IAEA-NDS ENDF Download System, v-2008-07-22 0 0 0 0 6.31540+ 4 1.52601+ 2 1 0 0 40 777 1451 1 0.00000+ 0 0.00000+ 0 0 0 171 0 777 1451 2 63-EU-154 BNL EVAL-DEC73 H.TAKAHASHI 777 1451 3 DIST-DEC74 REV-JUN75 777 1451 4 THIS MATERIAL CONTAINS THE EVALUATED RESULTS FOR THE NEUTRON 777 1451 5 CROSS SECTION FOR EUROPIUM ISOTOPES OF EU-154. NO EXPERIMENTAL 777 1451 6 DATA ARE AVAILABLE FOR THESE ISOTOPES EXCEPT FEW REACTIONS, SO 777 1451 7 THAT THE EVALUATIONS WERE MOSTLY CARRIED OUT BY NUCLEAR MODEL 777 1451 8 CALCULATIONS. 777 1451 9 * * * * * * 777 1451 10 MF=1,MT=457 RADIOACTIVE DECAY DATA SECTION EVALUATED BY 777 1451 11 R.SCHENTER (HEDL) FOR ENDF/B-IV FISS.PROD. FILE 777 1451 12 REFERENCES 777 1451 13 QBETA -A TOBIAS(10/72) RD/B/M2453 777 1451 14 EBETA-A TOBIAS(10/72) RD/B/M2453 777 1451 15 EGAMMA-A TOBIAS(10/72) RD/B/M2453 777 1451 16 HALF LIFE-N HOLDEN ET AL CHART OF NUCLIDES(1973) 777 1451 17 BRANCHING PROBABILITIES-MEEK AND RIDER(1974),NEDO-12154 777 1451 18 AWR- G GARVEY ET AL RMP41,NO4(1969) 777 1451 19 * * * * * * 777 1451 20 3. FILE 2 RESONANCE PARAMETERS 777 1451 21 3.1 RESOLVED RESONANCES 777 1451 22 THE RESOLVED RESONANCE PARAMETERS WERE MADE BY TAKING INTO 777 1451 23 ACCOUNT THEIR STATISTICAL PROPERTIES FOR LEVEL SPACING AND 777 1451 24 REDUCED NEUTRON WIDTH FLUCTUATION. THE METHOD USED IN THIS 777 1451 25 CALCULATION WAS SIMILAR TO THE PROCEDURE USED BY COOK. (1) 777 1451 26 HOWEVER, INSTEAD OF USING THE MONTE CARLO CALCULATION, THE 777 1451 27 LEVEL SPACING AND THE REDUCED NEUTRON WIDTH FLUCTUATION ARE 777 1451 28 DETERMINED BY USING THE STATISTICAL PROPERTIES OF EU-153. 777 1451 29 THE AVERAGE VALUES OF THESE QUANTITIES ARE DETERMINED IN THE 777 1451 30 SIMILAR WAY AS THE PROCEDURE OF BARR ET AL. (2) THAT IS, THE 777 1451 31 RATIOS OF THE AVERAGE VALUES FOR ODD EVEN NUCLEI TO THOSE FOR 777 1451 32 ODD-ODD NUCLEI WERE ESTIMATED FROM THEIR NEIGHBORING NUCLEI. 777 1451 33 THESE RATIOS WERE MULTIPLIED TO THE VALUES OF EU-153 TO OBTAIN 777 1451 34 THE ONES FOR EU-154. THE GAMMA RAY WIDTH WERE TAKEN AS 777 1451 35 CONSTANT VALUES FOR ALL RESONANCES. 