246 1451 266 estimates of the structure of 241U are needed. Also, further 9246 1451 267 work is needed to obtain better theoretical estimates of all the 9246 1451 268 cross sections but particularly fission. Additionally, 9246 1451 269 improvements to the evaluations of nubar and the fission neutron 9246 1451 270 spectra using the Madland-Nix approach will be considered in the 9246 1451 271 future. 9246 1451 272 9246 1451 273 **************************************************************** 9246 1451 274 9246 1451 275 REFERENCES 9246 1451 276 9246 1451 277 Ar82. E. D. Arthur, "Use of the Statistical Model for the 9246 1451 278 Calculation of Compound Nucleus Contributions to Inelastic 9246 1451 279 Scattering on Actinide Nuclei," Proc. of OECD/NEA Specialists' 9246 1451 280 Meeting on Fast Neutron Scattering on Actinide Nuclei, (Paris, 9246 1451 281 November, 1981), NEANDC-158 "U" (1982) p. 145. 9246 1451 282 9246 1451 283 Ba74 B. B. Back, O. Hansen, H. C. Britt, and J. D. Garrett, 9246 1451 284 "Fission of Doubly Even Actinide Nuclei Induced by Direct 9246 1451 285 Reactions, " Phys. Rev. C 9, 1924 (1974). 9246 1451 286 9246 1451 287 Br82 H. C. Britt, personal communication, 1982. 9246 1451 288 9246 1451 289 Du70 C. L. Dunford, "A Unified Model for Analysis of Compound 9246 1451 290 Nucleus Reactions,"AI-AEC-12931, Atomics Int. (1970). 9246 1451 291 9246 1451 292 Gi65 A. Gilbert and A. G. W. Cameron, "A Composite Nuclear- 9246 1451 293 Level Density Formula with Shell Corrections," Can. J. Phys. 43, 9246 1451 294 1446 (1965). 9246 1451 295 9246 1451 296 Ha82 G. Haouat, J. Lachkar, Ch. Lagrange, J. Jary, J. Sigaud, 9246 1451 297 and Y. Patin, "Neutron Scattering Cross Sections for 232Th, 9246 1451 298 233U, 235U, 238U, 239Pu, and 242Pu Between 0.6 and 3.4 MeV," 9246 1451 299 Nucl. Sci. and Engr. 81, 491 (1982). 9246 1451 300 9246 1451 301 Ka88 C. Kalbach, "Systematics of Continuum Angular 9246 1451 302 Distributions: Extensions to Higher Energies," Phys. Rev. C37, 9246 1451 303 2350 (1988); C. Kalbach and F. M. Mann, "Phenomenology of 9246 1451 304 Continuum Angular Distributions. I. Systematics and 9246 1451 305 Parameterization," Phys. Rev. C 23, 112 (1981). 9246 1451 306 9246 1451 307 Ko90 J. Kopecky and M.Uhl, "Test of Gamma-Ray Strength 9246 1451 308 Functions in Nuclear Reaction Model Calculations," Phys. Rev. C 9246 1451 309 42, 1941 (1990). 9246 1451 310 9246 1451 311 Ma72 F. Manero and V. A. Konshin, At. En. Rev. 10, 637 (1972). 9246 1451 312 9246 1451 313 Ma78 D. G. Madland and P. G. Young, "Neutron-Nucleus Optical 9246 1451 314 Potential for the Actinide Region," Proc. Int. Conf. on Neutron 9246 1451 315 Physics and Nuclear Data for Reactors and Other Applied 9246 1451 316 Purposes, Harwell, England (pub. by OECD), p. 349 (1978). 9246 1451 317 9246 1451 318 Mc74 J. H. McNally, J. W. Barnes, B. J. Dropesky, P. A. Seeger 9246 1451 319 and K. Wolfsberg, "Neutron-Induced Fission Cross Section of 9246 1451 320 237U," Phys. Rev. C 9, 717 (1974). 9246 1451 321 9246 1451 322 Mo95 P. Moller, J. R. Nix, W. D. Myers, and W. J. Swiatecki, 9246 1451 323 "Ground-State Masses and Deformations," Atomic Data Nucl. Data 9246 1451 324 Tables 59 (1995),1. 9246 1451 325 9246 1451 326 Ra70 J. Raynal, "Optical-Model and Coupled-Channel Calculations 9246 1451 327 in Nuclear Physics," IAEA SMR-9/8, Int. At. En. Agency (1970). 9246 1451 328 9246 1451 329 Yo88 P. G. Young and E. D. Arthur, "Calculation of 235U(n,n') 9246 1451 330 Cross Sections for ENDF/B-VI," Int. Conf. on Nucl. Data for 9246 1451 331 Science and Technology, Mito, Japan, May 30 - June 3, 1988 (Ed. 9246 1451 332 S. Igarasi, Saikon Publ. Co., Ltd., 1988) p. 603. 9246 1451 333 9246 1451 334 Yo92a P. G. Young and E. D. Arthur, "Theoretical Analyses of 9246 1451 335 (n,xn) Reactions on 235U, 238U, 237Np, and 239Pu for ENDF/B-VI," 9246 1451 336 Proc. Int. Conf. on Nu-clear Data for Science and Technology, 9246 1451 337 Julich, Germany, 13-17 May 1991 (LA-UR-91-1424), [Ed. S. M. 9246 1451 338 Qaim, Springer-Verlag, Germany (1992)], p. 894. 