777 1451 36 THE 96 RESONANCES WERE ASSIGNED BETWEEN 0.01EV AND 59.732EV. 777 1451 37 THERMAL NEUTRON CAPTURE CROSS SECTION HAD BEEN MEASURED BY 777 1451 38 HAYDEN ET AL. (3) AND WALKER (4). THE PRELIMINARY DRAFT OF NEW 777 1451 39 BNL-325 IS RECOMMENDING THOSE VALUES AS 1500 +/- 400 BARN FOR 777 1451 40 EU-154 (8 YEAR). THE PARAMETERS OF THE LOWEST RESONANCES WERE 777 1451 41 ADJUSTED SO THAT THE CALCULATED THERMAL NEUTRON CAPTURE 777 1451 42 CROSS SECTIONS AGREE WITH THE VALUES RECOMMENDED IN THE NEW 777 1451 43 BNL-325. (5) 777 1451 44 3.2 UNRESOLVED RESONANCES 777 1451 45 UNRESOLVED RESONANCE PARAMETERS WERE GIVEN THE ENERGY REGIONS 777 1451 46 FROM 60.0 EV TO 10 KEV. AS MENTIONED ABOVE, BARR AND DEVANEY (2) 777 1451 47 EVALUATED THE UNRESOLVED RESONANCE PARAMETERS BY STUDYING THE 777 1451 48 CHANGE OF THESE PARAMETERS FROM ODD-ODD NUCLEI TO ODD-EVEN 777 1451 49 NUCLEI OF LU-175, LU-176, AND TA-180, TA-181. THE UNRESOLVED 777 1451 50 RESONANCE PARAMETERS WERE ESTIMATED BY USING THE NEW BNL-325 777 1451 51 VALUES. 777 1451 52 4. FILE 3 (NEUTRON CROSS SECTION) 777 1451 53 4.1 TOTAL CROSS SECTION (MT = 1) 777 1451 54 BETWEEN 10000 EV TO 2.5 MEV NEUTRON ENERGY, THE TOTAL CROSS 777 1451 55 SECTIONS WERE CALCULATED USING THE ABACUS-2 CODE (6) OF THE 777 1451 56 OPTICAL MODEL. THE OPTICAL PARAMETERS USED IN THE CALCULATION 777 1451 57 WILL BE SHOWN IN THE LATER SECTION. ABOVE 2.5 MEV, THE TOTAL 777 1451 58 CROSS SECTIONS WERE ASSUMED TO BE THE SAME AS THE EXPERIMENTAL 777 1451 59 VALUES OF NATURAL EUROPIUM MEASURED BY FOSTER. (7) 777 1451 60 4.2 ELASTIC SCATTERING CROSS SECTION (MT = 2) 777 1451 61 THE ELASTIC SCATTERING CROSS SECTIONS IN THE ENERGY HIGHER 777 1451 62 THAN THE UNRESOLVED RESONANCE ENERGY WERE OBTAINED BY 777 1451 63 SUBSTRUCTING THE NON ELASTIC CROSS SECTION FROM THE EVALUATED 777 1451 64 TOTAL CROSS SECTION. 777 1451 65 4.3 NONELASTIC SCATTERING CROSS SECTION (MT = 3) 777 1451 66 THE NONELASTIC SCATTERING CROSS SECTION WAS CALCULATED BY 777 1451 67 SUMMING UP ALL CROSS SECTIONS EXCEPT THE ELASTIC SCATTERING 777 1451 68 CROSS SECTION. 777 1451 69 4.4 INELASTIC SCATTERING CROSS SECTION (MT=4,51,52...,91) 777 1451 70 THE INELASTIC SCATTERING CROSS SECTIONS WERE GIVEN AS TOTAL 777 1451 71 (MT = 4), DISCRETE LEVEL EXCITATION CROSS SECTION (MT=51...) FOR 777 1451 72 THE FIRST 5 LEVELS AND CONTINUUM LEVEL EXCITATION CROSS SECTION 777 1451 73 (MT = 91). THE LEVEL SCHEME FOR THESE DISCRETE LEVEL IS TAKEN 777 1451 74 FROM REF. (9,10,11,12,13). 