9246 1451 339 9246 1451 340 Yo92b P. G. Young, E. D. Arthur, and M. B. Chadwick, 9246 1451 341 "Comprehensive Nuclear Model Calculations: Introduction to the 9246 1451 342 Theory and Use of the GNASH Code," Los Alamos National 9246 1451 343 Laboratory report LA-12343-MS (1992). 9246 1451 344 9246 1451 345 Yo94 P. G. Young, "Preliminary Evaluation of n + 237U 9246 1451 346 Reactions," Los Alamos National Laboratory internal memo #T-2: 9246 1451 347 M-3669 (P. G. Young to R. C. Little, 3 February 1994). 9246 1451 348 9246 1451 349 Yo98 P. G. Young, "Preliminary Evaluation of n + 237U 9246 1451 350 Reactions," October, 1998. 9246 1451 351 9246 1451 352 **************************************************************** 9246 1451 353 Note that MF=12,13,14,15 were taken over directly from the 237U 9246 1451 354 ENDF/B-VI eval. Gamma production data are taken from an LLNL 9246 1451 355 evaluation. 9246 1451 356 **************************************************************** 9246 1451 357 9246 1451 358 M-3669 (P. G. Young to R. C. Little, 3 February 1994). 9246 1451 359 9246 1451 360 Yo98 P. G. Young, "Preliminary Evaluation of n + 237U 9246 1451 361 Reactions," October, 1998. 9246 1451 362 9246 1451 363 ******************************************************************9246 1451 364 Note that MF=12,13,14,15 were taken over directly from the 237U 9246 1451 365 ENDF/B-VI eval.Gamma production data are from an LLNL evaluation.9246 1451 366 ******************************************************************9246 1451 367 9246 1451 368 1 451 458 19246 1451 369 1 452 5 09246 1451 370 1 455 7 19246 1451 371 1 456 5 09246 1451 372 2 151 46 09246 1451 373 3 1 60 19246 1451 374 3 2 49 19246 1451 375 3 3 60 19246 1451 376 3 4 43 19246 1451 377 3 16 18 19246 1451 378 3 17 14 19246 1451 379 3 18 52 19246 1451 380 3 37 10 19246 1451 381 3 51 43 19246 1451 382 3 52 39 19246 1451 383 3 53 33 19246 1451 384 3 54 31 19246 1451 385 3 55 31 19246 1451 386 3 56 30 19246 1451 387 3 57 29 19246 1451 388 3 58 28 19246 1451 389 3 59 28 19246 1451 390 3 60 27 19246 1451 391 3 61 27 19246 1451 392 3 62 26 19246 1451 393 3 63 25 19246 1451 394 3 64 25 19246 1451 395 3 65 24 19246 1451 396 3 66 24 19246 1451 397 3 67 23 19246 1451 398 3 68 23 19246 1451 399 3 69 22 19246 1451 400 3 70 22 19246 1451 401 3 71 21 19246 1451 402 3 72 21 19246 1451 403 3 73 20 19246 1451 404 3 74 20 19246 1451 405 3 75 20 19246 1451 406 3 76 19 19246 1451 407 3 77 19 19246 1451 408 3 91 39 19246 1451 409 3 102 52 19246 1451 410 4 2 149 19246 1451 411 4 18 2 19246 1451 412 4 51 131 19246 1451 413 4 52 127 19246 1451 414 4 53 74 19246 1451 415 4 54 74 19246 1451 416 4 55 74 19246 1451 417 4 56 74 19246 1451 418 4 57 71 19246 1451 419 4 58 74 19246 1451 420 4 59 97 19246 1451 421 4 60 97 19246 1451 422 4 61 94 19246 1451 423 4 62 94 19246 1451 424 4 63 93 19246 1451 425 4 64 93 19246 1451 426 4 65 90 19246 1451 427 4 66 89 19246 1451 428 4 67 89 19246 1451 429 4 68 85 19246 1451 430 4 69 85 19246 1451 431 4 70 81 19246 1451 432 4 71 80 19246 1451 433 4 72 77 19246 1451 434 4 73 77 19246 1451 435 4 74 77 19246 1451 436 4 75 77 19246 1451 437 4 76 77 19246 1451 438 4 77 74 19246 1451 439 5 18 9 19246 1451 440 5 455 589 19246 1451 441 6 16 1566 19246 1451 442 6 17 849 19246 1451 443 6 37 453 19246 1451 444 6 91 2416 19246 1451 445 8 16 2 19246 1451 446 8 17 2 19246 1451 447 8 37 2 19246 1451 448 8 102 2 19246 1451 449 12 18 4 19246 1451 450 12 102 4 19246 1451 451 13 3 10 19246 1451 452 14 3 1 19246 1451 453 14 18 1 19246 1451 454 14 102 1 19246 1451 455 15 3 370 19246 1451 456 15 18 32 19246 1451 457 15 102 70 19246 1451 458 0.000000+0 0.000000+0 0 0 0 09246 1 099999 9.224100+4 2.389895+2 0 2 0 09246 1452 0 0.000000+0 0.000000+0 0 0 1 49246 1452 1 4 2 9246 1452 2 1.000000-5 2.234260+0 4.000000+6 2.917460+0 7.000000+6 3.415876+09246 1452 3 3.000000+7 7.344276+0 9246 1452 4 0.000000+0 0.000000+0 0 0 0 09246 1 099999 9.224100+4 2.389895+2 0 2 0 09246 1455 0 0.000000+0 0.000000+0 0 0 6 09246 1455 1 1.249577-2 3.037978-2 1.068975-1 3.240317-1 1.334253+0 9.544175+09246 1455 2 0.000000+0 0.000000+0 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