777 1451 75 SINCE NO EXPERIMENTAL DATA ARE AVAILABLE FOR THE INDIVIDUAL 777 1451 76 LEVEL EXCITATION CROSS SECTIONS, THEY WERE CALCULATED USING THE 777 1451 77 COMNUC-3 CODE (14,15) FOR ENERGIES UP TO 3 MEV. ABOVE 3 MEV, 777 1451 78 NEUTRON ENERGY, INELASTIC SCATTERING IS MOSTLY THE EXCITATION OF 777 1451 79 THE CONTINUUM OF LEVELS, SO THAT THE INELASTIC SCATTERING CROSS 777 1451 80 SECTION FOR DISCRETE LEVEL EXCITATION ABOVE THIS ENERGY WAS 777 1451 81 NEGLECTED AND THE INELASTIC SCATTERING CROSS SECTION FOR 777 1451 82 CONTINUUM LEVEL EXCITATION WAS CALCULATED BY THE CASCADE 777 1451 83 CALCULATION OF GROGI-3 CODE. (16) THE LEVEL DENSITY PARAMETERS 777 1451 84 FOR THE CONTINUUM OF LEVELS WERE TAKEN FROM COOK S DATA (18) FOR 777 1451 85 THE DEFORMED NUCLEI USING THE GILBERT-CAMERON FORMULA. (19) 777 1451 86 4.5 (N,P) AND (N,N ,P) CROSS SECTION (MT = 103, 28) 777 1451 87 NO EXPERIMENTAL VALUES WERE AVAILABLE, SO THAT WE CALCULATED 777 1451 88 THESE BY NUCLEAR MODEL CODES. FOR (N,P) REACTION, THE SEMI- 777 1451 89 EMPIRICAL STATISTICAL MODEL CODE THRESH (21) WAS USED. BUT THE 777 1451 90 EVALUATION (7) OF EU-151 AND EU-153 INDICATED THAT THE CROSS- 777 1451 91 SECTIONS AROUND 14 MEV CALCULATED BY THIS CODE WERE SMALL 777 1451 92 COMPARED TO THE EXPERIMENTAL VALUES. THUS, THE CALCULATED CROSS 777 1451 93 SECTIONS WERE NORMALIZED BY THE FACTORS OBTAINED FOR EU-151. 777 1451 94 THE (N,N P) CROSS SECTIONS WERE CALCULATED BY USING GROGI-3. 777 1451 95 4.6 (N,ALPHA) AND (N,N D) CROSS SECTION (MT = 107,22) 777 1451 96 THESE CROSS SECTIONS WERE OBTAINED IN THE SINILAR MANNER AS THE 777 1451 97 CASES OF (N,P) AND (N,N P) REACTIONS. 777 1451 98 4.7 (N,2N), (N,3N) CROSS SECTION (MT = 16, 17) 777 1451 99 THESE CROSS SECTIONS WERE CALCULATED BY USING THE GROGI-3 CODE. 777 1451 100 THE OPTICAL MODEL PARAMETERS DESCRIBED IN THE LATER SECTION WERE 777 1451 101 USED. 777 1451 102 4.8 (N,D),(N,T),AND(N,HE-3) REACTION CROSS SECTION (MT=104,105, 777 1451 103 AND 107) 777 1451 104 THE CROSS SECTIONS CALCULATED BY THRESH WERE ADAPTED AS THE 777 1451 105 EVALUATED CROSS SECTIONS. 777 1451 106 4.9 THE RADIATIVE CAPTURE CROSS SECTION (MT = 102) 777 1451 107 THE RADIATIVE CAPTURE CROSS SECTIONS AT LOW ENERGY RANGE WERE 777 1451 108 CALCULATED FROM THE RESONANCE PARAMETERS DISCUSSED IN THE SECTION 777 1451 109 OF FILE 2 AND ARE PRESENTED AS THE SMOOTH CROSS SECTIONS. THE 777 1451 110 CROSS SECTIONS BETWEEN 100 EV AND 10 KEV ARE PRESENTED AS THE 777 1451 111 UNRESOLVED RESONANCE PARAMETERS. 777 1451 112 FOR ENERGY HIGHER THAN 10 KEV, THE CROSS SECTIONS WERE EVALUATED 777 1451 113 BY THE COMNUC-3 CALCULATION. THE CALCULATION WAS DONE SIMILARLY 777 1451 114 TO THE ONES FOR EU-151 AND EU-153 (7). THAT IS, WE ASSUMED 777 1451 115 MOLDAUER S Q VALUE TO BE ZERO, AND THE CORRELATION CORRECTION 777 1451 116 FACTOR DUE TO THE DEGREE OF FREEDOM ASSOCIATED WITH OPEN CHANNEL 777 1451 117 WAS TAKEN INTO ACCOUNT IN THE CALCULATION. FROM 3 MEV TO 20 MEV, 777 1451 118 THE CAPTURE CROSS SECTION WAS OBTAINED BY GROGI-3 FOR COMPOUND 777 1451 119 PROCESS, BY THE CVELBAR S FORMULA (22) BASED ON LANE-LYNN (23) 777 1451 120 AND BROWN S (24) FORMULA FOR THE DIRECT AND SEMI-DIRECT 777 1451 121 REACTION. 777 1451 122 5. FILE 4 (ANGULAR DISTRIBUTION OF SECONDARY NEUTRONS) 777 1451 123 5.1 ELASTIC SCATTERING (MT = 2) 777 1451 124 THESE WERE CALCULATED BY ABACUS-2 (NABAK PDP-10 VERSION) (6) AND 777 1451 125 THE LEGENDRE COEFFICIENTS CALCULATED BY CHAD (NUCHAD IN PDP-10 777 1451 126 VERSION) (25) WERE GIVEN. SINCE THE ELASTIC SCATTERING DUE TO THE 777 1451 127 NUCLEAR COMPOUND PROCESS IS SMALL IN THE ENERGY RANGE ABOVE 3 777 1451 128 MEV, THE ANGULAR DISTRIBUTION OF ELASTIC SCATTERING NEUTRON 777 1451 129 WAS CALCULATED BY TAKING ONLY THE SHAPE ELASTIC SCATTERING INTO 777 1451 130 ACCOUNT ABOVE 3 MEV. 777 1451 131 5.2 INELASTICALLY SCATTERED NEUTRON, (N,2N),(N,3N),(N,N P), AND 777 1451 132 (N,N ALPHA) REACTION (MT=51,...,91, MT=16,17,22,23) 777 1451 133 NEUTRONS FROM THESE REACTIONS WERE ASSUMED TO BE ISOTROPIC IN 777 1451 134 THE CENTER OF MASS SYSTEM. 777 1451 135 6. FILE 5 (ENERGY DISTRIBUTION OF SECONDARY NEUTRONS) 777 1451 136 6.1 (N,2N), (N,3N), AND (N,N ) REACTIONS (MT=16,16,AND 91) 777 1451 137 THE ENERGY DISTRIBUTIONS OF NEUTRON FROM THE (N,2N), (N,3N) 777 1451 138 AND THE INELASTIC SCATTERING CROSS SECTION OF CONTINUUM PART WERE 777 1451 139 ASSUMED AS MAXWELLIAN. THE EFFECTIVE TEMPERATURE OF THESE 777 1451 140 MAXWELLIANS WERE OBTAINED BY THE WEISKOPF FORMULA. (26) 777 1451 141 1. J.L.COOK, AAEC/TM-549 (1969). 777 1451 142 2. D.W.BARR AND J.H.DEVANEY, LA-3643 (1967). 777 1451 143 3. R.J.HAYDEN, ET. AL., PHYS. REV. 75, 1500 (1949). 777 1451 144 4. W.H.WALKER, AECL-3037, PART I (1969). 777 1451 145 5. S.F.MUGHABGHAB, AND D.GARBER, BNL-325 THIRD EDIT. 777 1451 146 VOL 1. (1973). 777 1451 147 6. E.H.AUERBACH, BNL-6562 (1962). 777 1451 148 7. H.TAKAHASHI, EVALUATION OF THE NEUTRON AND GAMMA-RAY 777 1451 149 PRODUCTION CROSS SECTION FOR EU-151 AND EU-153 TO BE 777 1451 150 PUBLISHED AS BNL REPORT (1973). 777 1451 151 8. D.G.FOSTER JR., AND D.W.GLASGOW, PNWL UNPUBLISHED DATA (1966). 777 1451 152 9. T.LEWISE AND R.GRATZER, NUCL. PHYS. A162, 145 (1971). 777 1451 153 10. FAESLLER, NUCL. PHYS. 59, 1977 (1964). 777 1451 154 11. L.V.GROSHEV ET AL., NUCL. DATA TABLE A5, 1 (1968). 777 1451 155 12. D.J.HOREN ET AL., NUCLEAR LEVEL SCHEME A=45 THROUGH A=257, 777 1451 156 TO BE PUBLISHED IN NUCL. DATA TABLES. 777 1451 157 13. C.LEDERER, J.HOLLANDER AND I.PERLMAN, TABLE OF ISOTOPES, 777 1451 158 SIXTH EDITION (1967). 777 1451 159 14. C.DUNFORD, PRIVATE COMMUNICATION (COMNUC-3 CODE) (1971). 777 1451 160 15. C.DUNFORD, AI-AEC-12931 (1970). 777 1451 161 16. H.TAKAHASHI, GROGI-III, MODIFIED FROM GROGI-2. (17) 777 1451 162 17. J.GILAT, BNL-50246(T-580) (1969). 777 1451 163 18. J.COOK, H.FERGUSON AND A.MUSGROVE, AAEC/TM-392 (1967). 777 1451 164 19. A.GILBERT AND A.CAMERON, CAN. J. PHYS. 43, 1446 (1965). 777 1451 165 20. T.TAMURA, REV. MOD. PHYS. 37, 679 (1965). 777 1451 166 21. S.PEARLSTEIN, J. NUCL. ENER. 27, 81 (1973). 777 1451 167 22. F.CVELBAR, ET. AL., NIJS REPORT T-529 (1968). 777 1451 168 23. A.M.LANE AND J.E.LYNN, GENEVA CONFERENCE ON PEACEFUL USES OF 777 1451 169 ATOMIC ENERGY, 15, 4 (1958). 777 1451 170 24. G.E.BROWN, NUCL. PHYS. 57, 339 (1964). 777 1451 171 25. R.F.BERLAND, NAA-SR-11231 (1965). 777 1451 172 26. A.WEINBERG AND E.P.WIGNER, BOOK (1958). 777 1451 173 1 451 213 777 1451 174 1 457 5 777 1451 175 2 151 87 777 1451 176 3 1 418 777 1451 177 3 2 396 777 1451 178 3 3 85 777 1451 179 3 4 24 777 1451 180 3 16 9 777 1451 181 3 17 5 777 1451 182 3 22 7 777 1451 183 3 28 7 777 1451 184 3 51 17 777 1451 185 3 52 15 777 1451 186 3 53 14 777 1451 187 3 54 13 777 1451 188 3 55 11 777 1451 189 3 91 16 777 1451 190 3 102 68 777 1451 191 3 103 16 777 1451 192 3 104 12 777 1451 193 3 105 11 777 1451 194 3 106 5 777 1451 195 3 107 15 777 1451 196 3 251 21 777 1451 197 3 252 21 777 1451 198 3 253 21 777 1451 199 4 2 345 777 1451 200 4 16 10 777 1451 201 4 17 10 777 1451 202 4 22 10 777 1451 203 4 28 10 777 1451 204 4 51 10 777 1451 205 4 52 10 777 1451 206 4 53 10 777 1451 207 4 54 10 777 1451 208 4 55 10 777 1451 209 4 91 10 777 1451 210 5 16 7 777 1451 211 5 17 7 777 1451 212 5 91 7 777 1451 213 777 1 0 214 6.31540+ 4 1.52601+ 2 0 0 0 0 777 1457 215 2.71210+ 8 0.00000+ 0 0 0 4 2 777 1457 216 2.47000+ 5 0.00000+ 0 1.25000+ 6 0.00000+ 0 777 1457 217 6.31540+ 4 1.52600+ 2 0 0 6 1 777 1457 218 1.00000+ 0 0.00000+ 0 1.98000+ 6 0.00000+ 0 1.00000+ 0 0.00000+ 0 777 1457 219 777 1 0 220 777 0 0 221 6.31540+ 4 1.52601+ 2 0 0 1 0 777 2151 222 6.31540+ 4 1.00000+ 0 0 0 2 0 777 2151 223 8.89620- 1 6.00000+ 1 1 1 0 0 777 2151 224 3.00000+ 0 8.80000- 1 0 0 1 0 777 2151 225 1.52600+ 2 0.00000+ 0 0 0 432 72 777 2151 226 -1.00000- 2 3.00000+ 0 9.30020- 2 2.36500- 6 9.30000- 2 0.00000+ 0 777 2151 227 6.30950- 1 3.00000+ 0 9.30230- 2 2.32490- 5 9.30000- 2 0.00000+ 0 777 2151 228 1.14840+ 0 3.00000+ 0 9.16000- 2 5.99930- 4 9.10000- 2 0.00000+ 0 777 2151 229 1.55020+ 0 3.00000+ 0 9.64260- 2 4.26070- 4 9.60000- 2 0.00000+ 0 777 2151 230 2.05030+ 0 3.00000+ 0 9.75350- 2 5.35490- 4 9.70000- 2 0.00000+ 0 777 2151 231 2.92310+ 0 3.00000+ 0 9.60320- 2 3.23010- 5 9.60000- 2 0.00000+ 0 777 2151 232 4.59440+ 0 3.00000+ 0 1.19400- 1 3.96400- 4 1.19000- 1 0.00000+ 0 777 2151 233 6.30290+ 0 3.00000+ 0 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246 1.68320+ 1 3.00000+ 0 9.61620- 2 1.62310- 4 9.60000- 2 0.00000+ 0 777 2151 247 1.76180+ 1 3.00000+ 0 7.89640- 2 9.63710- 4 7.80000- 2 0.00000+ 0 777 2151 248 1.84290+ 1 3.00000+ 0 9.61590- 2 1.58980- 4 9.60000- 2 0.00000+ 0 777 2151 249 1.91970+ 1 3.00000+ 0 1.19240- 1 1.24400- 3 1.18000- 1 0.00000+ 0 777 2151 250 1.95680+ 1 3.00000+ 0 9.61470- 2 1.46770- 4 9.60000- 2 0.00000+ 0 777 2151 251 2.17780+ 1 3.00000+ 0 9.27710- 2 2.77140- 3 9.00000- 2 0.00000+ 0 777 2151 252 2.24840+ 1 3.00000+ 0 1.08240- 1 2.24260- 3 1.06000- 1 0.00000+ 0 777 2151 253 2.28180+ 1 3.00000+ 0 9.63190- 2 2.31920- 3 9.40000- 2 0.00000+ 0 777 2151 254 2.45820+ 1 3.00000+ 0 8.42120- 2 3.21220- 3 8.10000- 2 0.00000+ 0 777 2151 255 2.52010+ 1 3.00000+ 0 6.97820- 2 7.81790- 4 6.90000- 2 0.00000+ 0 777 2151 256 2.58260+ 1 3.00000+ 0 7.95360- 2 2.53620- 3 7.70000- 2 0.00000+ 0 777 2151 257 2.68540+ 1 3.00000+ 0 9.76770- 2 1.67720- 3 9.60000- 2 0.00000+ 0 777 2151 258 2.74540+ 1 3.00000+ 0 9.63700- 2 3.69800- 4 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